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951.
The Chengchao iron deposit,the largest high-grade skarn iron deposit in southeastern Hubei Province,contains considerable amounts of magnetite and by-product anhydrite.To obtain better understanding of the ore-formation process,this study carried out He-Ar-S-Pb multi-isotopic analyses on the pyrites formed during two stages of mineralization.The results indicate that the δ~(34)S values(ranging from 14.0‰ to 17.6‰) of pyrites formed from the two stages have no obvious differences,suggesting that they were not derived from a single magmatic sulfur source.The δ~(34)S values of anhydrite mostly range from 21.9‰ to 28.4‰,similar to that of the Middle Triassic sedimentary anhydrite in the Middle-Lower Yangtze River metallogenic belt(MLYRB).The Pb isotopic compositions of the pyrites of both stages are homogeneous,with values of ~(208)Pb/~(204)Pb,~(207)Pb/~(204)Pb,and~(206)Pb/~(204)Pb being 38.006-38.257,15.523-15.556,and 17.806-18.052,respectively,indicating a mixed crust-mantle source.The He-Ar results exhibit different compositions of the two stages:the ~3He/~4He(R/Ra) and ~(40)Ar/~(36)Ar values for the early-stage pyrite are 0.46-0.63 and 311-322,respectively,whereas the values for late-stage pyrite are 0.23-0.34 and 305-361,respectively.Both stages of pyrites indicate the multiple sources of the ore-forming fluids,with decreasing amount of magmatic water and increasing amount of modified meteoric water(MASW) during fluid evolution.The Triassic evaporites played an important role in the mineralization process. 相似文献
952.
953.
冲绳海槽中段表层沉积物物质来源的定量分离:Sr-Nd同位素方法 总被引:16,自引:2,他引:16
利用1994年85-904航次获取的冲绳海槽中段表层沉积物样品,测定其硅酸盐相的^87Sr/^86Cr和^143Nd/^144Nd比值,以定量研究冲绳海槽中段表层沉积物硅酸盐物质的来源,结果表明,冲绳海槽中段陆坡区表层沉积物硅酸盐相的^87Sr/^86Sr/^143Nd/^144Nd与东海陆架沉物硅酸盐相的^87Sr/^86Sr和^143Nd/^143Nd相当,槽底和东坡沉积物硅酸盐相的^87Sr/^86Cr和^143Nd/^144Nd值介于中国大陆硅酸盐物质和海槽水山碎屑的^87Sr/^86Sr,^143Nd/^144Nd比值之间,并大致具有两端员混合特征,利用以Sr同位素为参数的二端员混合方程进行物源定量分析的结果表明,冲绳海槽中段的西坡和槽底表层沉积物硅酸盐相以陆源物质为主,最大值为91.07%,由西向东,陆源物逐渐减少,在海槽东坡含量最小,最小值为9.93%,火山源物质在东坡含量最高,量大值为64.92%,由东向西,由北向东,火山源物质逐渐减少为零。 相似文献
954.
Tangential-flow ultrafiltration was used to isolate particulate and high-molecular-weight dissolved material from seawater collected at various depths and geographic regions of the Pacific and Atlantic Oceans. Ultrafiltration proved to be a relatively fast and efficient method for the isolation of hundreds of milligrams of material. Optical and electron microscopy of the isolated materials revealed that relatively fragile materials were recovered intact. Depth-weighted results of the size distribution of organic matter in seawater indicated that ˜ 75% of marine organic carbon was low-molecular-weight (LMW) dissolved organic carbon (< 1 nm), ˜ 24% was high-molecular-weight (HMW) dissolved organic carbon (1–100 nm), and ˜ 1% was particulate organic carbon (> 100 nm). The distribution of carbon in surface water was shifted to greater relative abundances of larger size fractions, suggesting a diagenetic sequence from macromolecular material to small refractory molecules. The average C:N ratios of particulate organic matter (POM) and HMW dissolved organic matter (DOM) were 7.7 and 16.7, respectively. Differences in C:N ratios between POM and HMW DOM were large and invariant with depth and geographic region, indicating that the aggregation of HMW DOM to form POM must be of minor significance to overall carbon dynamics. The stable carbon isotope composition (δ13C) of POM averaged −22.7%. in surface water and −25.2%. in subsurface water. Several possible explanations for the observed isotopic shift with depth were explored, but we were unable to discern the cause. The δ13C of HMW DOM samples was relatively constant and averaged −21.7%., indicating a predominantly marine origin for this material. The δ15N values of POM were highly variable (5.8–15.4%.), and the availability of nitrate in surface waters appeared to be the major factor influencing δ15N values in the equatorial Pacific. In the upwelling region nitrate concentrations were relatively high and δ15N values of POM were low, whereas to the north and south of the upwelling nitrate concentrations were low and δ15N values were high. The δ15N values of HMW DOM reflected the same trends observed in the POM fraction and provided the first such evidence for biological cycling of dissolved organic nitrogen (DON). Using the observed δ15N values and an estimate of meridional advection velocity, we estimated a turnover time of 0.3 to 0.5% day−1 for HMW DON. These results suggest a major role for DON in the upper ocean nitrogen cycle. 相似文献
955.
厦门湾水体中铀、钍同位素及悬浮颗粒物的粒径谱--颗粒物采集方法的影响 总被引:2,自引:0,他引:2
运用增强型混合纤雏素(CN-CA)膜、聚碳酸酯膜和聚丙烯滤芯过滤3种不同的方法采集、研究厦门湾水体中悬浮颗粒物(SPM)及其U、Th同位素的粒径谱.发现3种方法所得SPM总浓度和U、Th各同位素的总比活度具有很好的一致性,但粒级分布存在差异.SPM的浓度随粒径的增大而增加,并且SPM的粒径谱控制着颗粒活性很强的4种钍同位素的拉径谱.对于所研究的3种方法,采用聚碳酸脂膜过滤是研究沿岸海域SPM及颗粒活性核素粒级分布比较理想的方法。 相似文献
956.
Hodaka Kawahata Mayuri Inoue Masato Nohara Atsushi Suzuki 《Journal of Oceanography》2006,62(4):405-412
The δ18O, δ13C and trace element composition of pearls collected from Ago Bay, Japan, were investigated in order to evaluate biomineralization
in the cultured pearl oyster (Pinctada fucata martensii). The oxygen isotopic data suggest that the pearls were produced around 23–24°C, mainly in June to early July, which is consistent
with their occurrence in the field. Therefore the pearls were produced under or close to isotopic equilibrium conditions,
although they showed high calcification rates (higher than 0.2–1.0 g cm− 2yr−1) under which, for example, coral skeletons (calcification rate ∼0.28 g cm− 2yr−1) often show non-equilibrium isotope partitioning. The δ13C values were ∼− 2.9‰ lower than those calculated for offshore waters under equilibrium conditions. This may be due to low-δ13C bottom waters resulting from the degradation of organic matter (OM) or to a contribution of low-δ 13C food. In the latter case, a simple mass balance calculation gives a respiration component of 14%. Twelve trace elements
of bulk pearl samples were classified into four groups on the basis of their enrichment/depletion patterns relative to seawater
and inter-element relationships: group 1, Co, Cr, Pb; group 2, Ba, Cs, U; group 3, Cu, Sn, V, and group 4, Mn, Rb, Mo. Comparison
with coral skeletons suggests that Ba and Mn (groups 2 and 4) were definitely much enriched in proteinaceous OM relative to
aragonite crystals in pearls and that V (group 3) in pearls showed only slight enrichment in the organicrich layer. By contrast,
the other elements showed small differences between both layers (enrichment factor of <3), suggesting that these elements
occur largely in aragonite crystals. 相似文献
957.
对冲绳海槽Jade热液区块状硫化物中流体包裹体的氦、氖和氩同位素组成进行了测定,流体包裹体的3He/4He比值为(6.2~10.1)Ra,均值为7.8Ra,与大洋中脊玄武岩一致[3He/4He≈(6~11)Ra],20Ne/22Ne比值为10.7~11.3,明显高于大气值(9.8),而40Ar/36Ar比值的变化范围在287~334之间,接近大气值(295.5),这些结果表明,块状硫化物中热液流体捕获的稀有气体是地幔和海水源组分混合的产物,且流体包裹体中的氦主要来自地幔,氖和氩主要来自海水。 相似文献
958.
Distribution and sources of organic carbon, nitrogen and their isotopes in sediments of the subtropical Pearl River estuary and adjacent shelf, Southern China 总被引:17,自引:1,他引:17
The isotopic composition (δ13C and δ15N) and organic carbon (OC) and total nitrogen (TN, organic plus inorganic) content of 37 carbonate-free surficial sediments of the subtropical Pearl River estuary and the adjacent shelf of South China Sea (SCS) was determined. The δ13C values indicate that the sediment organic material is a mixture from two sources, terrestrial and marine. Several of the sediments have extremely low (< 4) OC / TN ratios, which could be due to low OC contents and/or to a significant fraction of the TN present as inorganic nitrogen adsorbed on clays. In general, the spatial patterns of OC, TN, δ13C and δ15N are similar. Values are low at the river mouth and on the western coast, suggesting proportionally greater accumulation of terrestrial particulate organic matter relative to marine phytodetritus, which is limited by low productivity in the turbid plume of the Pearl River. Algal-derived organic carbon (al-OC) content is estimated to be low (≤ 0.06%) at the river mouth and higher (up to 0.57%) on the adjacent inner shelf based on a mixing model of end members. 相似文献
959.
Ernesto Medina Marta Francisco Leonel Sternberg William T. Anderson 《Estuarine, Coastal and Shelf Science》2005,63(4):527-536
The 87Sr, 13C, and 15N isotopic signatures of organic matter in sediments from the continental shelf facing the Orinoco Delta were measured to determine the contribution of sediments transported from the Amazon River by the coastal Guayana current and the sediments transported by the Orinoco River. Box core samples between 60 and 300 m water depth collected along 4 transects located eastwards to the Orinoco Delta were analyzed. Carbon and nitrogen concentrations decreased with depth under water on the shelf, and were strongly correlated indicating homogeneity of organic matter composition. Phosphorus content was also associated to organic matter in most samples, but some of them revealed deposition of P-enriched sediments. The 87Sr/86Sr ratios showed a strong continental signature averaging 0.7117, therefore, limiting the possible carbon and nitrogen sources associated with these sediments to C3 trees, C4 grasses, or freshwater phytoplankton. The δ13C values were relatively high averaging −21‰, above values reported for sediments on the Amapá shelf and the Amazon River in Brazil. Average δ13C values did not differ significantly among transects. High δ13C values point to the influence of organic matter transported from the C4-plants dominated savannas in the northern fringe of the Orinoco River. δ15N values were positive and averaged 5‰, being within the range of values measured in the Marajo island (Amazon River) and the estuary of the Pará River. The δ15N values differed significantly among transects (4.9–5.2‰), lowest values corresponding to the northernmost transect near the coast of Trinidad, and the highest values corresponding to the transect located at the southernmost position. 相似文献
960.
南海沉积物中U,Th分布特征及其古环境意义 总被引:1,自引:0,他引:1
对采自南海深海中的两个柱样进行了分析。沉积速率分别为6.2cm·ka-1(317-82-25柱)和4.2cm·ka-1(90-37柱),均明显大于其他深海沉积速率,说明了南海这个边缘海的“放大效应”。此外,还分析了采自珠江口至外陆架的表层样,总结出从几元素在平面上的分布规律:从河口一陆架边缘~半深海,U,几含量的变化趋势均为多~少一多,Th/U比为小→大→小;而碳酸盐含量则显示出少→多→少的分布规律,即U,Th的含量与碳酸盐含量成反比,这可能是碳酸盐的所谓“稀释效应”所致。铀含量随柱样深度的变化曲线基本上与氧同位素曲线相吻合,其相关系数达0.67,证明U含量变化可能具有气候意义。Th的高含量点亦落在冷期之内。文中还探讨了水中铀的来源去向,说明了它能反映气候变化的原因。 相似文献