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51.
The electrical aerosol spectrometer (EAS) of the parallel measuring principle at Tartu University is an efficient instrument for rapid measurement of the unstable size spectrum of aerosol particles. The measuring range from 10 nm to 10 μm is achieved by simultaneously using a pair of differential mobility analyzers with two different particle chargers. The particle spectrum is calculated and measurement errors are estimated in real time by using a least-squares method. Experimental calibration ensures reliability of measurement. The instrument is well suited for continuous monitoring of atmospheric aerosol. 相似文献
52.
Mass size distribution of the crustal elements (Al, Ca, Fe, Mg, Si, Ti), anthropogenic elements (Zn, Mn, Cr, Cu, K, P, Pb) and sea elements (Na, Cl) were obtained from measurements carried out with an inertial cascade impactor in Sfax. A fitting procedure by data inversion was applied to those data. This procedure yields accurate size distributions of aerosols in the diameter range 0.1–25 μm in two different sites. In a coastal industrial site, the mass distribution of the aerosol showed a bimodal structure; and in urban area, the lower particle mode cannot be observed. The elemental dry deposition flux was calculated as a function of particle size. The element flux size distribution increased rapidly with particle size. The modelling results indicate that the majority of the crustal and anthropogenic elements flux (>90%) was due to particles larger than 3 μm in diameter. 相似文献
53.
Mark E. Hodson 《Chemical Geology》2002,190(1-4):91-112
Far-from-equilibrium batch dissolution experiments were carried out on the 2000–500, 500–250, 250–53 and 53–2 μm size fractions of the mineral component of the B horizon of a granitic iron humus podzol after removal of organic matter and secondary precipitates. The different size fractions were mineralogically and chemically similar, the main minerals present being quartz, alkali and plagioclase feldspar, biotite and chlorite. Specific surface area increased with decreasing grain size. The measured element release rates decreased in the order 53–2>>>2000–500>500–250>250–53 μm. Surface area normalised element release rates from the 2000–500, 500–250 and 250–53 μm size fractions (0.6–77×10−14 mol/m2/s) were intermediate between literature reported surface area normalised dissolution rates for monomineralic powders of feldspar (0.1–0.01×10−14 mol/m2/s) and sheet silicates (100×10−14 mol/m2/s) dissolving under similar conditions. Element release rates from the 53–2 μm fraction (400–3000×10−14 mol/m2/s) were a factor of 4–30 larger than literature reported values for sheet silicates. The large element release rate of the 53–2 μm fraction means that, despite the small mass fraction of 53–2 μm sized particles present in the soil, dissolution of this fraction is the most important for element release into the soil. A theoretical model predicted similar (within a factor of <2) bulk element release rates for all the mineral powders if observed thicknesses of sheet silicate grains were used as input parameters. Decreasing element release rates with decreasing grain size were only predicted if the thickness of sheet silicates in the powders was held constant. A significantly larger release rate for the 53–2 μm fraction relative to the other size fractions was only predicted if either surface roughness was set several orders of magnitude higher for sheet silicates and several orders of magnitude lower for quartz and feldspars in the 53–2 μm fraction compared to the other size fractions or if the sheet silicate thickness input in the 53–2 μm fraction was set unrealistically low. It is therefore hypothesised that the reason for the unpredicted large release rate from the 52–3 μm size fraction is due to one or more of the following reasons: (1) the greater reactivity of the smaller particles due to surface free energy effects, (2) the lack of proportionality between the BET surface area used to normalise the release rates and the actual reactive surface area of the grains and, (3) the presence of traces quantities of reactive minerals which were undetected in the 53–2 μm fraction but were entirely absent in the coarser fractions. 相似文献
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两个冰期-间冰期旋回的黄土记录及其古气候意义 总被引:9,自引:14,他引:9
北京邻区枣沟、斋堂和赤峰黄土-古土壤剖面粒度和磁化率变化在幅度和相位上都有明显的差异。在两个冰期-间冰期旋回,磁化率记录具有冰量变化模式,而粒度记录具有轨道周期特点,粒度和磁化率之间的相位关系在从冰期向间冰期转换和冰期向间冰期过渡的过程中,既有滞后也有超前的表现,很难单纯以成土作用来解释。由于黄土粒度主要反映粉尘源区环境和古风场强度的变化,而磁化率主要记录的是沉积区的成壤作用,反映夏季风的强度变化,因此剖面粒度和磁化率变化的不协调说明古风场和粉尘源区变化与粉尘沉积区气候变化之间不统一。这可能意味着控制夏季风强度变化和控制冬季风强度变化的机制存在差异。 相似文献
57.
坝上高原安固里淖粒度年纹层与环境变化 总被引:9,自引:2,他引:9
在安固里淖湖心区获取一未扰动沉积物样柱,分析发现了由冬季风搬运物与湖心沉积共同形成的粒度年纹层,建立了纹层年表,恢复了安固里淖湖区8507aB.P,以来的环境变化过程。8507-5429aB.P。冬季风活动较弱,后期的所波动;5429-3244aB.P.冬季风活动较强,3244-2494aB.P。冬季风活动减弱;2494-1165aB.P。冬季风活动略有增强;1165aB.P以来,冬季风活动减弱。安固里小淖粒度年纹层反映的冬季风变化情况与我国北方地区同期的环境变化和海平面变化有很好的对应关系。 相似文献
58.
黄河中游降雨特性对泥沙粒径的影响 总被引:6,自引:3,他引:6
以黄河中游36个有泥沙粒径资料的水文测站流域为样本,在不同自然地理类型流域划分的基础上,建立了流域泥沙粒径特片与降雨特性的关系。结果表明,在不同类型流域,流域泥沙的粗细与降雨季节性变率和年际变率之间存在着相当好的线性正相关关系;而与年降雨量和降雨不均匀系数之间呈明显的非线性关系。流域地面物质、植被和地貌发育程序等下垫面环境因素对泥沙粒径特性与降雨特性之间关系起着十分重要的控制作用。不同类型流域曲线的斜率各不相同,在图中所处的位置也不相同。 相似文献
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60.
辽南滨海黄土粒度环境信息高分辨率研究 总被引:11,自引:1,他引:11
对辽南滨海黄土粒度研究证明 ,滨海黄土是在第四纪冰期寒冷气候下的产物 ,但是 ,由于滨海黄土所处靠近沿海的地理位置使得这种黄土的形成机制具有独特性。冰期时渤海湾西岸海面下降出露的冲洪积物和海底砂是滨海黄土除西北内陆地区以外的另一重要物源 ,搬运以风砂跃移方式进行。滨海黄土的粒度中包涵了丰富的有关渤海湾海面变化的信息。辽南滨海黄土剖面中的粒度拟合值、 2 - 3Ф粒级百分含量反映了渤海的海退、海侵过程和末次冰期蒙古高压的强弱 ,这种变化与滨海黄土 3个孢粉组合带所反映的古气候环境相吻合 ,同邻近地区的海面升降变化和深海岩芯氧同位素阶段也存在良好的对应关系 ,滨海黄土粒度的拟合度是本区古环境变化的重要的替代指标。 相似文献