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The solubility of iron sulphides in synthetic and natural waters at ambient temperature 总被引:1,自引:1,他引:0
W. Davison 《Aquatic Sciences - Research Across Boundaries》1991,53(4):309-329
A critical evaluation of literature values for the solubility products, K
sp
NBS
= [Fe2+][HS–] Fe2+
HS– (H
NBS
+
)–1, of various iron sulphide phases results in consensus values for the pKs of 2.95 ± 0.1 for amorphous ferrous sulphide, 3.6 ± 0.2 for mackinawite, 4.4 ± 0.1 for greigite, 5.1 ± 0.1 for pyrrhotite, 5.25 ± 0.2 for troilite and 16.4 ± 1.2 for pyrite.Where the analogous ion activity products have been measured in anoxic freshwaters in which there is evidence for the presence of solid phase FeS, the values lie within the range of 2.6–3.22, indicating that amorphous iron sulphide is the controlling phase. The single value for a groundwater of 2.65 (2.98 considering carbonate complexation) agrees. In seawater four values range between 3.85 to 4.2, indicating that mackinawite or greigite may be the controlling phase. The single low value of 2.94 is in a situation where particularly high fluxes of Fe (II) and S (–II) may result in the preferential precipitation of amorphous iron sulphide. Formation of framboidal pyrite in these sulphidic environments may occur in micro-niches and does not appear to influence bulk concentrations. Calculations show that the formation of Fe2S2 species probably accounts for very little of the iron or sulphide in most natural waters. Previously reported stability constants for the formation of Fe (HS)2 and (Fe (HS)3)– are shown to be suspect, and these species are also thought to be negligible in natural waters. In completely anoxic pore waters polysulphides also have a negligible effect on speciation, but in tidal sediments they may reach appreciable concentrations and lead to the direct formation of pyrite. Concentrations of iron and sulphide in pore waters can be controlled by the more soluble iron sulphide phase. The change in the IAP with depth within the sediment may reflect ageing of the solid phase or a greater flux of Fe (II) and S (–II) nearer the sediment surface. This possible kinetic influence on the value of IAPs has implications for their use in geochemical studies involving phase formation. 相似文献
14.
Landslide susceptibility mapping for a landslide-prone area (Findikli,NE of Turkey) by likelihood-frequency ratio and weighted linear combination models 总被引:17,自引:0,他引:17
Landslides are very common natural problems in the Black Sea Region of Turkey due to the steep topography, improper use of
land cover and adverse climatic conditions for landslides. In the western part of region, many studies have been carried out
especially in the last decade for landslide susceptibility mapping using different evaluation methods such as deterministic
approach, landslide distribution, qualitative, statistical and distribution-free analyses. The purpose of this study is to
produce landslide susceptibility maps of a landslide-prone area (Findikli district, Rize) located at the eastern part of the
Black Sea Region of Turkey by likelihood frequency ratio (LRM) model and weighted linear combination (WLC) model and to compare
the results obtained. For this purpose, landslide inventory map of the area were prepared for the years of 1983 and 1995 by
detailed field surveys and aerial-photography studies. Slope angle, slope aspect, lithology, distance from drainage lines,
distance from roads and the land-cover of the study area are considered as the landslide-conditioning parameters. The differences
between the susceptibility maps derived by the LRM and the WLC models are relatively minor when broad-based classifications
are taken into account. However, the WLC map showed more details but the other map produced by LRM model produced weak results.
The reason for this result is considered to be the fact that the majority of pixels in the LRM map have high values than the
WLC-derived susceptibility map. In order to validate the two susceptibility maps, both of them were compared with the landslide
inventory map. Although the landslides do not exist in the very high susceptibility class of the both maps, 79% of the landslides
fall into the high and very high susceptibility zones of the WLC map while this is 49% for the LRM map. This shows that the
WLC model exhibited higher performance than the LRM model. 相似文献
15.
Complexity theory has received considerable attention over the past decade from a wide variety of disciplines. Some who write on this topic suggest that complexity theory will lead to a unifying understanding of complex phenomena; others dismiss it as a passing and disruptive fad. We suggest that for the analysis of coupled natural/human systems, the truth emerges from the middle ground. As an approach focused as much on the connections among system elements as the elements themselves, we argue that complexity theory provides a useful conceptual framework for the study of coupled natural/human systems. It is, if nothing else, a framework that leads us to ask interesting questions about, for example, sustainability, resilience, threshold events, and predictability.In this paper we attempt to demystify the ongoing discussions on complexity theory by linking its evocative and overloaded terminology to real-world processes. We illustrate how a shift in focus from system elements to connections among elements can lead to meaningful insight into human-environment interactions that might otherwise be overlooked. We ground our discussion in ongoing interdisciplinary research surrounding Yellowstone National Park’s northern elk winter range; a tightly coupled natural/human system that has been the center of debate, conflict, and compromise for more than 135 years. 相似文献
16.
National flood discharge mapping in Austria 总被引:5,自引:0,他引:5
This article presents the approach and the results of a study in which 30, 100 and 200 year return period flood discharges
were estimated for 26,000 km of Austrian streams. Three guiding principles were adopted: combination of automatic methods
and manual assessments by hydrologists to allow speedy processing and account for the local hydrological situation; combination
of various sources of information including flood peak samples, rainfall data, runoff coefficients and historical flood data;
and involvement of the Hydrographic Services to increase the accuracy and enhance the acceptance of results. The flood discharges
for ungauged catchments were estimated by the Top-kriging approach with manual adjustment to the local flood characteristics.
The adopted combination approach proved to be very efficient both in terms of the project time required and in terms of the
accuracy and acceptability of the estimated flood discharges of given return periods. 相似文献
17.
18.
Effect of Cyclic Loading Frequency on Undrained Behaviors of Undisturbed Marine Clay 总被引:2,自引:0,他引:2
Based on a series of cyclic triaxial tests, the effect of cyclic frequency on the undrained behaviors of undisturbed marine clay is investigated. For a given dynamic stress ratio, the accumulated pore water pressure and dynamic strain increase with the number of cycles. There exists a threshold value for beth the accumulated pore water pressure and dynamic strain, below which the effect of cyclic frequency is very small, but above which the accumulated pore water pressure and dynamic strain increase intensely with the decrease of cyclic frequency for a given number of cycles. The dynamic strength increases with the increase of cyclic frequency, whereas the effect of cyclic frequency on it gradually diminishes to zero when the number of cycles is large enough, and the dynamic strengths at different frequencies tend to the same limiting minimum dynamic strength. The test results demonstrate that the reasons for the frequency effect on the undrained soil behaviors are beth the creep effect induced by the loading rate and the decrease of sample effective confining pressure caused by the accumulated pore water pressure. 相似文献
19.
根据现有1907—1990年南海大面调查资料,按1°×1°网格进行逐月的标准水层的温度统计。在此基础上采用3次样条函数的插值方法计算出整个南海温跃层的深度、厚度和强度并予以相应分析。分析表明,南海温跃层主要分为两种类型:第一类为辐射型,主要分布在南海北部的陆架区内,季节变化显著;第二类为不同水体叠置型,主要分布在广大深水区,它长年存在,季节变化较小。一种温跃层的一维积分预报模式,该模式是基于忽略热平流作用和水平热扩散的前提下,从局部热平衡方程出发,建立了受海面热收支及风混合作用下求解温度垂直分布及温跃层的时空变化。在南海北部水深约300m处进行了单站温跃层后报,结果表明,温跃层的深度、厚度和强度的相对误差均在30%以下。 相似文献
20.