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The spatial distribution and source of arsenic, copper, tin and zinc within the surface sediments of the Fal Estuary, Cornwall, UK 总被引:2,自引:0,他引:2
Duncan Pirrie Matthew R. Power Gavyn Rollinson† G. Simon Camm Susan H. Hughes Alan R. Butcher‡ Peta Hughes‡ 《Sedimentology》2003,50(3):579-595
ABSTRACT Estuarine sediments commonly form major sinks for contaminants released during industrial activity. Many industrial processes lead to the release of metals initially in solution, which can then be adsorbed on to, for example, Fe hydroxides or clay minerals. However, in the mining industry, there are two major contaminant waste streams: (1) metals discharged in solution via mine drainage; and (2) particulate grains of the ore‐forming or related minerals released after ore processing. The release of particulate waste can have a major long‐term impact on environmental geochemistry. In this study, we have mapped the distribution of arsenic, copper, tin and zinc within the surficial sediments of the Fal Estuary, Cornwall, UK, an area that drains a historically important polymetallic mining district. There are clear spatial variations in the contaminants, with the highest levels (> 2800 p.p.m. As, > 5000 p.p.m. Cu, > 3000 p.p.m. Sn and > 6000 p.p.m. Zn) within Restronguet Creek on the western side of the estuary. Mineralogical studies show that small (< 20 µm) grains of detrital arsenopyrite, chalcopyrite, cassiterite and sphalerite are very abundant within the surface sediments. Most of the sulphide grains are fractured, but mineralogically unaltered, although some grains show alteration rims caused by oxidation of the sulphides. The geochemistry and mineralogy are indicative of sediment supply from the discharge of particulate waste into the estuary during historical mining activity. Subsequently, this particulate waste has been largely physically and biologically reworked within the surface sediments. Although considerable effort has been made to minimize contaminants released via mine drainage into the estuary, the potential flux of contaminants present within the intertidal and subtidal sediments has not been addressed. Benthic invertebrates living within the area have adapted to be metal tolerant, and it is likely that the dominant source of bioavailable metals is a result of alteration of the particulate mine waste present within the intertidal and subtidal sediments. 相似文献
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研究了硝酸钠-硫氰酸铵-罗丹明B-水液-固体系浮选分离锌的行为及其与常见离子分离的条件。结果表明,在NaNO3存在下,NH4SCN—RhB—Zn三元缔合物可浮于盐水相上形成界面清晰的液-固两相,从而使Zn^2 被定量浮选,而Cd^2 、Mn^2 、Al^2 、Ni^2 、Co^2 、Fe%2 等离子不被浮选。应用该方法对合成水样及加碘锌强化营养盐中微量锌进行了定量浮选分离测定,样品标准加入回收率为98.3%-101.8%。 相似文献
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Zeynep Özdemir 《Chemie der Erde / Geochemistry》2005,65(1):79-88
Soil and pine (Pinus brutia) samples were collected from 64 sites over chromite and ultramafic rocks near Musal?, and over clastic sediments of the Silifke-Anamur areas of Mersin, Turkey. Both sample media were analyzed for their Zn and Fe contents. The results showed similar concentration of both elements in the ash of needles and twigs, with each exhibiting lower concentration than the soils. Zinc was more concentrated in pines from the Silifke-Anamur area than at Musal?, but Fe concentrations were similar in both area. A positive correlation was observed between Zn and Fe in pine and soils (r=0.90 and 0.79, respectively). It is concluded that P. brutia can be used as a biogeochemical sample medium to detect concealed deposits of Zn and Fe. 相似文献
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Li Jianzhong Gansu Institute of Geology for Non-Ferrous Metals CNNC Lanzhou Gansu He Dianren North west Institute of Geology for Non-Ferrous Metals CNNC Xi''an Shaanxi Wu Jianmin Research Institute of Geology for Mineral Resources CNNC Guilin Guangxi 《《地质学报》英文版》1993,67(1)
Qinling-type Pb-Zn deposits are located in the Qinling fold belt, occurring in the fine-clastic and carbonate rocks of the Devonian marine facies. They are reformed sedimentary deposits originating from hydrothermal waters, and may be subdivided into 2 subtypes: hydrothermal sedimentary deposits (Changba subtype) and reformed hydrothermal sedimentary deposits (Bijiashan-Qiandongshan subtype). In comparison with some of the famous Palaeozoic Pb-Zn deposits in the world, the Qinling-type Pb-Zn deposits constitute an independent type, which possesses some characteristics of both hydrothermal sedimentary deposits (Meggen type) and reformed hydrothermal deposits (Mississippi Valley type). 相似文献
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This article presents the results of an experimental investigation on gas-phase coating of nanometer-sized NaCl aerosol particles with a condensing vapor of ZnCl2. The coating process has been carried out in a commercially available Venturi aspirator, where the NaCl at ambient temperature is mixed with the supersaturated ZnCl2 vapor. The operating conditions (ZnC12 vapor temperature, and ZnCl2/NaCl flow rate ratio) at which the ZnCl2 vapor preferentially nucleates onto the surface of the seed NaCl particles forming a coating layer on them, have been determined. Particle size growth as a function of the original seed diameter has also been determined. Smaller particles undergo a larger relative size growth ratio. It has also been shown that the presence of a coating layer does not affect the charge distribution of the original seed particles. 相似文献