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251.
Jianwei Wang 《Earth and Planetary Science Letters》2004,222(2):517-527
Molecular dynamics (MD) modeling of the 10-Å phase, Mg3Si4O10(OH)2·xH2O, with x=2/3, 1.0 and 2.0 shows complex structural changes with pressure, temperature and water content and provides new insight into the structures and stabilization of these phases under subduction zone conditions. The structure(s) of this phase and its role as a reservoir of water in the mantle have been controversial, and these calculations provide specific predictions that can be tested by in situ diffraction studies. At ambient conditions, the computed structures of talc (x=0) and the 10-Å phases with x=2/3 and 1.0 are stable over the 350-ps period of the MD simulations. Under these conditions, the 10-Å phases show phlogopite-like layer stacking in good agreement with previously published structures based on powder X-ray diffraction data for samples quenched from high-pressure and high-temperature experiments. The calculations show that the 10-Å phase with x=2.0 is unstable at ambient conditions. The computed structures at P=5.5 GPa and T=750 K, well within the known stability field of the 10-Å phase, change significantly with water content, reflecting changing H-bonding configurations. For x=2/3, the layer stacking is talc-like, and for x=1.0, it is phlogopite-like. The calculations show that transformation between these two stackings occurs readily, and that the talc-like stacking for the x=2/3 composition is unlikely to be quenchable to ambient conditions. For x=2.0, the layer stacking at P=5.5 GPa and T=750 K is different than any previously proposed structure for a 10-Å phase. In this structure, the neighboring basal oxygens of adjacent magnesium silicate layers are displaced by b/3 (about 3 Å) resulting in the Si atoms of one siloxane sheet being located above the center of the six-member ring across the interlayer. The water molecules are located 1.2 Å above the center of all six-member rings and accept H-bonds from the OH groups located below the rings. The b/3-displaced structure does not readily transform to either the talc-like or phlogopite-like structure, because neither of these stackings can accommodate two water molecules per formula unit. There is likely to be a compositional discontinuity and phase transition between the b/3-displaced phase and the phase with phlogopite-like stacking. The simulations reported here are the first to use the recently developed CLAYFF force field to calculate mineral structures at elevated pressures and temperatures. 相似文献
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A multi‐proxy approach was used to examine the geomorphic dynamics and environmental history of an upper deltaic ?oodplain tract in the Sacramento–San Joaquin Delta, California. Three long cores were collected from the McCormack–Williamson Tract (MWT) and these cores were analyzed for bulk density, loss‐on‐ignition, ?ne (clay and silt) content, Al concentration, magnetic susceptibility, pollen, and charcoal. Radiocarbon dates obtained for the cores were converted into calendar years and an age–depth model was constructed. Long‐term vertical accretion and sedimentation rates were estimated from the age–depth model. Cross‐core relations show that coarse sediment generally accumulates more rapidly and has greater magnetic susceptibility compared to ?ne sediment. Percentage ?ne and LOI data show a strong linear relationship that indicates ?ooding is the primary mechanism for the deposition of particular organic matter on the ?oodplain and that landscape wash load has contributed a highly consistent fraction of persistent organic matter averaging 5·5 per cent to the site. Down‐core grain size pro?les show two hydrological domains in the cores, namely millennial ?ne–coarse ?uctuations superimposed on general up‐core ?ning. Coarse sediment is viewed as channel or near‐channel overbank deposits, whereas ?ne deposits are considered to be distal overbank ?ood deposits. The coarse–?ne ?uctuations are indicative of changing depositional settings as channels migrated laterally across MWT, whereas the upward ?ning trend re?ects a combination of self‐limiting overbank deposition as ?oodplain elevation increased and decreasing competence as sea‐level rise reduced ?ood‐pulse energy slopes. MWT has been cross‐cut and incised numerous times in the past, only to have the channels abandoned and subsequently ?lled by ?ne sediment. The channels around MWT attained their modern con?guration about 4000 years ago. MWT likely came under tidal in?uence at about 2500 cal BP. Wetlands have recently developed on MWT, but they are inorganic sediment dominated. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
255.
为了加深对黄金带复杂断块油田进一步开发,针对该区断层复杂、储层变化大、油水关系复杂等特征,笔者综合运用岩心、分析化验及录井、测井资料,对其沉积特征、储层岩性、物性和非均质性进行详细研究。以JASON软件为平台,对含油砂体进行了追踪和预测,并在有利区提出井位部署,为该区的进一步开发提供了地质依据。 相似文献
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258.
大连市是我国严重缺水地区之一 ,至 2 0 0 5年城市缺水为 110 4 2 .5× 10 4m3 ,占需水量的 17.1% ,其中大连城区 (金州以南地区 )缺水 9890× 10 4m3 ,占缺水量的 89.6 %。开发利用滨海河谷地下水资源 ,建立滨海河谷型地下水库 ,不仅可以治理大连地区严重的海水入侵问题 ,增加水资源量 ,满足当地农业及生活用水 ,同时可弥补城市供水的不足。根据前人工作成果分析及野外实地勘查 ,大连市适于建设河谷型地下水库的滨海河谷有 2 2条 ,建成后的总库容量 10 36 0 2 .9× 10 4m3 ,开采资源量 2 5 76 6 .88× 10 4m3 ,可增加开采资源量 12 5 4 2 .4 5× 10 4m3 。 相似文献
259.
传统的水库汛限水位的控制,只利用了洪水的统计信息,使水库在汛期要时刻预防设计与校核洪水事件的发生,致使一些水库在汛期不敢蓄水而汛后又无水可蓄,造成洪水资源的浪费。提出水库汛限水位动态控制的新理念及其综合推理模式,适应当前预报技术的发展水平,考虑降雨径流洪水预报与一定时间内的短期降雨预报,排除不可能发生的洪水事件,预报可能发生的洪水,实施水库汛限水位的动态控制。但预报不可避免地存在误差,当小概率预报误差事件发生时,仍可采取弥补措施以确保大坝的防洪安全。 相似文献
260.
夏季红枫湖地区农田土壤-大气界面汞交换通量的初步研究 总被引:11,自引:2,他引:11
采用动力学通量箱法(Dynamic Flux Chamber)与高时间分辨率大气测汞仪联用技术对贵州红枫湖地区土壤-大气界面间汞交换通量进行了初步研究.结果显示,红枫湖地区土壤-大气界面间汞交换通量变化范围为-8.6 ng~215.3 ng@m-2@h-1,平均27.4士40.1 ng/m2@h(n=255);且土壤与大气界面间的汞交换是双向的既有土壤汞的释放,又有大气汞的沉降,主要以土壤汞的释放为主(n释放=253,n沉降=2n).土壤汞的释放通量与土壤温度、气温、光照强度有强相关关系,相关系数分别为0.80、0.83、0.74. 相似文献