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991.
文章通过对某地低品位软锰矿的试验研究 ,采用直接浸出工艺流程 ,可获得较好技术指标的硫酸锰产品 ,为同类型锰矿的开发利用进行了有益探索。 相似文献
992.
Sequential chemical extraction procedure has been widely used to partition particulate trace metals into vari-ous fractions and to describe the distribution and the statue of trace metals in geo-environment.One sequential chemical extraction procedure was employed here to partition various fractions of Mn in soils.The experiment was designed with quality controlling concept in order to show sampling and analytical error.Experimental results obtained on duplicate analy-sis of all soil samples demonstrated that the precision was less than 10%(at 95% confidence level).The accuracy was estimated by comparing the accepted total concentration of Mn in standard reference materials (SRMs) with the measured sum of the individual fractions.The recovery of Mn from SRM1 and SRM2 was 94.1% and 98.4%,respectively.The detection limit,accuracy and precision of the sequential chemical extraction procedure were discussed in detailed.All the results suggest that the trueness of the analytical method is satisfactory. 相似文献
993.
Karina?L.?LecomteEmail author Andrea?I.?Pasquini Pedro?J.?Depetris 《Aquatic Geochemistry》2005,11(2):173-194
By means of PHREEQC inverse modeling, we have simulated the weathering reactions in Los Reartes River, a mountainous (2400–670 m a.s.l.) drainage basin from the Sierras Pampeanas of Córdoba, Argentina, analyzing the effect of lithology, relief, and climate. The steep upper half of the basin (slopes > 20) is occupied by exposed granite; the remaining area is mostly metamorphic, with cropping out gneisses and progressively decreasing slopes (< 6). Climate is semihumid to semiarid; rainfall mainly occurs in summer and decreases with decreasing height. PHREEQC inverse models developed using water chemical data showed that (a) oligoclase was the major supplier of solutes, while the main precipitated phase was kaolinite in the granite domain; (b) muscovite is the chief supplier of solutes and illite is the main precipitated phase in the gneissic realm; (c) the steeper portions of the metamorphic reach are less crucial in supplying solutes than the lower ones, thus highlighting the importance of the water residence time in the kinetics of dissolution; (d) in the driest time of the year (winter, 20 mm/month) we registered the highest production of dissolved and precipitated phases; fluxes (mmol/month), however, are higher at the end of the rainy season; (e) CO2 consumption is important all along the Los Reartes drainage basin and, in terms of mmol/kg H2O, the lowermost portion of the basin is the most significant supplier; (f) CO2 accounts for over 50 of all the species involved in the weathering reactions occurring at the Los Reartes drainage basin. 相似文献
994.
Art F. White Marjorie S. Schulz Davison V. Vivit Alex E. Blum David A. Stonestrom 《Journal of Geochemical Exploration》2006,88(1-3):363
Spatial and temporal variations in pore water compositions are characterized for a deep regolith profile developed on a marine terrace chronosequence near Santa Cruz California. Variations are resolved in terms of the dominance of either a lithogenic process, i.e. chemical weathering, or a biogenic process, i.e. plant nutrient cycling. The concept of elemental fractionation is introduced describing the extent that specific elements are mobilized and cycled as a result of these processes. 相似文献
995.
The relative weathering of a sequence of five palaesols formed in different parent materials, including bedrock of phonolitic composition, is described and assessed. The three lower palaeosols (units 3–5) are considered to be of interglacial origin. The saprolite (unit 5), in phonolite, formed prior to deposition of the lower Brunhes-age till, is considered to be as old as the Brunhes Matuyama boundary (0.73 myr). The other two palaeosols in this group (units 3 and 4), derived from loess and till, respectively, formed over middle to late Brunhes time under palaeoclimates that were wetter (and presumably warmer), and of sufficient leaching power to move clay, as well as organically complexed extractable Fe and Al. The palaeosols in unit 3 are more complex than the lower ones. Their upper and lower horizons have about the same chemical composition as the lowest two palaeosols, while the middle horizons are similar to the upper two palaeosols (units 1 and 2). Radiocarbon dates for unit 3 are considered to be too young to account for the strong weathering in the upper and lower horizons. This interpretation is supported by high D/L ratios of aspartic acid. Overlying sediments, emplaced by episodic colluvial (unit 2) and slope wash (unit 1) processes, are less weathered; the lower colluvial unit in this group was emplaced during the late stade of the last glaciation. The surface sediments were emplaced more recently during the same interval and weathered mainly during the post-glacial period. Tentative correlations with core 82PCS18 from the Canary Basin show that upper unit 3 is probably equivalent to Isotope Stage 5e, lower unit 3 to Isotope Stage 7, unit 4 to Isotope Stage 8, and unit 5 to Isotope Stage 9. Units 1 and 2 are firmly correlated with Isotope Stage 2. 相似文献
996.
M. A. Romanova 《Mathematical Geology》1991,23(7):959-979
A hypothesis for effects of stable tectonic elements on chemical composition of Mesozoic granitoids in northeastern Asia is tested. Chemical compositional change of granitoid rocks is examined in nine-dimensional space of rock-forming oxides. Stable geologic structures of the region are outlined by trends of Euclidean distances between rock recognized as a standard in a space of major rock-forming oxides and composition of individual samples. A data-smoothing polynomial of the fourth order corresponds closely to the geology of the region. Chemically stable masses of quartz diorite are thought to be delivered directly from magmatic sources along deep faults. A great variety of acidic granites, which occupy for each analysis separate cells in the nine-dimensional classification, are presumed to be palingenetic in origin. 相似文献
997.
A numerical method for the calculation of equilibrium distributions of chemical species in aqueous solutions of electrolytes is presented. This method is constructed by transforming the problem of determining the set of unknown concentrations satisfying the mass balance and mass action equations into the equivalent problem of finding the limits of certain well-behaved mathematical sequences in a multivariable direct iteration scheme. The total (analytical) concentrations are taken as the starting estimates, and the recursive equations are constructed from the starting equations. It is shown that the sequences so constructed are both monotonic and bounded, hence convergent in an orderly fashion by a mathematical axiom. Each unknown free ion concentration (that is, each limit) is approached simultaneously from above and from below, being effectively sandwiched in an ever tightening manner. Strict error bounds therefore are easily constructed. The method has been found to be exceedingly efficient in practice, with the error bound (maximum fractional error in taking the upper estimate as the final answer) decreasing in an approximately exponential fashion with respect to iteration number, commonly 0.5–1.5 orders of magnitude per iteration. Correction for nonideality is presented, and the possibility of this giving rise to more than one solution is discussed in connection with three examples of natural waters of low-, medium-, and high-ionic strengths. 相似文献
998.
Astrid Holstad 《Computational Geosciences》2000,4(2):103-139
We formulate mathematical and numerical models for multispecies, multi-phase and non-isothermal reactive fluid flow in porous
media focusing on the chemical reactions and the transport of solutes. Mass conservation and stability in the time integration
are emphasized. We use cell-centered finite volume differencing in space and an implicit Runge-Kutta method in time. Assuming
two space dimensions, we introduce flux approximation for arbitrarily shaped convex quadrilaterals. On equidistant and variable
sized rectangular grids we choose limited κ=
related schemes to approximate the advective flux and the central difference scheme for the diffusive flux. On non-rectangular
grids we recommend the VF9 scheme for the estimation of the diffusive flux. Our model exists as a code.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
999.
1000.