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881.
本研究利用铵锌镉还原法将海水、湖水和自来水水体中硝酸盐转化为N2O气体测试氮、氧同位素, 结果表明当反应体系的pH值在6~8之间, NO3-还原为NO2-的转化率大于95%, NO2-还原为N2O的转化率大于99%。配置5种丰度的硝酸盐氮、氧同位素标样, 将实验结果与理论值绘制校准曲线, 氮同位素校准曲线斜率为0.48, 相关性良好(R2=0.999 8), 5种丰度δ15NN2O标准偏差在0.18‰~0.43‰之间(n=5);氧同位素校准曲线斜率为0.70, 相关性良好(R2=0.999 6), 5种丰度δ18ON2O标准偏差在0.27‰~0.46‰之间(n=5)。铵锌镉还原法与镉柱还原法测定硝酸盐氮、氧同位素结果的精密度和准确度一致, 同时海水、湖水和自来水3种不同类型水样的硝酸盐氮、氧同位素测试数据满足实验要求, 而且在实验流程的简洁性和高效性方面更具优势。 相似文献
882.
By combining the carbon cycle model with the records of carbonate and organic (kerogen) carbon isotope, this paper presents
the calculation of the fraction of organic carbon burial (f
org) of beds 23–40 at the global boundary stratotype section and point (GSSP) of the Permian-Triassic boundary at Meishan, Zhejiang
Province. The resulting calculation produces two episodes of f
org maxima observed to occur at beds 23–24 and 27–29, which respectively corresponds to the two episodic anoxic events indicated
by the flourish of green sulfur bacteria. Two episodic f
org minima occurred at beds 25–26 and 32–34, generally coincident with the flourish of cyanobacteria (bed 26 and upper part of
beds 29 to 34) as shown by the high value of 2-melthyhopnoanes. It appears that the f
org is related to the redox conditions, with greater f
org values observed under the reductive condition. The relationship between f
org and the total organic carbon (TOC) content was complex. The f
org value was low at some beds with a high TOC content (such as bed 26), while high observed at some beds with a low TOC content
(e.g. bed 27). This association infers the important contribution of primary productivity to the TOC content. The original
organic burial could be thus calculated through the configuration of the function of the primary productivity and f
org, which can be used to correct the residual TOC measured today. This investigation indicates that compiling the organic-inorganic
carbon isotopes with the carbon cycle model favors to understand the fraction of organic carbon burial, providing information
for the reconstruction of the coupling among biota, environments and organic burial.
Journal of China University of Geosciences, 2007, 32(6): 767–773 [译自: 地球科学—中国地质大学学报] 相似文献
883.
激光探针质谱分析碳酸盐碳、氧同位素技术 总被引:1,自引:1,他引:1
用激光显微装置和MAT 2 5 1质谱计原位分析碳酸盐的碳、氧同位素 ,与常规酸解法有同样的分析精度(标准偏差 0 .0 6‰~ 0 .0 8‰ ) ,δ1 3 C值无明显差异 ,而δ1 8O值比酸解法偏负约 1.11‰~ 1.2 3‰ ,可能是温度效应的结果 ,可以进行系统校正。 相似文献
884.
Zuoheng Zhang Jingwen Mao Jianmin Yang Zhiliang Wang Zhaochong Zhang 《Resource Geology》2003,53(2):101-114
Abstract. The Ta'ergou tungsten deposit in Gansu province, northwestern China, is located in the western part of the North Qilian Caledonian orogen, and consists of scheelite skarn bodies and wolframite quartz veins. The tungsten‐bearing skarn developed by the replacement of carbonate layers intercalated in the Precambrian schist and amphibolite whereas wolframite‐quartz ore veins developed along a group of fractures that cut through horizontal skarns. The Ta'ergou tungsten deposit is genetically related to the Caledonian Yeniutan granodiorite intrusion and occurs ca. 500 m wide in the exo‐contact zone 300 ~ 500 m apart from the intrusion. The granodiorite displays a lower grade of differentiation, low content of SiO2 and high contents of mafic components. There are three types of fluid inclusions in the wolframite‐quartz vein systems, i. e. aqueous, CO2‐H2O and CO2‐rich. The homogenization temperature of aqueous inclusion ranges from 140 to 380d?C and their salinities from 6.4 to 17.4 equivalent wt% NaCl. Laser Raman spectroscopy shows that the inclusions contain a relatively high content of CO2. The δ34S values of skarn type sulfides range from +8.1 to +12.7 per mil and those of quartz vein sulfides from +9.3 to +14.9 per mil, similar to sulfides of the granodiorite with from +6.0 to +11.7 per mil. The δ18O values of quartz are between +10.5 and +13.3 per mil and those of wolframite between +3.4 and +5.1 per mil. The δ18O water values of ore forming fluids range from +0.6 to +6.4 per mil and suggest the mixture of magmatic fluids with meteoric water formed the ore‐forming fluids. It has been proved that Precambrian strata in the west sector of North Qilian region are enriched in tungsten. We propose the strata were remelted to be tungsten‐granitoid during subduction. The polymetallic tungsten was gradually accumulated into the roof pendants of the granite intrusion by fractional crystallization and then was deposited by hydrothermal fluids during metasomatism and infilling along fractures. On the other hand, the granite intrusion also acted as “heating machine” to make hydrothermal fluids leach out the metals from Precambrian strata and these metals joined the ore‐forming hydrothermal system. 相似文献
885.
886.
试论胶东金成矿区成矿物质条件 总被引:9,自引:1,他引:9
对胶东群、粉子山群和蓬莱群的岩石学、地球化学等特征研究认为,胶东群是金的主要矿源层;粉子山群和煌斑岩脉也提供了部分金的来源。花岗质岩浆活动促使成矿物质转移。 相似文献
887.
888.
川西雀儿山花岗岩的地球化学和岩石成因 总被引:5,自引:1,他引:5
位于川西义敦岛弧北端的雀儿山花岗岩体主要由岩体边部或者作为包体的花岗闪长岩、主体似斑状花岗岩和较晚的呈条带状或者脉状伟晶质、细晶质花岗岩组成。这些花岗质岩石表现了较宽的常量元素变化范围,属于高钾钙碱性到shoshonite亚铝到过铝质岩石系列,表现了较平坦式具有负Eu异常的稀土配分模式。在原始地幔标准化的多元素图解上所有这些岩石表现Rb、Th和K等大离子亲石元素强烈富集,Nb、Sr、P和Ti等元素明显亏损。Sm-Nd同位素分析结果表明似斑状花岗岩亏损地幔模式年龄tDM=1.23~1.61Ga,εNd(t)=-5.3~-6.3,细晶花岗岩脉tDM=2.30Ga,εNd(t)=-6.9。这些岩石的εNd(t)分布在康定杂岩的Nd同位素演化范围内和上部。岩石地球化学和Nd同位素特征研究揭示其花岗岩岩浆起源于上部地壳杂砂岩、砂页岩和泥质岩石的部分熔融,经历了早期阶段的铁镁质矿物和副矿物的分离结晶,晚期钾长石等卷入了分离结晶。雀儿山花岗质岩浆活动发生于同碰撞到碰撞后隆升构造背景。 相似文献
889.
Hydrothermal Fluid Sources of the Fengjia Barite–fluorite Deposit in Southeast Sichuan,China: Evidence from Fluid Inclusions and Hydrogen and Oxygen Isotopes 下载免费PDF全文
The Fengjia barite–fluorite deposit in southeast Sichuan is a stratabound ore deposit which occurs mainly in Lower Ordovician carbonate rocks. Here we present results from fluid inclusion and oxygen and hydrogen isotope studies to determine the nature and origin of the hydrothermal fluids that generated the deposit. The temperature of the ore‐forming fluid shows a range of 86 to 302 °C. Our detailed microthermometric data show that the temperature during mineralization of the fluorite and barite in the early ore‐forming stage was higher than that during the formation of the calcite in the late ore‐forming stage. The salinity varied substantially from 0.18% to 21.19% NaCl eqv., whereas the density was around 1.00 g/cm3. The fluid composition was mainly H2O (>91.33%), followed by CO2, CH4 and traces of C2H6, CO, Ar, and H2S. The dominant cation was Na+ and the dominant anion Cl‐, followed by Ca2+, SO42‐, K+, and Mg2+, indicating a mid–low‐temperature, mid‐low‐salinity, low‐density NaCl–H2O system. Our results demonstrate that the temperature decreased during the ore‐forming process and the fluid system changed from a closed reducing environment to an open oxidizing environment. The hydrogen and oxygen isotope data demonstrate that the hydrothermal fluids in the study area had multiple sources, primarily formation water, as well as meteoric water and metamorphic water. Combined with the geological setting and mineralization features we infer that the stratabound barite–fluorite deposits originated from mid–low‐temperature hydrothermal fluids and formed vein filling in the fault zone. 相似文献
890.
The C and H isotopic compositions of the methane in more than 160 gas samples from 10 basins in China are presented in this paper.The natural gases are classified as four types: biogenic gas ,bio-thermocatalytic transitional gas, gas associated with condensate oil ,and coal-type gas. The isotopic compositions of these gases closely related to the depositional basins, the types of organic matter,the stages of thermal evolution and the genetic characteristics of different gas reservoirs.Studies of the C and H isotopic compositions of terrigenous natural gases will provide valua-ble information on the prospecting and development of natural gases of different genetic types. 相似文献