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291.
I. E. Paukov N. K. Moroz Yu. A. Kovalevskaya I. A. Belitsky 《Physics and Chemistry of Minerals》2002,29(4):300-306
The heat capacity of paranatrolite and tetranatrolite with a disordered distribution of Al and Si atoms has been measured
in the temperature range of 6–309 K using the adiabatic calorimetry technique. The composition of the samples is represented
with the formula (Na1.90K0.22Ca0.06)[Al2.24Si2.76O10]·nH2O, where n=3.10 for paranatrolite and n=2.31 for tetranatrolite. For both zeolites, thermodynamic functions (vibrational entropy, enthalpy, and free energy function)
have been calculated. At T=298.15 K, the values of the heat capacity and entropy are 425.1 ± 0.8 and 419.1 ±0.8 J K−1 mol−1 for paranatrolite and 381.0 ± 0.7 and 383.2 ± 0.7 J K−1 mol−1 for tetranatrolite.
Thermodynamic functions for tetranatrolite and paranatrolite with compositions corrected for the amount of extraframework
cations and water molecules have also been calculated. The calculation for tetranatrolite with two water molecules and two
extraframework cations per formula yields: C
p
(298.15)=359.1 J K−1 mol−1, S(298.15) −S(0)=362.8 J K−1 mol−1. Comparing these values with the literature data for the (Al,Si)-ordered natrolite, we can conclude that the order in tetrahedral
atoms does not affect the heat capacity. The analysis of derivatives dC/dT for natrolite, paranatrolite, and tetranatrolite has indicated that the water- cations subsystem within the highly hydrated
zeolite may become unstable at temperatures above 200 K.
Received: 30 July 2001 / Accepted: 15 November 2001 相似文献
292.
293.
Abstract: Carbonate rocks of Cambrian (18 samples) and lower-middle Ordovician (11 samples) ages from South Korea were analyzed for sulfur contents of structurally substituted sulfate (SSS) and sulfides and their δ34 S values. The δ34 S values of SSS ranging from +25.9 to +45.2 permil, are averaged as +33.6 and +33.5 permil for the Cambrian and Ordovician rocks, respectively, which indicate high δ34 S values of the Cambro-Ordovician seawater. The SSS contents in the carbonate rocks are low being 2.9 to 17.3 ppm S (averaged as 7.0 ppm S). Sulfide sulfur, on the contrary, is much abundant containing 3 to 1,880 ppm S and the δ34 S values range widely between –17.6 and +31.1 permil. Sulfide sulfur of the studied rocks excluding impure carbonates has an average content of 187 ppm S and δ34 S value of +12.8 permil (n=24). The estimated δ34 S (sulfate–sulfide) values, which range from 13.8 to 25.4 permil in general with a few exceptions from 36.5 up to 52.3 permil for some impure carbonates, may provide evidence for the persistent oceanic anoxia with its temporary recovery during the Cambro-Ordovician time.
The SSS and sulfide sulfurs have often higher δ34 S values than the Mesozoic-Cenozoic ore sulfur (Ishihara et al., 2000). Since carbonate rocks are very reactive with circulating hydrothermal ore solution, high δ34 S values of the Korean ore deposits might be caused to some extent by 34 S enrichment from the host carbonates, resulting in the low SSS contents observed. 相似文献
The SSS and sulfide sulfurs have often higher δ
294.
295.
1 INTRODUCTION Extensive literature (Brown et al., 1985; Sawhney et al., 1981; Bierman and Swain, 1982; Connolly, 1980; Lopez-Avila and Hites, 1980; O扖onnor, 1988) described lots of sorbed pollutants or toxic substances in bed sediments of rivers, even after the effluent was halted for a long time. This is particularly true for hydrophobic organic compounds that can be sorbed on the particles and accumulated in the river bed sediments (Karickhoff et al., 1979). Pollution events of… 相似文献
296.
MODIFIED MASS FLUX CUMULUS CONVECTIVE PARAMETERIZATION SCHEME AND ITS SIMULATION EXPERIMENT—PART Ⅰ:MASS FLUX SCHEME AND ITS SIMULATION OF THE 1991 FLOOD EVENT*
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Based on the existing cumulus convective parameterization schemes,a mass flux scheme (MFS) for cumulus convective parameterization has been successfully developed by reference to the work of Chen et al. (1996).The MFS is a comprehensive scheme.In MFS,not only the importance of the large-scale moisture convergence is taken into account,but also it includes the cumulus updrafts and downdrafts,cumulus-induced subsidence in the environmental air.entrainment,detrainment and evaporation.The interaction between the cumulus and the environment is described by using a one-dimensional bulk model.At the same time the scheme includes the penetrative and shallow convections.The MFS has been successfully incorporated into the regional climate model RegCM2 developed by NCAR.The new model has been applied to simulate summer monsoon characteristics and their variations of heavy rainfall process in the Changjiang-Huaihe River Basins for three months from May to July 1991.The results show that the new model can successfully simulate this rainfall prolonged process.By comparising the model outputs of RegCM2.using the Kuo scheme and the MFS.it is found that the MFS is better in simulating the surface temperature,rainfall position and amount,and rainfall duration. 相似文献
297.
JIANG Guorong ZHANG Ren SHA Wenyu YAN Junyue YAO Huadong 《Acta Meteorologica Sinica》2002,16(1):123-132
In the context of tower measured radiation datasets.following the correction principle meeting a diagnostic equation in data quality control and in terms of a technique for model construction on data and ANN (artificial neural network) retrieval for BP correction of radiation measurements with rough errors available,a BP model is presented.Evidence suggests that the developed model works well and is superior to a convenient multivariate linear regression model,indicating its wide applications. 相似文献
298.
本文针对数字影像设备(如CT、MRI等)日益突出的图像存储和管理问题,进行深入的分析和研究。鉴于不同厂家和时期设备配置不同,提出了4种切实可行的解决方案:胶片扫描,视频采集,光盘或MOD输入,DICOM接口连接,完全解决了图像长期大量存储的问题。同时具有网络联机查询,图文报告,电子病历管理,激光相机接口等丰富的增值功能,是数字化医院的理想选择。 相似文献
299.
扩频通信技术是基于信息容量和信息传输差错概率理论而建立的先进的无线通讯方式、多次野外实地证实它具有抗干扰性强、可实现码分多址等优点。通过分析传输试验数据,我们有理由相信扩频通信技术在遥测地震台风中具有较高的应用和广阔的发展前景。 相似文献
300.
地震波传播算子的计算效率和精度是制约三维叠前深度偏移的关键因素. 广义屏传播算子(GSP, Generalized Screen Propagator)是一种在双域中实现的广角单程波传播算子. 这一方法略去了在非均匀体之间发生的交混回响,但它可以正确处理包括聚焦、衍射、折射和干涉在内的各种多次前向散射现象. 通过背景速度下的相移和扰动速度下的陡倾角校正,广义屏算子能够适应地层速度的强烈横向变化. 这种算子可以直接应用于炮集叠前偏移,通过将广义屏算子作用于双平方根方程,还可以获得一种高效率、高精度的炮检距域叠前深度偏移方法,用于二维共炮检距道集和三维共方位角道集的深度域成像. 本文首先简述了炮检距域广义屏传播算子的理论,进而讨论了共照射角成像(CAI, Common Angle Imaging)条件,由此给出各个不同照射角(炮检距射线参数)下的成像结果,进而得到共照射角像集. 由于照射角和炮检距的对应关系,共照射角像集又为偏移速度分析和AVO(振幅随炮检距变化)分析等提供了有力工具. 相似文献