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运用已建立的气溶胶核化清除的物理化学模式,研究了云的动力学因子(如:气块上升速度、夹卷作用)对云滴化学非均匀性的影响。计算结果表明:较强烈的云发展(较大的气块上升速度)可加强由于气溶胶核化和云滴凝结增长造成的云滴化学的非均匀程度。夹卷作用抑制了云的发展,因而减弱了这种非均匀程度。夹卷作用同时也造成总体液态水中S(VI)、H+等浓度的增加,在Smax附近可达1个量级。如果考虑气溶胶粒子的夹卷,则可使气块内云滴污染物浓度随云滴大小的变化更加复杂化,如:不仅云滴污染物浓度随云滴大小而变化,即使对于相同大小的云滴之间,其污染物浓度也可相差很大。 相似文献
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Verification of our previous definition of preferred earthquake nucleation areas in Kanto-Tokai, Japan 总被引:2,自引:0,他引:2
We have proposed that points of future initiation of rupture may be mapped, based on minima in local recurrence times, which are equivalent to local maxima in the probability for main shocks to occur. These minima are often controlled by anomalously low b-values (logN = a − bM). Of the Kanto-Tokai area, approximately 12% showed anomalously short recurrence times and was proposed as asperities, based on seismicity up to 1999. During the period 1999–2003.5, about 75% of the earthquakes with M ≥ 3.5 fell into the asperities, earlier defined (for example 19 out of 23 M ≥ 3.8 events). The probability for this to occur by chance is approximately 2 10− 14. This supports our idea that the most likely volumes to produce main shocks may be mapped by minima in local recurrence times. 相似文献
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Mechanicalmodelofprecursorysourcepro┐cesforstrongearthquakesinwesternYun┐nanarea——conceptandnumericalsimula┐tionYOU-JINSU(苏有... 相似文献
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震源成核过程研究综述 总被引:5,自引:1,他引:5
大地震相应于断裂的快速传播。震源核是启动这个快速传播的断裂的动态体(或动态过程)。这个动态体或动态过程可以是震源端部的传播速度由慢渐快的裂缝,其内可有静态的或动态的应力化学腐蚀过程。可以是大震震源断层预滑时某处的突然快速失稳区,也可以是震源断层面上某一部分在临震前物性变弱而在其端部产生应力集中的一个动态体;另外,还可以是深部高压高温流体强迫插入积累巨大弹性应变能的地段的动态体。以上这些动态体或动态 相似文献
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Nucleation scavenging and the formation of a cloud interstitial aerosol (CIA) were theoretically studied in terms of the chemical composition of atmospheric aerosol particles. For this study, we used our air-parcel cloud model, which includes the entrainment of air and detailed microphysics, for determining the growth and interaction of aerosol particles and drops. Maritime and remote continental aerosol particle spectrums were used whose size distributions were superpositions of three log-normal distributions, each of a prescribed chemical composition. Our results show (1) that the CIA exhibits a size distribution with a distinctive cut-off at a specific radius of the dry as well as of the wet particle size distribution. All particles above this limiting size become activated to cloud drops and, thus, are not present in the CIA spectrum. This limiting size was found to be independent of the chemical composition of the particles and only dependent on the prevailing supersaturation. Below this specific size, the CIA spectrum becomes depleted of dry aerosol particles in a manner which does depend on their chemical composition and on the supersaturation in the air. (2) The number of aerosol particles nucleated to cloud drops depends critically on the chemical composition of the particles and on the prevailing supersaturation. 相似文献
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Growth of homogeneously nucleated water droplets: a quantitative comparison of experiment and theory
The formation of aerosols proceeds through nucleation, growth and aging stages. The understanding of nucleation and droplet growth is essential for handling the more complex atmospheric condensation processes. To achieve this goal, measurements of the nucleation rate of various systems are performed in an expansion chamber. In this manner nucleation and growth are decoupled by applying a short nucleation pulse of about 1 ms during which the nuclei are formed. The subsequent droplet growth is quantitatively monitored by Mie-scattering. To this end, the Mie-maxima and -minima are detected as a function of time and compared to theoretical Mie-scattering calculations for increasing radii. In this fashion, a wealth of growth curves for pure water depending on supersaturations, number densities of droplets, and temperatures were obtained. Following the approach of Fuchs and Sutugin [Fuchs, N.A., Sutugin, A.G., 1970. Highly Dispersed Aerosols. Ann Arbor Science Publishers, Ann Arbor; Fuchs, N.A., Sutugin, A.G., 1971. In: Hidy, G.M., Brock, J.R. (Eds.), International Reviews in Aerosol Physics and Chemistry: Topics in Current Aerosol Research (Part 2), Pergamon, New York, p. 1], we calculated theoretical growth curves taking into account the depletion of water vapor, the increase of droplet- and system-temperature, temperature-dependent functions of the diffusion coefficient, surface tension, liquid density and latent heat of condensation. The calculated growth curves and experimental data for 230, 240 and 250 K with number densities of droplets between 5×102 and 2×106 droplets/cm3 yield quantitative agreement between theory and experiment. This is remarkable in so far as the theory contains no adjustable parameters and assumes the sticking probability of the vapor molecules to be unity. Using a sticking probability smaller than 0.8 in the calculation leads to growth functions already outside the experimental error. 相似文献