Mass Concentration and Mineralogical Characteristics of Aerosol Particles Collected at Dunhuang During ACE-Asia

Measurements were performed in spring 2001 and 2002 to determine the characteristics of soil dust in the Chinese desert region of Dunhuang, one of the ground sites of the Asia-Pacific Regional Aerosol Characterization Experiment (ACE-Asia). The mean mass concentrations of total suspended particle matter during the spring of 2001 and 2002 were 317 μg m?3 and 307 μg m?3, respectively. Eleven dust storm events were observed with a mean aerosol concentration of 1095 μg m?3, while the non-dusty days with calm or weak wind speed had a background aerosol loading of 196 μgm?3 on average in the springtime. The main minerals detected in the aerosol samples by X-ray diffraction were illite, kaolinite, chlorite, quartz, feldspar, calcite and dolomite. Gypsum, halite and amphibole were also detected in a few samples. The mineralogical data also show that Asian dust is characterized by a kaolinite to chlorite (K/C) ratio lower than 1 whereas Saharan dust exhibits a K/C ratio larger than 2. Air mass back-trajectory analysis show that three families of pathways are associated with the aerosol particle transport to Dunhuang, but these have similar K/C ratios, which further demonstrates that the mineralogical characteristics of Asian dust are different from African dust.     

“海葵”台风(1211号)暴雨雨滴谱特征分析

利用常规气象观测资料、加密自动气象观测站资料、NCEP/NCAR再分析资料以及安徽省滁州、黄山山底站地基雨滴谱观测资料,分析了2012年8月8-9日“海葵”台风暴雨过程的降水特征与环流背景,重点分析了该过程前后两个阶段(即台风本体造成的降水阶段与冷空气入侵引发的降水阶段)降水的雨滴谱特征。结果表明:(1)“海葵”台风降水过程中,安徽滁州站和黄山山底站平均谱谱宽都较大,均有6~8 mm的大降水粒子出现;黄山山底站具有更高的雨滴数浓度和较小的雨滴直径。(2)整个降水过程中,滁州站平均谱接近后一阶段的雨滴谱型,而黄山山底站平均谱接近前一阶段的雨滴谱型;不同雨强下两站的雨滴谱谱型基本相似,且随着降水强度增大,谱宽和雨滴数浓度均呈增大趋势。(3)前后两个降水阶段,滁州和黄山山底站表现出不同的滴谱特征。前一阶段,滁州站雨强(R)、雨滴质量加权平均直径(Dm)和标准化数浓度(Nw)的均值均小于黄山山底站;至后一阶段,滁州站的R、Dm明显增大,均大于黄山山底站。(4)从台风本体降水阶段到冷空气入侵降水阶段,滁州站雨滴谱型变化明显,呈现出谱宽由窄变宽且随雨滴直径增大而雨滴数浓度均增大的特点;黄山山底站雨滴谱型差异不大,表现出谱宽由宽变窄、雨滴数浓度随雨滴直径增大先增后减的特点。     

Concentration profiles of particles settling in the neutral and stratified atmospheric boundary layer

An expression for the vertical equilibrium concentration profile of heavy particles, including the effects of canopy on the eddy diffusivity as well as corrections for atmospheric stability, is proposed. This expression is validated against measurements of vertical concentration profiles of corn pollen above a corn field. The fitted theoretical profiles show that particle settling is correctly accounted for. The sensitivity to variations in the turbulent Schmidt number, settling velocity and stability corrections are explicitly characterized. The importance of independent measurements of the surface flux of pollen in future experiments is noted.     

营口市一氧化碳中毒事件发生日气象条件分析

利用近10 a营口市一氧化碳浓度监测资料和气象监测资料,分析了一氧化碳中毒事件发生与一氧化碳浓度的关系,探讨了一氧化碳中毒事件发生日的地面天气形势和局地气象条件特征。结果表明:一氧化碳中毒事件发生日空气中一氧化碳浓度值偏高;弱高压类、低压类和均压类天气形势均可能发生一氧化碳中毒事件;气压梯度小,风速小,气温变化小,不利于污染物扩散是造成一氧化碳中毒的主要原因。     

Vertical structures of PM10 and PM 2.5 and their dynamical character in low atmosphere in Beijing urban areas

The vertical structures and their dynamical character of PM2.5 and PM10 over Beijing urban areas are revealed using the 1 min mean continuous mass concentration data of PM2.5 and PM10 at 8, 100, and 320 m heights of the meteorological observation tower of 325 m at Institute of Atmospheric Physics, Chinese Academy of Sciences (IAP CAS tower hereafter) on 10―26 August, 2003, as well as the daily mean mass concentration data of PM2.5 and PM10 and the continuous data of CO and NO2 at 8, 100 (low layer), 200 (middle layer), and 320 m (high layer) heights, in combination with the same period meteorological field observation data of the meteorological tower. The vertical distributions of aerosols observed on IAP CAS tower in Beijing can be roughly divided into two patterns: gradually and rapidly decreasing patterns, I.e. The vertical distribution of aerosols in calm weather or on pollution day belongs to the gradually decreasing pattern, while one on clean day or weak cold air day belongs to the rapidly decreasing pattern. The vertical distributive characters of aerosols were closely related with the dynamical/thermal structure and turbulence character of the atmosphere boundary layer. On the clean day, the low layer PM2.5 and PM10 concentrations were close to those at 8 m height, while the concentrations rapidly decreased at the high layer, and their values were only one half of those at 8 m, especially, the concentration of PM2.5 dropped even more. On the clean day, there existed stronger turbulence below 150 m, aerosols were well mixed, but blocked by the more stronger inversion layer aloft, and meanwhile, at various heights, especially in the high layer, the horizontal wind speed was larger, resulting in the rapid decrease of aerosol concentration, I.e. Resulting in the obvious vertical difference of aerosol concentrations between the low and high layers. On the pollution day, the concentrations of PM2.5 and PM10 at the low, middle, and high layers dropped successively by, on average, about 10% for each layer in comparison with those at 8 m height. On pollution days, in company with the low wind speed, there existed two shallow inversion layers in the boundary layer, but aerosols might be, to some extent, mixed below the inversion layer, therefore, on the pollution day the concentrations of PM2.5 and PM10 dropped with height slowly; and the observational results also show that the concentrations at 320 m height were obviously high under SW and SE winds, but at other heights, the concentrations were not correlated with wind directions. The computational results of footprint analysis suggest that this was due to the fact that the 320 m height was impacted by the pollutants transfer of southerly flow from the southern peripheral heavier polluted areas, such as Baoding, and Shijiazhuang of Hebei Province, Tianjin, and Shandong Province, etc., while the low layer was only affected by Beijing's local pollution source. The computational results of power spectra and periods preliminarily reveal that under the condition of calm weather, the periods of PM10 concentration at various heights of the tower were on the order of minutes, while in cases of larger wind speed, the concentrations of PM2.5 and PM10 at 320 m height not only had the short periods of minute-order, but also the longer periods of hour order. Consistent with the conclusion previously drawn by Ding et al., that air pollutants at different heights and at different sites in Beijing had the character of "in-phase" variation, was also observed for the diurnal variation and mean diurnal variation of PM2.5 and PM10 at various heights of the tower in this experiment, again confirming the "in-phase" temporal/spatial distributive character of air pollutants in the urban canopy of Beijing. The gentle double-peak character of the mean diurnal variation of PM2.5 and PM10 was closely related with the evident/similar diurnal variation of turbulent momentum fluxes, sensible heat fluxes, and turbulent kinetic energy at various heights in the urban canopy. Besides, under the condition of calm weather, the concentration of PM2.5 and PM10 declined with height slowly, it was 90% of 8 m concentration at the low layer, a little lesser than 90% at the middle layer, and 80% at the high layer, respectively. Under the condition of weak cold air weather, the concentration remarkably dropped with height, it was 70% of 8 m concentration at the low layer, and 20%―30% at the middle and high layers, especially the concentration of PM2.5 was even lower.     

非常定自适应网格模式在台风路径数值预报中的应用

本文将作者在前文中介绍的非常定自适应网格模式用于台风路径的数值预报。由于自适应网格在台风中心附近安排了较密的网格，有效地提高了网格的分辨率，使得台风环流的结构在预报48小时以后仍能保持，其预报的路径与实况相比令人鼓舞。     

液态水含量和冰晶浓度对闪电频数影响的数值模拟研究

假定在软雹和冰晶碰撞的非感应起电机制为主要的起电机制成立的条件下，数值模拟研究了国际上公认的Fletcher和H—M冰晶产生机制以及云中的液态水含量对雷暴云放电过程（区分了云闪和地闪）的影响。结果表明，随着气压和温度的变化，在两种冰晶产生机制假定下，冰晶浓度分布有很大差异，这直接导致了雷暴云内电活动的差异。液态水含量的增加将使得首次放电时间延迟，同时将引起放电位置的下降和闪电频数的减少。     

煤层气在煤储层中的扩散及其影响因素

煤层气在煤储层中的扩散是指从煤基质孔隙表面上解吸的煤层气运移到割理系统的主要过程。发生扩散的前提条件是气体浓度差的出现，衡量扩散能力大小的重要参数是扩散系数。前者为由解吸速度、解吸气量和煤层气产量、井孔压力降等因素控制的动态参数，而后者为主要受扩散物质性质、扩散介质特征、扩散系统的温度、压力和孔隙结构形态等因素影响的静态参数。煤层气在煤储层中的扩散量与煤层气浓度差和扩散系数呈正比关系。     

中国东部主要河流稀土元素地球化学特征

在2007年底至2008年初的枯水期间,系统采集了中国东部流域面积和径流量较大的33条河流沉积物、悬浮颗粒物和水样,采用等离子质谱法、X荧光光谱法等方法测定了14种稀土元素含量以及常量组分和水体pH值等理化指标。研究发现中国河流稀土元素浓度总体高于世界均值,且南方河流沉积物、悬浮物稀土元素含量高于北方河流,南方河流悬浮物态中稀土、重稀土呈现一定程度的相对富集,与我国上地壳稀土丰度和稀土矿产种类的南北分异相吻合。展示了以中国东部泥质岩稀土元素丰度标准化后的稀土配分模式及Ce、Eu异常特征,发现河流沉积物的中、重稀土元素相对富集,悬浮物轻稀土相对富集,溶解相重稀土富集的特征;北方河流溶解相稀土元素浓度明显大于南方河流,且除小清河外,溶解相Eu不同于沉积物与悬浮物而呈强烈的正异常,主要与河水理化性质影响下的稀土分异有关。研究发现小清河等少数河流沉积物中稀土元素为异常高值,经Al标准化处理、计算拟合剩余值后,认为小清河等河流稀土元素已受人为污染的影响。     

Multi-scale Characteristics and Comprehensive Evaluation of Precipitation Heterogeneity in Guangxi

Aiming at the uneven spatial and temporal distribution of precipitation and frequent occurrence of drought and waterlogging disasters in Guangxi, the multi-scale characteristics and comprehensive evaluation of precipitation heterogeneity can provide scientific support for regional response to drought and waterlogging disasters and intelligent management of water resources. Based on the daily precipitation data of 87 grid points from 1961 to 2017 in Guangxi, the Precipitation Concentration Degree (PCD) and Precipitation Concentration Period (PCP) index were used to build day, pentad, ten days, month, season precipitation heterogeneity of multiple time scale level evaluation system. By using R/S analysis and geographical spatial analysis methods, the space-time evolution characteristics and climate division in Guangxi were discussed. The study showed that the spatial and temporal variation characteristics of PCD and PCP at the diurnal, synoptic and monthly scales were relatively consistent, and the heterogeneity of precipitation in Guangxi could be better expressed than that at the monthly and seasonal scales. The diachronic change of PCD in precipitation in Guangxi shows an increasing trend in northeast China and a decreasing trend in southwest China, and the trend of its future period is the same as the diachronic evolution. The spatial distribution of PCD in Guangxi has significant spatial autocorrelation and stratification heterogeneity, which are mainly reflected in the mean value, coefficient of variation and frequency of PCD. The comprehensive heterogeneity of precipitation in Guangxi is highly dispersed in the northeast, highly concentrated in the south, and slightly concentrated or dispersed in the northwest and central regions. The time-scale within a month is the best scale to express the non-uniformity of precipitation in Guangxi. If the advantages of more stable climatic and ten-day scales and more fine daily scales are taken into account, the use of climatic scale for daily sliding calculation and analysis will be the best way.