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21.
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Concentrations of total recoverable inorganic tin (TRISn), monomethyltin (MeSn3+), dimethyltin (Me2Sn2+), trimethyltin (Me3Sn+) and (3-dimethylsulphonio)propionate (DMSP) were determined in leaves of Spartina alterniflora from three sites in the Great Bay estuary (NH) from 8 May to 15 September 1989. Total methyltin concentration increased from 8·9 ng g−1 (fresh weight) on 8 May to 472 ng g−1 on 23 May, decreased to 52 ng g−1 on 7 June and 16ng g−1 on 20 June, and remained low until the last sample on 18 September. Statistical calculations showed that methyltin concentrations varied significantly with sampling week, but not with site. DMSP concentrations showed very different behaviour. During the same sampling period DMSP concentrations varied only from 7·5 to 26 μmol g−1 (fresh weight). DMSP concentrations varied significantly for site, but not sampling week. 相似文献
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A remarkable invariance in the ratio of 1,3-dimethylcarbazole (DMC) to 1,6-DMC was discovered in crude oils from the Pearl River Mouth Basin, South China Sea. The remarkably invariant ratio is kept at a constant of about unity regardless of their concentrations, sources or maturities for the sampies. In combination with the molecular structures of 1,3- and 1,6-DMCs, the invariance might indicate that the nitrogen compounds share a common precursor with a skeleton of 1-methylcarbazole and are formed through methylation at C3 and C6 with an essentially identical rate. 相似文献
25.
Sets of 20 soda ash glasses, 16 soda lime glasses and 23 wood ash glasses mainly from excavations in Europe (additional soda ash glasses from Egypt) were analysed on 61 chemical elements. Average SiO2 is about 62% in soda glasses and 50% in wood ash glasses. The three groups of glasses contain on average 13% Na2O, 18% Na2O and 13% K2O as fluxes to lower the melting temperature of quartz at their production. The starting materials beside quartz were halophytic plant ash for soda ash glass, trona (Na3H(CO3)2·2H2O) and lime (clamshells) for soda lime glass and beech ash for wood ash glass. Each of the three major glass types contains specific Rare Earth Element (REE) concentrations mainly contained in quartz and its intergrown minerals. 50 Paleozoic and Mesozoic sandstones from Central Europe represent the quartz composition. The REE pattern of these glasses apparently indicates major compositional stages of the Continental Earth's Crust. The boron to lithium and sodium to potassium ratios as in seawater suggest reactions of materials for soda glass with seawater. Negative Ce anomalies in the three glasses are caused by reactions of quartz with seawater. 相似文献
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回顾分析Matilda医院超速CT室筛选首批病人中99例中国人资料,很明显从通常采用130-100Hounsfield单位作为检出冠状血管钙化的基数应用至中国人身上其阈值数目需要降低,同时,我们也发现如果病人年龄按每10年范围分组(21-30,30-40,41-50,51-60)而计算其超速CT的钙化指数会较随机男女一起按平均计算更易区分其差异.进一步分析显示,男性中年时候超速CT指数已达最高值,而女性则晚10年方达最高值,因此,为了更易探测冠脉循环内钙化倾向应作出超速CT检出钙化的指数数目.这些实践经验对动脉粥样硬化过程的预测或预防有实际意义. 相似文献
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认识沉积环境有机碳留存状况是阐述油气形成过程中有机碳早期成岩的关键内容。以南海珠江口盆地及其邻近海域为背景,通过研究表层沉积物中脂类化合物的形态组成,认识脂类有机碳的来源和留存状态,阐述特征脂类分子的早期成岩特征。结果表明,研究区域表层沉积物有机碳含量为0.22%~0.66%,有机碳稳定同位素分布在-20.88‰~-22.93‰之间,表现为显著的海源特征。沉积物中共检测出21种脂肪酸、6种脂肪醇、8种甾醇和植醇;总脂肪酸、脂肪醇、甾醇和植醇含量分别为12.57~40.27μg/g、5.35~8.98μg/g、0.15~3.75μg/g和0.01~3.99μg/g干重,总体表现为靠近珠江口和台湾海峡略高。脂类化合物的存在形态以游离态(FR)和碱性水解态(BH)为主,酸性水解态(AH)贡献较低;其中植醇和甾醇呈现显著的BH优势,植醇中未检出AH组分的贡献。脂类化合物主要来自于海洋现场生产,海洋微藻和细菌的相对贡献率分别为21.18%~33.78%和11.02%~15.64%,陆源高等植物贡献低于5%。来源于硫酸盐还原菌的支链脂肪酸在靠近珠江口海域高达1.79~2.62μg/g,占总脂肪酸的5.14%~6.50%,并与硫酸盐还原过程相关的古菌分布相一致。 相似文献
30.
Air was injected through a well in a thin transparent tank filled with saturated glass beads to study how the size and air
saturation of air sparging plumes are affected by particle size and gradation; operational parameters such as injection pressure,
well depth, injection pressure pulsing; and well outlet configuration. V-shaped air plumes with an apex between 40° and 60°
were obtained for all tests. The air pressure required to initiate sparging agreed closely with the sum of the air entry pressure
and the hydrostatic pressure, with higher initiation pressures required in the fine and well-graded beads. Higher air flow
rates and air saturations were obtained in coarser beads at a given pressure, and the variation in flow rate was consistent
with estimated air permeabilities. Peak average air saturations were 28–56% for the coarse-medium beads, 10% for the well-graded
beads, and 8% for the fine beads. Air saturation and the radius of influence increased modestly (<40%) as the normalized injection
pressure exceeded 0.1. Radius of influence increased by approximately a factor of two as the well depth increased, but leveled
off once the ratio of radius of influence to well depth reached 0.60–1.05. Pulsing of injection pressure had no effect on
the initiation pressure, air flow rate, or air saturation, but increased the size of the air plume and the radius of influence
slightly (<15%). Well outlet configuration had only a slight affect the radius of influence (<10%), air saturation (<10%),
or air flow rate (<12%). Dye testing showed that water surrounding the air plume circulated during continuous and pulsed sparging.
However, pulsed sparging resulted in greater and more defined circulation of water within and adjacent to the air plume, which
should reduce mass transfer limitations during sparging. 相似文献