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301.
2013年以来几次严重的雾霾污染事件引起了公众的广泛关注,此后中国实施了一系列有关大气污染防治的政策、法规和措施来改善大气质量。为了分析近年来中国大气质量的时空变化特征,本文选取2015—2019年生态环境部国控站点监测的大气污染关键参数,对比分析了空气质量指数和6种大气污染物的季均、年均浓度变化结果,并利用组合指标分析法和相关分析法探讨了不同大气污染物之间的相关性。结果表明:① PM2.5、PM10、SO2、CO和NO2浓度和AQI均有明显下降,2019年均浓度较2015年均浓度分别下降4.5%、3.84%、7.86%、3.74%、0.95%,AQI下降了19.31%,同时,O3浓度则上升了0.79%;② 从空间分布来看,中国北方地区PM10、PM2.5、O3、NO2、SO2、CO年均质量浓度和AQI分别比南方地区高25.2%、18.73%、4.95%、17.6%,32.74%、16.17%、28.3%;③ 从季节性变化规律来看,除了O3呈现出夏季浓度高,冬季浓度低外,其他5种污染物和AQI都呈现相反的季节变化规律;④ 总体而言,目前中国大气污染以PM2.5和O3为主,PM2.5与NO2、SO2、CO之间有极显著的正相关关系(r>0.85,p<0.01),而O3与其前体物NO2和CO之间存在显著的负相关关系(r>0.8,p<0.01)。 相似文献
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Chemical elements and persistent organic pollutants (POPs) are globally present in aquatic systems and their potential transfer to loggerhead marine turtles (Caretta caretta) has become a serious threat for their health status. The environmental fate of these xenobiotics may be traced by the analysis of turtles’ tissues and blood. Generally, loggerhead turtles exhibited a higher metal load than other turtle species, this could be explained by differences in diet habits being food the main source of exposure. Literature shows that muscle, liver and kidney are most considered for the quantification of chemical elements, while, organic compounds are typically investigated in liver and fat.This paper is an overview of the international studies carried out on the quantification of chemical elements, polychlorinated biphenyls (PCBs), organochlorines (OCs) and perfluorinated compounds (PFCs), in tissues, organs and fluids of C. caretta from the Mediterranean Sea, the Atlantic and the Pacific Oceans. 相似文献
304.
Revealing the drivers and scale effects of water pollutant discharges is an important issue in the study of the environmental consequences during urban agglomeration evolution. It is also a prerequisite for realizing collaborative water pollutant reduction and environmental governance in urban agglomerations. This paper takes 305 counties in the Yangtze River Delta (YRD) as an example and selects chemical oxygen demand (COD) and ammonia nitrogen (NH3-N) as two distinctive pollutant indicators, using the Spatial Lag Model (SLM) and Spatial Error Model (SEM) to estimate the drivers of water pollutant discharges in 2011 and 2016. Then the Multiscale Geographically Weighted Regression (MGWR) model is constructed to diagnose the scale effect and spatial heterogeneity of the drivers. The findings show that the size of population, the level of urbanization, and the economic development level show global-level increase impacts on water pollutant discharges, while the level of industrialization, social fixed assets investment, foreign direct investment, and local fiscal decentralization are local-level impacts. The spatial heterogeneity of local drivers presents the following characteristics: Social fixed assets investment has a strong promoting effect on both COD and NH3-N discharges in the Hangzhou-Jiaxing-Huzhou region and the coastal area of the YRD; industrialization has a promoting effect on COD discharges in the Taihu Lake basin and Zhejiang province; foreign direct investment has a local inhibitory effect on NH3-N discharge, and the pollution halo effect is more prominent in the marginal areas of the YRD such as northern Jiangsu, northern Anhui, and southern Zhejiang; local fiscal decentralization has a noticeable inhibitory effect on COD discharge in the central areas of the YRD, reflecting the positive impacts on improved local environmental awareness and stronger constraints of multilevel environmental regulations in the urban agglomeration. Therefore, it is recommended to guide greener development to reduce the water pollutant discharge; to embed an environmental push-back mechanism in the fields of industrial production, capital investment, and financial income and expenditure; and to establish a high-quality development pattern of urban agglomerations systematically compatible with the carrying capacity of the water environment. 相似文献
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306.
有机污染物在改性黄土中的吸附和迁移滞后性研究 总被引:3,自引:0,他引:3
用阳离子表面活性剂十六烷基三甲基溴化铵(HDTMA-Br)和阴离子型表面活性剂十二烷基苯磺酸钠(SDBS)对黄土进行改性处理,并制备了一系列土壤样品。比较了甲苯在天然黄土和改性土中的不同吸附特性,并探讨了它们不同的吸附机理。通过比较甲苯在两类土壤中的吸附特性可以发现,等温吸附曲线均符合弗德里希方程式.但改性黄土的吸附能力为天然黄土的3—6倍。当同时用阴一阳离子表面活性剂进行黄土改性,吸附能力比单独使用阳离子表面活性剂改性的黄土增强15%-20%。土柱实验证明改性黄土对有机污染物对硝基苯胺的迁移具有明显的滞后性,使污染带前锋到达土柱出水口的时间延迟了50倍,也使土柱被穿透的时间延长了3.5倍。可见用表面活性剂对黄土改性能有效地在包气带滞留污染物。在一定程度上延缓或防止地面石油泄漏对含水层的污染。 相似文献
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308.
Marcus Schulz Olaf Büttner Martina Baborowski Michael Böhme Michael Matthies Wolf von Tümpling 《洁净——土壤、空气、水》2009,37(3):209-217
Beside damages of infrastructure in industrial regions, extreme floods can cause contamination with particle‐bound pollutants, e. g., due to erosion of soils and sediments. In order to predict contamination with inorganic pollutants, the transport and fate of arsenic, lead, and mercury during a fictive flood event of River Vereinigte Mulde in the region of Bitterfeld (Germany) with 200 years recurrence time was modeled. The finite element model system Telemac2D, which is subdivided into a hydrodynamic (Telemac‐2D), a transport (Subief‐2D), and a water quality module (wq2subief) was applied. The transport and water quality model models were calibrated using results of sediment trap exposures in the floodplain of River Vereinigte Mulde. Model results exhibited that the spatial patterns of particle‐associated arsenic and lead concentrations significantly changed. Extended, mostly agriculturally used areas showed arsenic and lead concentrations between 150 and 200 mg kg–1 and 250 and 300 mg kg–1, respectively, while urban areas were to a great extent spared from high contamination with arsenic and lead. Concentrations of particle‐associated mercury showed a pattern distinct from those of arsenic and lead. Outside of small patches with concentrations up to 63 mg kg–1, concentrations of particle‐associated mercury remained close to zero. Differences in the spatial patterns of the three pollutants regarded mainly arise from significantly different initial and boundary conditions. Sensitivity analyses of initial and boundary conditions revealed a high sensitivity of particle‐bound pollutant concentrations, whereas the sensitivities of concentrations of suspended sediments and soluble pollutants were mediocre to negligible. 相似文献
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310.
CHAO Na JI Dong-Sheng CHEN Jia-Shan XIN Jin-Yuan HU Bo WANG Yue-Si WANG Hui MENG Ze 《大气和海洋科学快报》2014,(4):340-345
Measurements of gaseous pollutants (03, NOx, SO2, and CO) were conducted at Dinghushan background station in southern China from January to December 2013. The levels and variations of O3, NOx, SO2, and CO were analyzed and their possible causes discussed. The annual average concentrations of 03, NOx, SO2, and CO were 24.6 ± 23.9, 12.8 ± 10.2, 4.0 ± 4.8, and 348 ± 185 ppbv, respectively. The observed levels of the gaseous pollutants are comparable to those at other background sites in China. The most obvious diurnal variation of 03 was observed in autumn, with minima in the early morning and maxima in the afternoon. The diurnal variations of SO2 showed high values during the day. The diurnal cycles of NOx showed higher values in the morning and lower values during the night. Higher CO concentrations were observed in spring followed by winter, autumn, and summer. Biomass burning, in combination with the transport of regional pollution, is an important source of CO, SO2, and NOx in spring and winter. Backward trajectories were calculated and analyzed together with corresponding pollutant concentrations. The results indicate that air masses passing over polluted areas are responsible for the high concentrations of gaseous pollutants at the Dinghushan background station. 相似文献