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61.
62.
高岭石插层复合物作为新型矿物材料现已被广泛应用。然而,插层复合物热稳定性较难控制使其在聚合物中的应用一直受到限制。本文应用热分析、X射线衍射、质谱及发射红外光谱等表征技术对煤系高岭石/醋酸钾插层复合物受热分解产物及微结构变化进行了研究。结果表明,煤系高岭石/醋酸钾插层复合物热相变主要经历以下几个阶段:插层水脱嵌(约350℃),插层剂醋酸钾脱嵌(约400℃),脱羟基(约450℃),偏高岭石形成(450~550℃),KHCO3出现(约600℃),KHCO3热分解形成K2CO3和KAl Si O4出现(约700℃),热解产品K2Al2Si O4出现(约800℃),K4Al2Si2O3出现(900~1000℃),大量K3Al O3形成阶段(1100℃及以上)。此外,还发现通过控制插层率和加热温度,可实现高岭石插层复合物的可控分解、新物相合成与转变,从而有利于新材料的合成。 相似文献
63.
为探讨更新世以来河北平原东部植被演化和气候变化特征,研究分析了大厂凹陷S9钻孔的孢粉植物群。根据S9钻孔中孢粉的分布,自下而上划分了6个孢粉组合,组合I和组合II为以针叶树为主的针阔叶混交林,组合IV—IV为疏林草原植被,整体为稀树草原型植被环境。根据孢粉组合的变化特征,还原了研究区更新世以来的气候变化规律: 研究区在早更新世气候温暖半干旱; 中更新世早期气候变冷,之后气候总体呈变暖变干旱的趋势; 晚更新世早期气候持续变暖,由湿润向干旱转变。研究区的孢粉演化模式与我国中北部许多地区的植被演化模式相似,同时与东亚、北太平洋以及南半球的气候变化特征表现出了较好的一致性。 相似文献
64.
65.
Constancy in predator/prey ratio (PPR) is a controversial issue in ecological research. Published reports support both constancy and inconstancy of the ratio in animal communities. Only a few studies, however, specifically address its course through time. Here we study the course of predator/prey ratio in communities of large Plio-Pleistocene mammals in Italy. After controlling for taphonomic biases, we find strong support for PPR inconstancy through time. Extinction, dispersal events, and differences in body size trends between predators and their prey were found to affect the ratio, which was distributed almost bimodally. We suggest that this stepwise dynamic in PPR indicates changes in ecosystem functioning. Prey richness was controlled by predation when PPR was high and by resources when PPR was low. 相似文献
66.
In marine strata from Sinian to Middle Triassic in South China, there develop four sets of regional and six sets of local
source rocks, and ten sets of reservoir rocks. The occurrence of four main formation periods in association with five main
reconstruction periods, results in a secondary origin for the most marine gas pools in South China. To improve the understanding
of marine gas pools in South China with severely deformed geological background, the dominant control factors are discussed
in this paper. The fluid sources, including the gas cracked from crude oil, the gas dissolved in water, the gas of inorganic
origin, hydrocarbons generated during the second phase, and the mixed pool fluid source, were the most significant control
factors of the types and the development stage of pools. The period of the pool formation and the reconstruction controlled
the pool evolution and the distribution on a regional scale. Owing to the multiple periods of the pool formation and the reconstruction,
the distribution of marine gas pools was complex both in space and in time, and the gas in the pools is heterogeneous. Pool
elements, such as preservation conditions, traps and migration paths, and reservoir rocks and facies, also served as important
control factors to marine gas pools in South China. Especially, the preservation conditions played a key role in maintaining
marine oil and gas accumulations on a regional or local scale. According to several dominant control factors of a pool, the
pool-controlling model can be constructed. As an example, the pool-controlling model of Sinian gas pool in Weiyuan gas field
in Sichuan basin was summed up. 相似文献
67.
In this study are discussed new SEM-EDS analyses performed on glass shards from five cores collected in the Central Adriatic Sea and two cores recovered from the South Adriatic Sea. A total of 26 tephra layers have been characterized and compared with the geochemical features of terrestrial deposits and other tephra archives in the area (South Adriatic Sea and Lago Grande di Monticchio, Vulture volcano). The compositions are compatible with either a Campanian or a Roman provenance. The cores, located on the Central Adriatic inner and outer shelf, recorded tephra referred to explosive events described in the literature: AP3 (sub-Plinian activity of the Somma-Vesuvius, 2710 ± 60 14C years BP); Avellino eruption (Somma–Vesuvius, 3548 ± 129 14C years BP); Agnano Monte Spina (Phlegrean Fields, 4100 ± 400 years BP); Mercato eruption (Somma–Vesuvius, 8010 ± 35 14C years BP; Agnano Pomici Principali eruption (Phlegrean Fields, 10,320 ± 50 14C years BP); Neapolitan Yellow Tuff (Phlegrean Fields, 12,100 ± 170 14C years BP). Some of these layers were also observed in the South Adriatic core IN68-9 in addition to younger (AP2, sub-Plinian eruption, Somma–Vesuvius, 3225 ± 140 14C years BP), and older layers (Pomici di Base eruption, Somma–Vesuvius, 18,300 ± 150 14C years BP). Significant is the tephra record of core RF95-7 that, for the first time in the Adriatic Sea, reports the occurrence of tephra layers older than 60 ka: the well known Mediterranean tephra layers X2 (ca. 70 ka), W1 (ca. 140 ka) and V2 (Roman origin, ca. 170 ka) as well as other tephra layers attributed, on the basis of geochemistry and biostratigraphy, to explosive eruptions occurred at Vico (138 ± 2 and 151 ± 3 ka BP) and Ischia (147–140 ka BP). 相似文献
68.
The sensitive and selective determination of polyalcohols without chromophores or fluorophores in the lower ppb-level is still an analytical task of high interest, especially in the field of environmental investigations. This paper describes a cation-exchange HPLC procedure for the separation and fluorescence detection of two quaternary ammonium compounds with polyalcoholic groups (degradation products of fabric softener) after derivatization with 9-fluorenylmethyl chloroformate (FMOC). Detailed experiments were carried out to determine optimum reaction conditions (pH, reaction time, temperature), linear range, detection limits, and kinetics of the reaction. The HPLC separation on a cation-exchange column includes a gradient program which provides complete separation from neutral compounds also reacting with FMOC and its hydrolysis products formed during the reaction in alkaline medium. High specificity for both investigated ammonium compounds with detection limits in the range of 1 ppb could be achieved. 相似文献
69.
The structural activities took place extensively in the Asia continent during the Cenozoic era owing to the strong continent-to-continent
collision and continuous compression between the India Plate and the Eurasia Plate. Huang Jiqing called such structural activities
Himalayan movement. China’s sedimentary basins developed and took shape mainly during the Himalayan movement period. It is
also the main period for formation and development of the oil and gas reservoirs. Of 366 large and medium-sized oil and gas
fields currently found in China, 212 reservoirs were formed in the Neogene-Quaternary period. The proportion is as high as
68.2%. The oil and gas migration and accumulation in the latest geological period, which were controlled by the times, properties,
styles and strength of the Himalayan movement, took place mainly in eight regions, such as the low uplift area of Bohai Sea,
the onshore faulted sag area of Bohai Bay, anticlinorium zone in Daqing, the foreland fold-and-thrust belt in West China,
the tilted structural zone in West China, the cratonic palaeohigh in the Tarim Basin, the zone of fault and fold belt in the
East Sichuan Basin, and the biological gas zone in the East Qaidam Basin. The oil and gas pool formations in those regions
have their own characteristics. With the great potential and broad prospect, those regions are the main exploration areas
in China in the future. 相似文献
70.
Abstract The late Quaternary calcareous nannofossil assemblages from Ocean Drilling Program Holes 807A and 846B, located in the western and eastern equatorial Pacific Ocean, respectively, were analyzed to clarify changes in surface-water conditions during the last 500 000 years. The uppermost Quaternary sediments in both holes contain abundant nannofossils, and their assemblages are characterized by high species diversity. The absolute abundances of coccoliths (specimens/g) and relative numbers of small reticulofenestrids decreased drastically in both holes between 0.3 and 0.2 Ma, whereas the relative abundance of warm-water species and Florisphaera profunda increased suddenly at this time. These data indicate that upwelling around the western and eastern equatorial Pacific regions weakened after 0.2 Ma, which was caused by a decrease in trade-wind strength. 相似文献