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11.
Th sorption and export models in the water column: A review 总被引:2,自引:3,他引:2
Nicolas Savoye Claudia Benitez-Nelson Adrian B. Burd J. Kirk Cochran Matthew Charette Ken O. Buesseler George A. Jackson Matthieu Roy-Barman Sabine Schmidt Marc Elskens 《Marine Chemistry》2006,100(3-4):234
Over the past few decades, the radioisotope pair of 238U / 234Th has been widely and increasingly used to describe particle dynamics and particle export fluxes in a variety of aquatic systems. The present paper is one of five review articles dedicated to 234Th. It is focused on the models associated with 234Th whereas the companion papers (same issue) are focused on present and future methodologies and techniques (Rutgers van der Loeff et al.), C / 234Th ratios (Buesseler et al.), 234Th speciation (Santschi et al.) and present and future applications of 234Th [Waples, J.T., Benitez-Nelson, C.R., Savoye, N., Rutgers van der Loeff, M., Baskaran, M., Gustafsson, Ö., this issue. An Introduction to the application and future use of 234Th in aquatic systems. Marine Chemistry, FATE special issue]. In this paper, we review current 234Th scavenging models and discuss the relative importance of the non-steady state and physical terms associated with the most commonly used model to estimate 234Th flux. Based on this discussion we recommend that for future work the use of models should be accompanied by a discussion of the effect that model and data uncertainty have on the model results. We also suggest that future field work incorporate repeat occupations of sample sites on time scales of 1–4 weeks in order to evaluate steady state versus non-steady state estimates of 234Th export, especially during high flux events (> ca. 800 dpm m− 2 d− 1). Finally, knowledge of the physical oceanography of the study area is essential, particularly in ocean margins and in areas of established upwelling (e.g., Equatorial Pacific). These suggestions will greatly enhance the application of 234Th as a tracer of particle dynamics and flux in more complicated regimes. 相似文献
12.
13.
气相色谱指纹法在海上油污染源鉴别中的应用 总被引:4,自引:0,他引:4
通过一个具体案例,探讨了气相色谱指纹法在海上油污染源鉴别中的应用。该鉴别方法基于样品的正构烷烃气相色谱指纹分析,选择既能表征油种固有特性,又受风化影响较小的正十七烷(n-C17)、正十八烷(n-C18)、姥鲛烷(phy)、植烷(phy)和正二十烷(n-C20)等特征烷烃作为判据,可信度大,而且整个操作流程短(一般不超过半天),较简便易行。 相似文献
14.
15.
塔河油田2区三叠系油藏是西北分公司开发较早的碎屑岩油藏之一,开发层系有上油组、中油组,油柱高度在15~20m,储层为辫状三角洲相辫状三角洲前缘亚相水下分流河道、河口坝、分流间湾微相沉积,非均质性严重。本区上油组砂体厚度40~0m,中油组25~35m,分布较稳定,物性为中孔、中高渗储层,原油属低粘度轻质油。但2区三叠系油藏实钻变化大,见水快、产量递减快、含水上升快、采出程度低,开发效果较差,经过多次调整虽有一定程度改善,仍存在一些问题。本文认为2区三叠系油藏开发效果较差的原因之一是对本区油藏类型的认识上存在问题即2区三叠系油藏是以断裂控制的断块油藏而非背斜油藏,并延伸分析正在投入开发评价的S96-T901井区、TK232-T453井区及T206-T208井区等都为断块(断背斜)油藏。应用断块油藏的观点对塔河地区三叠系油藏勘探开发有重要指导意义。 相似文献
16.
Changing grading of soil: effect on critical states 总被引:6,自引:3,他引:3
Examples of situations are presented where the grading of a soil changes during its lifetime either by crushing of particles
leading to an increase of fine material or by slow transport of fine particles with seepage leading to a decrease of fine
material. Such grading changes influence the basic constitutive properties of the soil, in particular properties such as critical
states which are dependent on the available range of densities of packing. Discrete element modelling is used to show the
dependence of critical state conditions on grading and the way in which the particle assembly seeks out new critical state
conditions as the grading changes. 相似文献
17.
The petroleum generation potential and effective oil window of humic coals related to coal composition and age 总被引:1,自引:0,他引:1
A worldwide data set of more than 500 humic coals from the major coal-forming geological periods has been used to analyse the evolution in the remaining (Hydrogen Index, HI) and total (Quality Index, QI) generation potentials with increasing thermal maturity and the ‘effective oil window’ (‘oil expulsion window’). All samples describe HI and QI bands that are broad at low maturities and that gradually narrow with increasing maturity. The oil generation potential is completely exhausted at a vitrinite reflectance of 2.0–2.2%Ro or Tmax of 500–510 °C. The initial large variation in the generation potential is related to the original depositional conditions, particularly the degree of marine influence and the formation of hydrogen-enriched vitrinite, as suggested by increased sulphur and hydrogen contents. During initial thermal maturation the HI increases to a maximum value, HImax. Similarly, QI increases to a maximum value, QImax. This increase in HI and QI is related to the formation of an additional generation potential in the coal structure. The decline in QI with further maturation is indicating onset of initial oil expulsion, which precedes efficient expulsion. Liquid petroleum generation from humic coals is thus a complex, three-phase process: (i) onset of petroleum generation, (ii) petroleum build-up in the coal, and (iii) initial oil expulsion followed by efficient oil expulsion (corresponding to the effective oil window). Efficient oil expulsion is indicated by a decline in the Bitumen Index (BI) when plotted against vitrinite reflectance or Tmax. This means that in humic coals the vitrinite reflectance or Tmax values at which onset of petroleum generation occurs cannot be used to establish the start of the effective oil window. The start of the effective oil window occurs within the vitrinite reflectance range 0.85–1.05%Ro or Tmax range 440–455 °C and the oil window extends to 1.5–2.0%Ro or 470–510 °C. For general use, an effective oil window is proposed to occur from 0.85 to 1.7%Ro or from 440 to 490 °C. Specific ranges for HImax and the effective oil window can be defined for Cenozoic, Jurassic, Permian, and Carboniferous coals. Cenozoic coals reach the highest HImax values (220–370 mg HC/g TOC), and for the most oil-prone Cenozoic coals the effective oil window may possibly range from 0.65 to 2.0%Ro or 430 to 510 °C. In contrast, the most oil-prone Jurassic, Permian and Carboniferous coals reach the expulsion threshold at a vitrinite reflectance of 0.85–0.9%Ro or Tmax of 440–445 °C. 相似文献
18.
辽河盆地冷家油田沙河街组三段储层岩相古地理 总被引:2,自引:0,他引:2
辽河盆地在沙河街组三段早期水体较深,主要形成扇三角洲及盆底扇;沙三晚期水体较浅,发育湖泊砂体.依据沉积相分布规律,沙三早、中、晚3个时期可进一步分别划分出湖泊扩张和收缩阶段.盆地西部凹陷的冷家油田为东陡西缓的箕状洼陷.研究区内沙三段的古地理格局是决定相分布的关键因素,河流和湖泊能量相对强弱决定扇体沉积的规模.受相对湖平面变化的影响,纵向扇三角洲主要形成于湖泊扩张时期,并且有相带窄、过渡快、以粗碎屑沉积为主的特点.扇体沉积中主要发育前缘分流河道充填沉积,但位于河口前缘或侧缘的滩坝及前三角洲中的盆底扇局部也较发育. 相似文献
19.
车镇凹陷古近系沙河街组三段上亚段-二段下亚段是较为典型的深断陷型三级层序.层序的发育主要受控于幕式断陷作用,可进一步划分出低位体系域、湖侵体系域和高位体系域.通过岩心观察、薄片镜下鉴定、粒度分析、古生物及遗迹化石分析,并综合利用测井曲线和地震相特征,认为该时期主要发育有扇三角洲、三角洲、近岸水下扇、湖底扇、滨浅湖滩坝等骨架砂体相,以及滨浅湖、半深湖-深湖等沉积相及其亚相.综合考虑物源特征、沉积环境、沉积体系平面展布以及生、储、盖组合关系,认为有利的沉积相带主要是三角洲、扇三角洲前缘、湖底扇、近岸水下扇的中扇和外扇以及滨浅湖中发育的滩坝和砂坝. 相似文献
20.
A. Ankilov A. Baklanov M. Colhoun K. -H. Enderle J. Gras Yu. Julanov D. Kaller A. Lindner A. A. Lushnikov R. Mavliev F. McGovern T. C. O'Connor J. Podzimek O. Preining G. P. Reischl R. Rudolf G. J. Sem W. W. Szymanski A. E. Vrtala P. E. Wagner W. Winklmayr V. Zagaynov 《Atmospheric Research》2002,62(3-4)
During an international workshop at the Institute for Experimental Physics of the University of Vienna, Austria, which was coordinated within the Committee on Nucleation and Atmospheric Aerosols (IAMAS-IUGG), 10 instruments for aerosol number concentration measurement were studied, covering a wide range of methods based on various different measuring principles. In order to investigate the detection limits of the instruments considered with respect to particle size, simultaneous number concentration measurements were performed for monodispersed aerosols with particle sizes ranging from 1.5 to 50 nm diameter and various compositions.The instruments considered show quite different response characteristics, apparently related to the different vapors used in the various counters to enlarge the particles to an optically detectable size. A strong dependence of the 50% cutoff diameter on the particle composition in correlation with the type of vapor used in the specific instrument was found. An enhanced detection efficiency for ultrafine hygroscopic sodium chloride aerosols was observed with water operated systems, an analogous trend was found for n-butanol operated systems with nonhygroscopic silver and tungsten oxide particles. 相似文献