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This paper deals with dissolved inorganic carbon (DIC) and organic carbon (DOC) in pore waters from a 150 m deep hole drilled through the carbonate barrier reef of Tahiti and its underlying basalt basement. Alkalinity-pH measurements were used to calculate the DIC species concentration, and DOC was analysed according to the high temperature catalytic oxidation technique. Salinity was used as a conservative tracer to help identify water origin and mixing within the hole. Water mixing, calcium carbonate dissolution and mineralization of organic carbon combined to form three distinct groups of pore water. In the deeper basalt layers, pore water with alkalinity of 1.4 meq kg–1 pH of 7.6 and p(CO2) of 1.2 mAtm was undersaturated with respect to both aragonite and calcite. In the intermediate carbonate layer, pore water with alkalinity of more than 2.0 meq kg–1, pH of 7.70 and p(CO2) of 1.4 mAtm was supersaturated with respect to both aragonite and calcite. The transition zone between those two groups extended between 80 and 100 m depth. The shift from aragonite undersaturation to supersaturation was mainly attributed to the mixing of undersaturated pore waters from the basalt basement with supersaturated pore waters from the overlaying limestone. In the top of the reef, inputs from a brackish water lens further increased p(CO2) up to 5.6 times the atmospheric P(CO2). 相似文献
54.
A core from the Cambay Shale Formation of the Cambay Basin, containing immature Type III organic matter, was pyrolysed at 300°C for different durations of time to different maturation levels. Fractionation effects were studied employing a three-step extraction technique after removal of the expelled pyrolysate. The extractable organic matter (EOM) obtained on extraction of the whole core is assumed to be that present in open pores, while that obtained on finely crushing the sample is assumed to be that present in closed pores. The EOM obtained from 1 cm chips is termed EOM from semi-open pores. The gross composition of the pyrolysates expelled during pyrolysis is not similar to the oils reservoired in the area, and there is no significant fractionation observed between expelled pyrolysates and unexpelled EOM. Our study indicates movement of fluids between closed, semi-open and open pores. In both systems, there is a higher concentration of EOM in open pores than in semi-open and closed pores, and the fraction of EOM in open pores is much greater in the artificial system than in the natural system. Fractionation effects on n-alkane and isoprenoid hydrocarbon-based parameters were also studied. n-Alkenes are present in semi-open and closed pores of the immature core and in the core after it was pyrolysed to 300°C for 6 and 48 h, but are absent in the open pores. n-Alkenes are present in closed pores in the naturally matured core. Presence of n-alkenes in the pyrolysates expelled during the 6 and 48 h experiments, but their absence in the open pores of the core, indicates that expulsion also occurs through temporary microfractures during laboratory pyrolysis, whereas in the natural system expulsion from closed pores seems to be only via semi-open and open pores. 相似文献
55.
A Study on Organic Inclusions in Clastic Reservoir Rocks and Their Application to the Assessment of Oil and Gas Accumulations 总被引:5,自引:0,他引:5
Terrigenous clastic reservoir rocks are widespread in China,and nearly all the industrial oil and gas accumulations in eastern China occur in the clastic rocks.The study shows that organic inclusions are mostly distributed in the secondary fissures and pores which were ormed in the process of oil-rock interaction,rather than in the cements or secondary enlargements. The organic inclusions are dominantly organic gas-rich or are composed of pure hydrocarbons.Homogenization temperatures range mainly from 120℃ to 130℃,which shows a relatively high maturity of organic matter.Vertical and horizontal temperature changes provide the grounds for the investigation of basin evolution and thermal fluid-kinetics-model.Fluorescence spectral characteristics o the organic inclusions indicate that oils and gases in the area studied probably have experienced two-stage or two-time migration.Micro-fluorescence rescearch is one of the effective approaches to oil/source correlation and oil migration-stage determination.The abundance and occurrence of organic inclusions is one of the indicators of oil and gas abundance and accumulation in rock layers.With the help of other informatio,organic inclusions can provide the basis for the prospective assessment of oil and gas in clastic reservoir rocks. 相似文献
56.
The Turpan-Harmi (abbreviated to Tuha below) Basin is a typical basin of coal-generated oil accumulation in China. The Middle-Lower
Jurassic coal measures are considered the main source beds. Hence, both desmocollinite and suberinite are considered the contributors
for coal-generated oil. Principal geochemical features of the crude oil in the Tuha Basin are rich in alkanes (70%—80%), high
pristane/phytane ratio (6—8), abundant heavy carbon isotope (δ13C PDB= -26%–-23%) and absolute GP sterane predominance. The hydrocarbon generation process from the coal series is characterized
by multistages, early generation and early expulsion. 相似文献
57.
Monitoring and modelling of pore water pressure changes and riverbank stability during flow events 总被引:1,自引:0,他引:1
Pore water pressures (positive and negative) were monitored for four years (1996–1999) using a series of tensiometer‐piezometers at increasing depths in a riverbank of the Sieve River, Tuscany (central Italy), with the overall objective of investigating pore pressure changes in response to ?ow events and their effects on bank stability. The saturated/unsaturated ?ow was modelled using a ?nite element seepage analysis, for the main ?ow events occurring during the four‐year monitoring period. Modelling results were validated by comparing measured with computed pore water pressure values for a series of representative events. Riverbank stability analysis was conducted by applying the limit equilibrium method (Morgenstern‐Price), using pore water pressure distributions obtained by the seepage analysis. The simulation of the 14 December 1996 event, during which a bank failure occurred, is reported in detail to illustrate the relations between the water table and river stage during the various phases of the hydrograph and their effects on bank stability. The simulation, according to monitored data, shows that the failure occurred three hours after the peak stage, during the inversion of ?ow (from the bank towards the river). A relatively limited development of positive pore pressures, reducing the effective stress and annulling the shear strength term due to the matric suction, and the sudden loss of the con?ning pressure of the river during the initial drawdown were responsible for triggering the mass failure. Results deriving from the seepage and stability analysis of nine selected ?ow events were then used to investigate the role of the ?ow event characteristics (in terms of peak stages and hydrograph characteristics) and of changes in bank geometry. Besides the peak river stage, which mainly controls the occurrence of conditions of instability, an important role is played by the hydrograph characteristics, in particular by the presence of one or more minor peaks in the river stage preceding the main one. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
58.
GE Heping SUN Yan LU Xiancai ZHU Wenbin GUO Jichun LIU Deliang & Chi-yuen Wang . Department of Earth Sciences Nanjing University State Key Laboratory of Mineral Deposit Nanjing China . Department of Earth Space Sciences University of Science Technology of China Hefei China . Department of Geology Geophysics University of California Berkeley CA USA 《中国科学D辑(英文版)》2004,47(3)
In the 1990s of the 20th century, we participated in the research of the stress field in fissure tectonics of scientific deep bore cores for the Deep Observation and Sampling of the Earths Continental Crust (DOSECC for short). Spherical and enriched ul-tra-micro granular textures (nm size), which enriches Nb element (Wang & Sun, 1990; Sun & Wang, 1993)[1,2], were found during the observation of ul-tra-micro slipping lamellae of ductile and brittle oc-curring in Late Mesozoic granites us… 相似文献
59.
Weathering: Toward a Fractal Quantifying 总被引:1,自引:0,他引:1
Klaudia Oleschko Jean-Francois Parrot Gerardo Ronquillo Sergey Shoba Georges Stoops Vera Marcelino 《Mathematical Geology》2004,36(5):607-627
Weathering occurs over a wide range of scales. To link features through these scales is a major challenge for interdisciplinary weathering studies. Fractal approach seems to be specially useful for this purpose. We introduce a multistep fractal weathering assessment scheme devoted to extract fractal weathering classifiers from texture analysis of the mineral's image. Our scheme enables to quantitatively estimate the global and local information about the geometry of the weathering pattern. This information is basic to develop geometrical indices of weathering, which can significantly enrich the common qualitative and semiquantitative weathering assessment schemes. To justify the fractal approach, a strong statistical self-similarity has been documented for both the weathering and fresh features of two common silica minerals: quartz and biogenic A-opal (phytolith) over four orders of length scales. The procedure is fast, drastically reduces thresholding bias, promises to be universal, it is valid for genetically different minerals and rock types, scale independent, and specially useful for monitoring the changes in the mineral's roughness during the alteration. Two of the proposed classifiers seem to be potentially useful for direct application in the field and be used by nonspecialist. 相似文献
60.
T. N. Yang 《Journal of Metamorphic Geology》2004,22(7):653-669
The Qinglongshan eclogites in the Southern Sulu ultrahigh pressure metamorphic (UHPM) terrane show very different retrograded textures from their counterparts in the Northern Sulu terrane, implying a different thermal history. Scanning electron and optical microscope observations indicate that the peak assemblage of the Qinglongshan eclogite is anhydrous, composed of Grt + OmpI + Rt + (Ky + coesite). These primary minerals were replaced by second and third stage minerals, resulting in symplectite pseudomorphs or coronas. The following relationships are inferred: OmpI → OmpII + Ab + Fe‐oxide symplectite (type I) and Rt → Rt + Ilm intergrowth; and, Ky → Pg, OmpII (+Pl) → Amp (+Pl) symplectite (type II), and Grt → Prg (+Fe‐oxide). Mineral chemistry and mass‐balance demonstrate that the pseudomorphed textures were developed by metasomatism involving dissolution and precipitation intensified by fluids along grain boundaries. The formation of symplectite type I produced Fe, Mg and Na but consumed Ca and Si. The Mg and Fe diffused to garnet where exchange of (Mg, Fe) with Ca of the garnet resulted in compositional zonation with decreased Ca towards the edge of garnet grains where Ca was consumed during symplectite formation. The replacement of kyanite by paragonite consumed the extra Na. In the later stage, fluid infiltration partially transformed symplectite type I to type II, and narrow rims of pargasite resorbed garnet from their boundaries. Mass balance suggests that the transformation and resorption would have been coupled during fluid infiltration. In the latest stage, epidote and quartz were precipitated at very late stage as a result of fluid activity along microfractures. Tentative P–T conditions based on mineral reactions and thermocalc software suggest that the retrograded eclogite did not record the granulite facies retrograde evolution characteristic of eclogites from the Northern Sulu terrane. The difference in retrograde evolution between the Southern and Northern Sulu eclogites suggests a different exhumation history. 相似文献