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31.
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The early diagenesis of trace elements (V, Cr, Co, Cu, Zn, As, Cd, Ba, U) in anoxic sediments of the Achterwasser, a shallow lagoon in the non-tidal Oder estuary in the Baltic Sea, was investigated in the context of pyrite formation. The dissolved major redox parameters show a two-tier distribution with transient signals in the occasionally re-suspended fluid mud layer (FM) and a permanently established diagenetic sequence in the sediment below. Intense microbial respiration leads to rapid depletion of O2 within the uppermost mm of the FM. The reduction zones of Mn, Fe and sulfate overlap in the FM and in the permanently anoxic sediment section which appears to be a typical feature of estuarine sediments, under low-sulfate conditions. Degrees of pyritization (DOP) range from 50% in the FM to remarkably high values > 90% at 50 cm depth. Pyrite formation at the sediment surface is attributed to the reaction of Fe-monosulfides with intermediate sulfur species via the polysulfide pathway. By contrast, intense pyritization in the permanently anoxic sediment below is attributed to mineral growth via adsorption of aqueous Fe-sulfide complexes onto pyrite crystals which had originally formed in the surface layer.The studied trace elements show differential behavior patterns which are closely coupled to the diagenetic processes described above: (i) Zn, Cu and Cd are liberated from organic matter in the thin oxic layer of the sediment and diffuse both upwards across the sediment/water boundary and downwards to be trapped as monosulfides, (ii) V, Cr, Co and As are released during reductive dissolution of Mn- and Fe-oxyhydroxides, (iii) U removal from pore water occurs concomitantly to Fe reduction in the FM and is attributed to reduction of U(VI) to U(IV), (iv) the Ba distribution is controlled by reductive dissolution of authigenic barite in the sulfate reduction zone coupled with upward diffusion and re-precipitation. The incorporation of trace elements into pyrite is most intense for Co, Mn and As, intermediate for Cu and Cr and little to negligible for U, Zn, Cd, V and Ba. The observed trend is largely in agreement with previous studies and may be explained with differing rates for ligand exchange. Slow and fast ligand exchange and thus precipitation kinetics are also displayed by downcore increasing (Mn, Cr, Co and As) or constantly low (Zn, Cu, Cd) pore water concentrations. The downward increasing degrees of trace metal pyritization (DTMP) for Co, Cu, Zn and As are, in analogy to pyrite growth, assigned to adsorption of sulfide complexes or As oxyanions onto preexisting pyrite minerals. 相似文献
33.
长江三角洲晚更新世末期古土壤与古环境 总被引:4,自引:0,他引:4
长江三角洲地区第一暗绿色硬粘土层是上海地区主要建筑持力层之一,也是划分全新统与更新统的标志层,前人已做过大量研究,但尚缺乏古土壤方面的系统研究工作。本文首次从古土壤学的角度系统研究了该层的古土壤特征,通过粒度分析发现有粘粒的生成,微形态研究发现有粘粒及铁锰、碳酸盐等化学组分的迁移与淀积,化学全量分析得出该层的硅铝率为2.80~3.37,说明该层已发生较强的成土作用,可以确认该层为古土壤层,并进一步把该层划分为4个B层、3个A层,亦即该层为复合古土壤层。根据该层的成土特征,将其命名为古潮土 相似文献
34.
Relationship between biogeochemical features of biogenic elements and flocculation in the Changjiang Estuary 总被引:1,自引:3,他引:1
RelationshipbetweenbiogeochemicalfeaturesofbiogenicelementsandflocculationintheChangjiangEstuary¥LinYi'an;TangRenyou;LiYan;Do... 相似文献
35.
Although the Yellow River Delta and Bohai Sea coastal zone are long distance and different environment with Po River Delta and Adriatic Sea coastal zone, the comparison of data of two different areas and the evolution trend of two areas are quite similar. The influence of natural climatic changes on the evolution of the deltas and coastal zones exists both in ancient and modern times. The cold/wet period occurred in 1300—1400A. D. and 1550 —1850 A.D. within this"large scale" climatie cycle, and shorter periods (10— 35 years) of cold rainy weather alternated with warm/dry period are known as "Bruckner cycles" which have influence on the evolution of the deltas and coastal zones. 相似文献
36.
珠江口现代沉积速率及其反映的沉积特征 总被引:2,自引:0,他引:2
文章分析了珠江河口海区泥沙来源及淤积动态,采用以历史海图分析对比为主,~(210)Pb测年数据校核等方法,参考有关沉积速率定性方面的标志,推算出珠江口不同地段的现代沉积速率,并相应划分出高速率沉积、快速率沉积、中速率沉积和慢速率沉积或稍有侵蚀等4个分区.进而,还论述了沉积作用的特征. 相似文献
37.
Variation of reactivity of particulate and sedimentary organic matter along the Zhujiang River Estuary 总被引:3,自引:0,他引:3
To investigate organic matter source and reactivity in the Zhujiang River (Pearl River)Estuary and its adjacent areas, particulate organic carbon (POC), particulate hydrolysable amino acids (PHAA), and Chl a during two cruises in July 1999 and July 2000 were measured. The highest POC and PHAA concentration was observed in the waters with maximum Chl a. The spectra distribution,relative content (dry weight in milligram per gram), PHAA-C% POC and other indicators such as the ratios of amino acids vs. amino sugars (AA/AS) and glucosamine vs. galactosamine (Glum/Gal) suggested that particulate amino acids in the water column and sediments in the Zhujiang River Estuary were mainly derived from biogenic processes rather than transported from terrestrial erosion. In inner estuary where high turbidity was often observable, organic matter was mainly contributed by re-suspension of bottom sediments with revealed zooplankton, microbial reworked characteristics, which suggest that these organic matters were relatively “old“. In the estuarine brackish region, organic matter in water column is mainly contributed by relatively fresh, easily degradable phytoplankton derived organic matter.During physical - biological processes within the eastuary, organic matter derived from phytoplankton was subjected to alteration by zooplankton grazing and bacterial reworking. 相似文献
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基于拉格朗日余流及其输运过程的一种三维空间弱非线性理论,进一步假定Si在河口的无因次化学转移项量级为k^2,给出了Si的长期输运方程。对于一种二维模型河口,数值求解了零阶天文潮,欧拉余流、斯托克斯漂移、拉格朗日余流和盐度的分布;分别计算了平均逼留时间为13,30,60,180d等所对应的Si浓度分布;给出了Si-s相关图,讨论了河口中Si的保守性问题。 相似文献