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941.
I. E. Paukov N. K. Moroz Yu. A. Kovalevskaya I. A. Belitsky 《Physics and Chemistry of Minerals》2002,29(4):300-306
The heat capacity of paranatrolite and tetranatrolite with a disordered distribution of Al and Si atoms has been measured
in the temperature range of 6–309 K using the adiabatic calorimetry technique. The composition of the samples is represented
with the formula (Na1.90K0.22Ca0.06)[Al2.24Si2.76O10]·nH2O, where n=3.10 for paranatrolite and n=2.31 for tetranatrolite. For both zeolites, thermodynamic functions (vibrational entropy, enthalpy, and free energy function)
have been calculated. At T=298.15 K, the values of the heat capacity and entropy are 425.1 ± 0.8 and 419.1 ±0.8 J K−1 mol−1 for paranatrolite and 381.0 ± 0.7 and 383.2 ± 0.7 J K−1 mol−1 for tetranatrolite.
Thermodynamic functions for tetranatrolite and paranatrolite with compositions corrected for the amount of extraframework
cations and water molecules have also been calculated. The calculation for tetranatrolite with two water molecules and two
extraframework cations per formula yields: C
p
(298.15)=359.1 J K−1 mol−1, S(298.15) −S(0)=362.8 J K−1 mol−1. Comparing these values with the literature data for the (Al,Si)-ordered natrolite, we can conclude that the order in tetrahedral
atoms does not affect the heat capacity. The analysis of derivatives dC/dT for natrolite, paranatrolite, and tetranatrolite has indicated that the water- cations subsystem within the highly hydrated
zeolite may become unstable at temperatures above 200 K.
Received: 30 July 2001 / Accepted: 15 November 2001 相似文献
942.
As a legacy of the centrally planned economy, the economies in transition of Central and Eastern Europe (CEE) have a unique
potential to reduce their greenhouse gas emissions through the improvement in their high energy intensities. Since much of
this `low-hanging fruit' in energy-efficiency improvements can be highly cost-effective, many developed countries facing difficulties
in meeting their greenhouse gas (GHG) emission targets domestically are eager to find such opportunities in the CEE region.
Therefore, studies analysing the potentials and costs of carbon dioxide reduction through technology improvement in the region
have come into the limelight. While there are a few excellent studies in the region aimed at analysing climate change abatement
potentials, they all embark on different assumptions, methodologies and boundary conditions. It is hence difficult, if not
impossible, to compare and analyse the results of these studies across different authors, countries or time horizons. Consequently,
the purpose of this paper is to place four leading studies on GHG mitigation through technology improvement from the CEE region
into an internationally comparable framework. Four studies were selected from three countries, Poland, Hungary and Estonia,
which are all the results of major national and international efforts to assess costs and potentials of GHG reduction. The
paper places their assumptions, methods and final results into a framework which enables policy-makers and project designers
to compare these across geographical and technological boundaries. Since other studies from around the globe have been analysed
in this framework in the literature, this paper provides a vehicle for the findings of these four studies to be compared to
others worldwide. In addition, the paper highlights a few areas where similar studies to be completed in the future in the
region may be enhanced by incorporating features used in GHG mitigation research in other parts of the world.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
943.
Authigenic albites in carbonate rocks typically grow in a high-grade diagenetic to low-grade metamorphic environment and often show Roc-Tourné-twinning sensu Füchtbauer. Based on an investigation of four Middle to South European occurrences, they show Mn2+- and Fe3+-activated cathodoluminescence (CL), as revealed by combined high resolution spectroscopy of cathodoluminescence emission (HRS-CL), electron paramagnetic resonance (EPR), and proton-induced X-ray emission (μPIXE). 相似文献
944.
Understanding the nature and impacts of tsunamis within the Aegean Sea region ofGreece is of importance to both the academic community and those organisationsconcerned with tsunami disaster management. In order to determine hazard and riskand consequently pre-plan mitigative strategies, it is necessary to analyse historical(documentary) and geological records of former tsunami events. Therefore, firstlythis paper provides a summary of the written sources of information on Aegeantsunamis paying particular attention to published catalogues. From the availabledata, it is noted that a large number of events have been reported during the last3500 years. Secondly, the paper provides a review of the published on-shore(terrestrial) geological records of tsunamis within the region. From this analysisit is seen that little geological evidence has been identified for the large numberof tsunamis reported in the catalogues. Thirdly, the paper considers the reliabilityof the written and geological records and how problems of accuracy, coverage,extent and reliability, may have potential implications for the estimation of hazardand risk. The paper concludes by making recommendations for disaster managers,geologists and historians to work closely together. 相似文献
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949.
大横路地区出露地层主要为元古界老岭群大栗子组和珍珠门组的低绿片岩相 -高绿片岩相到低角闪岩相的变质岩系 ,北部有少量英云闪长岩 -奥长花岗岩和表壳岩残块。侵入岩主要以燕山期基性 -中基性为主。铜钴矿床产于含碳绢云千枚岩中 ,矿体长 36 0~ 140 0m ,宽 95~ 80 0m ,厚 3~ 10 8.7m ,呈层状、似层状、分枝状 ,矿石以浸染状为主 ,次为脉状、网脉状。矿床属多期多成因类型 ,主要受大栗子组地层、北东向断裂构造和变质作用控制 ,并有岩浆热液的叠加。 相似文献
950.
Abstract: Carbonate rocks of Cambrian (18 samples) and lower-middle Ordovician (11 samples) ages from South Korea were analyzed for sulfur contents of structurally substituted sulfate (SSS) and sulfides and their δ34 S values. The δ34 S values of SSS ranging from +25.9 to +45.2 permil, are averaged as +33.6 and +33.5 permil for the Cambrian and Ordovician rocks, respectively, which indicate high δ34 S values of the Cambro-Ordovician seawater. The SSS contents in the carbonate rocks are low being 2.9 to 17.3 ppm S (averaged as 7.0 ppm S). Sulfide sulfur, on the contrary, is much abundant containing 3 to 1,880 ppm S and the δ34 S values range widely between –17.6 and +31.1 permil. Sulfide sulfur of the studied rocks excluding impure carbonates has an average content of 187 ppm S and δ34 S value of +12.8 permil (n=24). The estimated δ34 S (sulfate–sulfide) values, which range from 13.8 to 25.4 permil in general with a few exceptions from 36.5 up to 52.3 permil for some impure carbonates, may provide evidence for the persistent oceanic anoxia with its temporary recovery during the Cambro-Ordovician time.
The SSS and sulfide sulfurs have often higher δ34 S values than the Mesozoic-Cenozoic ore sulfur (Ishihara et al., 2000). Since carbonate rocks are very reactive with circulating hydrothermal ore solution, high δ34 S values of the Korean ore deposits might be caused to some extent by 34 S enrichment from the host carbonates, resulting in the low SSS contents observed. 相似文献
The SSS and sulfide sulfurs have often higher δ