华南黑碳气溶胶浓度与南海夏季风关系的年代际突变

利用重建的华南区域黑碳气溶胶(Black Carbon,BC)浓度资料,分析其与南海夏季风在年际尺度上的关系.结果 表明,华南区域BC浓度与南海夏季风的关系在2000年前后有明显的突变,由显著负相关变为显著正相关,即由高BC浓度弱季风变为高BC浓度强季风.通过合成对比分析,发现1988-1999年(第一时间段)的华南B...     

大气气溶胶中的铁及其溶解度研究综述

生物活性铁(Fe) 进入生物地球化学循环中能够调节碳循环,影响海洋初级生产力,间接影响全球气候变化。决定 Fe生物可利用度的关键因子是可溶Fe含量,其中大气气溶胶的长距离传输是上层海洋获取生物可利用Fe的重要来源。近年来,对气溶胶中的Fe及溶解度的研究取得了重要进展,包括对不同区域Fe质量浓度和溶解度的观测以及对Fe溶解度影响因素的讨论。基于以上研究成果,汇总了近二十年全球部分陆地和海洋站点观测所得的不同粒径气溶胶颗粒物中的Fe质量浓度及其溶解度数据;重点介绍了气溶胶沉降入海洋前影响Fe溶解度的主要因素,包括Fe的来源、大气物理过程以及大气化学和传输混合过程等,并就各影响因素间的关联及相对重要性展开讨论;对未来气溶胶 Fe的研究方向和方法提出建议。     

Ekman边界层动力学的理论研究

大气边界层及其与自由大气之间的相互作用具有明显的非线性特征,而这些特征是经典Ekman理论所不能描述的,因此,发展中等复杂程度(介于完全模式与经典Ekman模型之间)的大气边界层动力学模式,简称中间模式,对人们从理论上认识大气边界层动力学过程的非线性特征具有重要意义。本文对目前最具代表性的几个中间边界层模型:地转动量近似边界层模型、Ekman动量近似边界层模型以及弱非线性边界层模型进行了总结和分析,阐述了Ekman层主要动力学特征。通过分析上述各模型的理论框架,揭示了各模型的物理意义及其在描述Ekman边界层基本动力特征上的优点和局限性,并指出尽管在细节定量描述上有差异,但各中间模型对Ekman层动力学特征的定性描述具有很好的一致性。对于这些Ekman边界层近似理论模型的进一步应用问题,主要回顾和总结了利用上述模型探讨地形边界层结构、大气锋生过程、低层锋面结构和环流以及边界层日变化、低空急流形成等动力学问题的研究,并对这些研究所揭示的Ekman层动力学特征及其对自由大气低层运动的影响进行了分析,结果表明,这些Ekman边界层近似模型可以较好地揭示大气边界层动力学特征,在大气边界层动力学及其与自由大气相互作用的研究上具有重要价值。另外,还对目前Ekman边界层理论研究中存在的问题进行了一些分析,提出了有待进一步研究的科学问题。     

An Observational Study of the Mesoscale Mistral Dynamics

We investigate the mesoscale dynamics of the mistral through the wind profiler observations of the MAP (autumn 1999) and ESCOMPTE (summer 2001) field campaigns. We show that the mistral wind field can dramatically change on a time scale less than 3 hours. Transitions from a deep to a shallow mistral are often observed at any season when the lower layers are stable. The variability, mainly attributed in summer to the mistral/land–sea breeze interactions on a 10-km scale, is highlighted by observations from the wind profiler network set up during ESCOMPTE. The interpretations of the dynamical mistral structure are performed through comparisons with existing basic theories. The linear theory of R. B. Smith [Advances in Geophysics, Vol. 31, 1989, Academic Press, 1–41] and the shallow water theory [Schär, C. and Smith, R. B.: 1993a, J. Atmos. Sci. 50, 1373–1400] give some complementary explanations for the deep-to-shallow transition especially for the MAP mistral event. The wave breaking process induces a low-level jet (LLJ) downstream of the Alps that degenerates into a mountain wake, which in turn provokes the cessation of the mistral downstream of the Alps. Both theories indicate that the flow splits around the Alps and results in a persistent LLJ at the exit of the Rhône valley. The LLJ is strengthened by the channelling effect of the Rhône valley that is more efficient for north-easterly than northerly upstream winds despite the north–south valley axis. Summer moderate and weak mistral episodes are influenced by land–sea breezes and convection over land that induce a very complex interaction that cannot be accurately described by the previous theories.     

兰州市大气气溶胶的特征及其对呼吸道疾病的影响

根据2000年6月至2001年5月兰州市大气气溶胶的监测资料,分析了兰州市大气气溶胶的浓度、尺度谱分布及其年、月、日变化规律,进而探讨了大气气溶胶对人体舒适度的影响,分析了大气气溶胶浓度与呼吸道疾病发病人数之间的关系。结果表明:PM10月均浓度与同期呼吸道疾病月发病人数的变化趋势基本一致,两者呈显著性正相关;当PM10日均浓度明显升高后1～2 d,呼吸道疾病发病人数也随之增多。     

2004年冬季华北平原持续大雾天气的诊断分析

利用GTS1型数字式探空仪探测的资料、NCEP 1°×1°的6小时资料和常规观测资料,对2004年冬季华北平原历史上少见的持续大雾天气进行了天气动力学诊断分析。结果表明:华北平原近地面气层900hPa以下的负涡度平流、冷温度平流和弱辐合上升运动引起该层气温下降,900-500hPa的正涡度平流、暖温度平流和辐散下沉运动造成该层气温升高,在上升和下沉运动区的界面层中形成逆温层,逆温层的高度和强度影响雾的形成和状况。夜间辐射热力强迫作用和950hPa以下的微风是大雾形成的动力因子。大雾边界层中存在的水汽饱和层是在特定的环流形势下华北平原低空盛行东和东南向岸气流,将北部海面的水汽向西向北平流到冷近地面气层中的结果。     

2004年春季中国沙尘天气特征分析

利用全国681个站的沙尘天气观测资料分析得出,2004年春季中国北方的沙尘天气明显偏少、偏弱,主要表现在：（1）2004年春季681个站累计的沙尘天气日数2 080 d,相当于历史平均值的46.9%,是近四十余年中第三个偏少年份。沙尘暴的总面积约190万km2,仅为历史平均值的37.3%。（2）危害性较大的沙尘暴和强沙尘暴过程6次,不足2001年的一半。（3）4月和5月沙尘天气明显偏少导致整个春季显著偏少。沙尘天气出现时,PM10浓度相对增加,空气质量恶化,但与历史上较典型的强沙尘暴个例相比,PM10浓度增加的幅度不大。进一步分析表明,2004年春季沙尘天气偏少、偏弱的主要原因是大气动力条件不足,是比较特殊的一个年份。     

On the nonlinear response of lower stratospheric ozone to NOx and ClOx perturbations for different CH4 sources

The impact of sulfate aerosol, ClOx and NOx perturbations for two different magnitudes of CH4 sources on lower stratospheric ozone is studied by using a heterogeneous chemical system that consists of 19 species belonging to 5 chemical families （oxygen, hydrogen, nitrogen, chlorine and carbon）. The results show that the present modeled photochemical system can present several different solutions, for instance, periodic states and multi-equilibrium states appearing in turn under certain parameter domains, through chlorine chemistry and nitrogen chemistry together with sulfate aerosol as well as the increasing magnitude of CH4 sources. The existence of catastrophic transitions could produce a dramatic reduction in the ozone concentration with the increase of external sources.     

Tangling Turbulence and Semi-Organized Structures in Convective Boundary Layers

A new mean-field theory of turbulent convection is developed based on the idea that only the small-scale region of the spectrum is considered as turbulence, whereas its large-scale part, including both regular and semi-organized motions, is treated as the mean flow. In the shear-free regime, this theory predicts the convective wind instability, which causes the formation of large-scale semi-organized motions in the form of cells. In the presence of wind shear, the theory predicts another type of instability, which causes the formation of large-scale semi-organized structures in the form of rolls and the generation of convective-shear waves propagating perpendicular to the convective rolls. The spatial characteristics of these structures, such as the minimum size of the growing perturbations and the size of perturbations with the maximum growth rate, are determined. This theory might be useful for understanding the origin of large-scale cells and rolls observed in the convective boundary layer and laboratory turbulent convection     

An Intercomparison of Large-Eddy Simulations of the Stable Boundary Layer

Results are presented from the first intercomparison of large-eddy simulation (LES) models for the stable boundary layer (SBL), as part of the Global Energy and Water Cycle Experiment Atmospheric Boundary Layer Study initiative. A moderately stable case is used, based on Arctic observations. All models produce successful simulations, in as much as they generate resolved turbulence and reflect many of the results from local scaling theory and observations. Simulations performed at 1-m and 2-m resolution show only small changes in the mean profiles compared to coarser resolutions. Also, sensitivity to subgrid models for individual models highlights their importance in SBL simulation at moderate resolution (6.25 m). Stability functions are derived from the LES using typical mixing lengths used in numerical weather prediction (NWP) and climate models. The functions have smaller values than those used in NWP. There is also support for the use of K-profile similarity in parametrizations. Thus, the results provide improved understanding and motivate future developments of the parametrization of the SBL.