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611.
GPS掩星资料三维变分同化对台风模式预报的改进试验 总被引:1,自引:0,他引:1
本文尝试了GPSRO COSMIC资料在中尺度数值模式中的应用,利用COSMIC资料受云和降水影响较小,且有高数据精度、高垂直分辨率等优点,以改善模式初始场,进而提高预报准确度。模式采用中尺度气象模式WRF V3.0.1版本及其三维变分同化系统3DVAR,利用NCEP再分析资料、GTS资料和COSMIC资料对2009年第8号台风"莫拉克"登陆台湾岛前到登陆台湾岛的过程进行了模拟试验,并对温度、露点温度、对流有效位能等要素进行了诊断分析。试验结果表明:该项试验成功将COSMIC资料同化进模式,加深对"莫拉克"热力结构特征的了解,有效改善台风降水和路径预报,其中仅屏东县单点降水预报提高600 mm左右,24 h预报路径误差提高80 km以上。同时对提高台风强度预报起到积极作用。 相似文献
612.
N. Carrasco J. F. Doussin M. O’Connor J. C. Wenger B. Picquet-Varrault R. Durand-Jolibois P. Carlier 《Journal of Atmospheric Chemistry》2007,56(1):33-55
This article presents a complete study of the diurnal chemical reactivity of the biogenic volatile organic compound (BVOC), 2-methyl-3-buten-2-ol (MBO) in the troposphere. Reactions of MBO with OH and with ozone were studied to analyse the respective parts of both processes in the global budget of MBO atmospheric reactivity. They were investigated under controlled conditions for pressure (atmospheric pressure) and temperature (298 ± 2 K) using three complementary European simulation chambers. Reaction with OH radicals was studied in the presence of and in the absence of NO
x
. The kinetic study was carried out by relative rate study using isoprene as a reference. The rate constant found for this reaction was 366r011546/10874_2006_9041_Article_IEq1.gif" alt="$$k_{{{\text{MBO}} + {\text{OH}}}} = {\left( {5.6 \pm 0.6} \right)} \times 10^{{ - 11}} $$" align="middle" border="0"> molecule−1 cm3 s−1. FTIR spectroscopy, DNPH- and PFBHA-derivatisation analyses were performed for reactions with both OH radicals and ozone. In both reactions, the hydroxycarbonyl compound, 2-hydroxy-2-methylpropanal (HMPr) was positively identified and quantified, with a yield of 366r011546/10874_2006_9041_Article_IEq2.gif" alt="$$R_{{{\text{HM}}\Pr }} = 0.31 \pm 0.11$$" align="middle" border="0"> in the reaction with OH, and a yield of 366r011546/10874_2006_9041_Article_IEq3.gif" alt="$$R_{{{\text{HM}}\Pr }} = 0.43 \pm 0.12$$" align="middle" border="0"> and 0.84 ± 0.08 in the reaction with ozone under dry (HR < 1%) and humid conditions (HR = 20%–30%). A primary production of two other carbonyl compounds, acetone 366r011546/10874_2006_9041_Article_IEq4.gif" alt="$$R_{{{\text{acetone}}}} = 0.39 \pm 0.22$$" align="middle" border="0">, and formaldehyde 366r011546/10874_2006_9041_Article_IEq5.gif" alt="$$R_{{{\text{HCHO}}}} = 0.44 \pm 0.05$$" align="middle" border="0"> was found in the case of the dry ozonolysis experiments. Under humid conditions, only formaldehyde was co-produced with HMPr as a primary carbonyl compound, with a yield of 366r011546/10874_2006_9041_Article_IEq6.gif" alt="$$R_{{{\text{HCHO}}}} = 0.55 \pm 0.03$$" align="middle" border="0">. For the reaction with OH, three other carbonyl compounds were detected, acetone 366r011546/10874_2006_9041_Article_IEq7.gif" alt="$$R_{{{\text{acetone}}}} = 0.67 \pm 0.05$$" align="middle" border="0">, formaldehyde 366r011546/10874_2006_9041_Article_IEq8.gif" alt="$$R_{{{\text{HCHO}}}} = 0.33 \pm 0.08$$" align="middle" border="0"> and glycolaldehyde 366r011546/10874_2006_9041_Article_IEq9.gif" alt="$$R_{{{\text{glycolaldehyde}}}} = 0.78 \pm 0.20$$" align="middle" border="0">. In addition some realistic photo-oxidation experiments were performed to understand in an overall way the transformations of MBO in the atmosphere. The realistic photo-oxidation experiments were conducted in the EUPHORE outdoor simulation chamber. It was found that this compound is a weak secondary aerosol producer (less than 1% of the carbon balance). But it was confirmed that it is a potentially significant source of acetone, Δ[Acetone]/Δ[MBO] = 0.45. With our experimental conditions ([MBO]0 = 200 ppb, [NO]o = 50 ppb), an ozone yield of Δ[O3]/Δ[MBO] = 1.05 was found. 相似文献
613.
添加剂对KAlSi_3O_8-CaSO_4-CaCO_3体系反应表观活化能的影响 总被引:2,自引:0,他引:2
首先测定了KAlSi3O8-CaSO4-CaCO3体系在不同焙烧条件下钾长石转化成可溶性氧化钾的转化率,进而通过模拟计算表明:KAlSi3O8-CaSO4-CaCO3体系的固相扩散动力学过程符合金斯特林格动力学方程,反应表观活化能Ea为128.92kJ/mol。并着重考察了4种添加剂Na2SO4、Na2SO3、NaCl和NaF对KAlSi3O8-CaSO4-CaCO3体系的影响,结果表明:向体系中分别加入占反应物总质量3%的Na2SO4、Na2SO3、NaCl和1%的NaF后,体系的反应表观活化能Ea从原来的128.92kJ/mol依次下降至87.15、98.71、117.38和126.14kJ/mol,这表明4种添加剂中Na2SO4的效果最好,它能较大程度上降低反应表观活化能,从而降低反应温度和提高固相反应速率。 相似文献
614.
615.
针对中国一些沿海地区地下水超采及由此带来的海水入侵问题,将地表水补给、抽水量及地下水位等相嵌在一起,建立了沿海地区地下水模拟优化管理模型。将人工鱼群算法和基于MODFLOW2000的变密度地下水流及溶质运移模型耦合起来,对沿海地区地下水模拟优化管理模型进行求解。以山东省威海市节水示范区为例,验证模型的有效性和可靠性。结果表明,10、11、12月份抽水量最大,以后至第2年5月份依次是减少的;从区域分布上看,在临海区域1号井处抽水量是3500~1120m3/月,在其它井处是6540~2920m3/月;与现行方案相比,增加总有效供水1990m3,地下水平均水位升高0.29m,海水入侵问题能够得到解决。计算结果合理可行,为沿海地区地下水资源的科学管理和持续利用提供可靠依据。 相似文献
616.
617.
ULRICH HEIMHOFER DANIEL ARIZTEGUI MARC LENNIGER STEPHEN P. HESSELBO DAVID M. MARTILL ARISTOTELES M. RIOS‐NETTO 《Sedimentology》2010,57(2):677-694
The laminated limestones of the Early Cretaceous Crato Formation of the Araripe Basin (North‐eastern Brazil) are world‐famous for their exceptionally well‐preserved and taxonomically diverse fossil fauna and flora. Whereas the fossil biota has received considerable attention, only a few studies have focused on the sedimentary characteristics and palaeoenvironmental conditions which prevailed during formation of the Crato Fossil Lagerstätte. The Nova Olinda Member represents the lowermost and thickest unit (up to 10 m) of the Crato Formation and is characterized by a pronounced rhythmically bedded, pale to dark lamination. To obtain information on palaeoenvironmental conditions, sample slabs derived from three local stratigraphic sections within the Araripe Basin were studied using high‐resolution multiproxy techniques including detailed logging, petrography, μ‐XRF scanning and stable isotope geochemistry. Integration of lithological and petrographic evidence indicates that the bulk of the Nova Olinda limestone formed via authigenic precipitation of calcite from within the upper water column, most probably induced and/or mediated by phytoplankton and picoplankton activity. A significant contribution from a benthonic, carbonate‐secreting microbial mat community is not supported by these results. Deposition took place under anoxic and, at least during certain episodes, hypersaline bottom water conditions, as evidenced by the virtually undisturbed lamination pattern, the absence of a benthonic fauna and by the occurrence of halite pseudomorphs. Input of allochthonous, catchment‐derived siliciclastics to the basin during times of laminite formation was strongly reduced. The δ18O values of authigenic carbonate precipitates (between ?73;1 and ?53;1‰) point to a 18O‐poor meteoric water source and support a continental freshwater setting for the Nova Olinda Member. The δ13C values, which are comparatively rich in 13C (between ?03;1 and +13;9‰), are interpreted to reflect reduced throughflow of water in a restricted basin, promoting equilibration with atmospheric CO2, probably in concert with stagnant conditions and low input of soil‐derived carbon. Integration of lithological and isotopic evidence indicates a shift from closed to semi‐closed conditions towards a more open lake system during the onset of laminite deposition in the Crato Formation. 相似文献
618.
The Laverton region, located in the eastern Yilgarn Craton (EYC) Western Australia, is second only to the Kalgoorlie region for gold endowment. The integration of high-density, potential-field data, regional- and camp-scale seismic reflection data, regional- and mine-scale structural analysis, and geochronologically-constrained stratigraphy, provided new insights into the 4D architecture and tectonic evolution of Laverton region. 相似文献
619.
塔里木盆地寒武系层序地层格架 总被引:16,自引:0,他引:16
通过露头、钻测井及地震层序地层特征综合分析,建立了塔里木盆地寒武系三级层序地层格架,将寒武系划分出6个可全盆地追踪与对比的三级层序。结合反映全球海平面相对变化的全岩碳同位素旋回与反映沉积古水深相对变化的沉积旋回的对比分析,可将塔里木盆地寒武系三级层序分为主要受全球海平面变化控制形成的全球海平面层序(层序CSQ2、CSQ4、CSQ5、CSQ6)及主要受地区性构造沉降作用控制形成的构造层序(层序CSQ1、CSQ3)2类。塔北轮南地区寒武系台地边缘总体呈现由早寒武世的缓坡向中—晚寒武世的镶边台地的演变以及由西向东的进积叠置型式,推测主要与寒武纪全球海平面总体微弱下降及塔里木盆地基底沉降速率总体稳定且较小有关。 相似文献
620.