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481.
K. N. Bower T. W. Choularton M. W. Gallagher R. N. Colvile K. M. Beswick D. W. F. Inglis C. Bradbury B. G. Martinsson E. Swietlicki O. H. Berg S. -I. Cederfelt G. Frank J. Zhou J. N. Cape M. A. Sutton G. G. McFadyen C. Milford W. Birmili B. A. Yuskiewicz A. Wiedensohler F. Stratmann M. Wendisch A. Berner P. Ctyroky Z. Galambos S. H. Mesfin U. Dusek C. J. Dore D. S. Lee S. A. Pepler M. Bizjak B. Divjak 《Atmospheric Research》1999,50(3-4)
During March and April of 1995 a major international field project was conducted at the UMIST field station site on Great Dun Fell in Cumbria, Northern England. The hill cap cloud which frequently envelopes this site was used as a natural flow through reactor to examine the sensitivity of the cloud microphysics to the aerosol entering the cloud and also to investigate the effects of the cloud in changing the aerosol size distribution, chemical composition and associated optical properties. To investigate these processes, detailed measurements of the cloud water chemistry (including the chemistry of sulphur compounds, organic and inorganic oxidised nitrogen and ammonia), cloud microphysics and properties of the aerosol and trace gas concentrations upwind and downwind of the cap cloud were undertaken. It was found that the cloud droplet number was generally strongly correlated to aerosol number concentration, with up to 2000 activated droplets cm−3 being observed in the most polluted conditions. In such conditions it was inferred that hygroscopic organic compounds were important in the activation process. Often, the size distribution of the aerosol was substantially modified by the cloud processing, largely due to the aqueous phase oxidation of S(IV) to sulphate by hydrogen peroxide, but also through the uptake and fixing of gas phase nitric acid as nitrate, increasing the calculated optical scattering of the aerosol substantially (by up to 24%). New particle formation was also observed in the ultrafine aerosol mode (at about 5 nm) downwind of the cap cloud, particularly in conditions of low total aerosol surface area and in the presence of ammonia and HCl gases. This was seen to occur at night as well as during the day via a mechanism which is not yet understood. The implications of these results for parameterising aerosol growth in Global Climate Models are explored. 相似文献
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以阴离子表面活性剂硬脂酸钠为改性剂制备了硬脂酸钠改性蒙脱石(NaSTA-MMT).FI-IR和XRD分析表明插层剂已进入蒙脱石层间,且随着硬脂酸钠量的增加蒙脱石层间距从1.274 nm增加到4.805 nm。亚甲基蓝吸附实验表明,硬脂酸钠改性蒙脱石吸附行为遵循伪二级动力学方程。平衡吸附量与平衡质量浓度之间的关系符合Langmuir等温吸附方程所描述的规律。硬脂酸钠改性膨润吸附亚甲基蓝表现为自发的表面物理吸附过程,吸附活化能、吸附焓变和熵变分别为2.36 kJ/mol-、21.47 kJ/mol和-44.45 J/mol.K。 相似文献
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改性坡缕石粘土的全孔分布研究 总被引:10,自引:2,他引:10
为改善坡缕石粘土的表面性能和提高其实用价值,采用酸浸、酸浸 加热、酸浸 加热 甲醛浸渍3种方法处理天然坡缕石粘土,并通过扫描电镜(SEM)、傅立叶变换红外光谱(FT_IR)、X荧光光谱(XRF)、BET_比表面积分析(BET_SSA)及全孔分布等分析手段来评估坡缕石粘土的处理效果。结果表明与未经处理的原土相比,经过3种方法处理,坡缕石粘土内部细长而致密有序的晶束被打断、破碎和分散,微晶表面粗糙度增大;杂质特别是碳酸盐的去除效果显著,比表面积是原土的2倍多,总孔容积几乎增加1倍,中孔容积从0.092cm3/g增加到0.15cm3/g左右,平均孔径减小2~3nm;处理后坡缕石粘土的假孔分布峰值在17nm,比原土假孔分布峰值22nm减小约5nm,而且4个样品中的孔几乎都在介孔2~50nm范围内,大孔和微孔很少。但3种处理方法对于坡缕石粘土的处理结果没有太大的差异。 相似文献
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文章根据我国地质勘查规范中有关饰面用灰岩工业指标与广西饰面用灰岩勘查与开发利用的不匹配案例,分析了广西饰面用灰岩勘查与开发利用的实际情况,认为有必要结合开发现状和市场需求,对饰面用灰岩矿产工业指标具体内容进行调整和灵活运用。 相似文献
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Effects of short flexible seagrass Zostera noltei on flow,erosion and deposition processes determined using flume experiments 下载免费PDF全文
Florian Ganthy Laura Soissons Pierre‐Guy Sauriau Romaric Verney Aldo Sottolichio 《Sedimentology》2015,62(4):997-1023
Innovative flume experiments were conducted in a recirculating straight flume. Zostera noltei meadows were sampled in their natural bed sediments in the field at contrasting stages of their seasonal growth. The aims of this study were: (i) to quantify the combined effects of leaf flexibility and development characteristics of Zostera noltei canopies on their interaction with hydrodynamics; and (ii) to quantify the role of Zostera noltei meadows in suspended sediment trapping and bed sediment resuspension related with changes in hydrodynamic forcing caused by the seasonal development of seagrasses. Velocity within the canopy was significantly damped. The attenuation in velocity ranged from 34 to 87% compared with bare sediments and was associated with a density threshold resulting from the flow‐induced canopy reconfiguration. The reduction in flow was higher in dense canopies at higher velocities than in less dense canopies, in which the reduction in flow was greater at low velocities. These contrasted results can be explained by competition between a rough‐wall boundary layer caused by the bed and a shear layer caused by the canopy. The velocity attenuation was associated with a two to three‐fold increase in bottom shear stress compared with unvegetated sediment. Despite the increase in near‐bed turbulence, protection of the sediment against erosion increased under a fully developed meadow, while sediment properties were found to be the main factor controlling erosion in a less developed meadow. Deposition fluxes were higher on the vegetated bed than on bare sediments, and these fluxes increased with leaf density. Fewer freshly deposited sediments were resuspended in vegetated beds, resulting in an increase in net sediment deposition with meadow growth. However, in the case of a very high leaf area index, sediment was mostly deposited on leaves, which facilitated subsequent resuspension and resulted in less efficient sediment trapping than in the less developed meadow. 相似文献