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R. Hellmann J.-M. Penisson R. L. Hervig J.-H. Thomassin M.-F. Abrioux 《Physics and Chemistry of Minerals》2003,30(4):192-197
Using an approach combining high-resolution and energy-filtered transmission electron microscopy (HRTEM and EFTEM), we have studied with Å to nm-spatial resolution the interfacial region that delimits the near-surface altered zone and non-altered labradorite feldspar after dissolution under acid pH conditions. The interface is characterized by extremely sharp and spatially coincident changes in structure and chemistry. The 500-nm-thick altered zone is depleted in interstitial cations (Ca, Na, K) and Al, a framework element, whereas it is enriched in H, O, and Si. Modeling H+-alkali interdiffusion within a 500-nm-thick altered zone shows that volume interdiffusion cannot reproduce the sharp chemical interfaces measured by EFTEM. Based on these new data, we propose that the near-surface altered zone is a result of interfacial dissolution-reprecipitation, and not of preferential leaching of cations and interdiffusion with H+. This implies an intrinsic dissolution process that is stoichiometric, where the breaking of bonds and release of interstitial cations and framework elements (Al, Si, and O) to solution occur contemporaneously at equal relative rates from the original fluid–mineral interface. 相似文献
135.
确定结构基底等效输入地震动的简化方法 总被引:1,自引:0,他引:1
本文用理论和实例计算分析了土与结构间的动力相互作用。根据基底等效输入的地震动相对入射地震动的传递函数特点研究出了一种等效输入的方法,该方法比较好地反映了场地和结构的动力特性对基底等效输入的影响。为利用刚性基底假设理论来分析土-结构动力相互作用提供了一种方法。 相似文献
136.
饱和土地基在既有房屋长期荷载作用下,地基土强度参数值随着地基土的排水固结和压密而提高,地基极限承载力也同时增大,如何估算此提高值而挖掘其潜力,传统方法只是借助于统计回归讨论了设计承载力。本文从土力学基本原理出发,借助Prandtl假定,对既有房屋饱和土地基极限承载力的增长进行了探讨。 相似文献
137.
Organic pollutants associated with macromolecular soil organic matter: Mode of binding 总被引:2,自引:0,他引:2
H. H. Richnow R. Seifert J. Hefter M. Link W. Francke G. Schaefer W. Michaelis 《Organic Geochemistry》1997,26(11-12)
A study of ether-linked moieties in macromolecular bound residues of polycyclic aromatic hydrocarbons (PAH) generated in bioremediation experiments was performed using high temperature hydrolysis degradation with subsequent analysis of the products by GC-MS. This hydrolysis reaction was specifically designed to cleave ether bonds including relatively stable diarylether structures. Among the reaction products, aromatic alcohols representing typical microbiologically derived metabolites of PAH were found in addition to natural compounds. Thus, parts of the bound residues appeared to be linked within the macromolecular material by ether bonds. Model experiments with an oxidoreductase enzyme and aromatic alcohols indicate the formation of these ether bonds to be an enzyme-catalysed process. 相似文献
138.
Javier Castro-Larragoitia Utz Kramar Harald Puchelt 《Journal of Geochemical Exploration》1997,58(1):81-91
The Ag---Pb---Zn---Cu---Au mining district of Santa María de La Paz has been extensively exploited for approximately 200 years. Consequences of these activities are several deposits of tailings with high As and heavy metal concentrations, which are completely unstable. The climate is semiarid and as the dumps have no protective cover, material from the dumps is dispersed by strong winds. It is also washed out during seasonally heavy rainfalls. By these processes approximately 100 km2 of surrounding have been contaminated by dump material. The As and heavy metal content of the soils was determined as well as their level in crops (Zea Maize) from agricultural lands in the vicinity of the dumps. In the direction of prevailing winds concentrations up to 1000 ppm Zn, 400 ppm Pb, 16 ppm Cd, 550 ppm Cu and 300 As have been detected in top soils. Using fuzzy cluster analysis the different contamination sources could be identified. Grains of corn from contaminated sites showed no critical concentrations, but leaves which are also used tor fodder, have As-concentrations up to 20 ppm. 相似文献
139.
我国特殊岩土研究 总被引:1,自引:0,他引:1
顾宝和 《水文地质工程地质》1997,24(2):43-45
本文分析,总结了我国特殊岩土理论与应用研究方面的新进展,内容涉及湿陷性黄土,软土膨胀岩土,红土,软岩和特殊土的结构性,指出需要进一步研究的问题,最后对特殊土的研究方法做了阐述。 相似文献
140.
土壤表面蒸发阻力模型与田间测定方法 总被引:6,自引:0,他引:6
土壤表面蒸发阻力是计算土壤蒸发率的关键参数。本文讨论土壤表面蒸发阻力的概念,一层,二层理论模型与经验模型,并以在澳大利亚进行的田测定为例,说明田间测定与计算方法,并以计算沟中的蒸发率为例,介绍其应用方法。 相似文献