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971.
A laboratory inorganic carbonate precipitation experiment at high pH of 8.96 to 9.34 was conducted, and the boron isotopic
fractionations of the precipitated carbonate were measured. The data show that boron isotopic fractionation factors (αcarb-3) between carbonate and B(OH)3 in seawater range 0.937 and 0.965, with an average value of 0.953. Our results together with those reported by Sanyal and
collaborators show that the αcarb-3 values between carbonate and B(OH)3 in solution are not constant but are negatively correlated with the pH of seawater. The measured boron isotopic compositions
of carbonate precipitation (δ11Bcarb) do not exactly lie on the best-fit theoretical δ11B4-pH curves and neither do they exactly parallel any theoretical δ11B4-pH curves. Therefore, it is reasonable to argue that a changeable proportion of B(OH)3 with pH of seawater should also be incorporated into carbonate except for the dominant incorporation of B(OH)4
− in carbonate. Hence, in the reconstruction of the paleo-pH of seawater from boron isotopes in marine biogenic carbonates,
the use of theoretical boron isotopic fractionation factor (α4−3) between B(OH)4
− and B(OH)3 is not suitable. Instead, an empirical equation should be established.
Supported by National Natural Science Foundation of China (Nos. 40573013 and 40776071), State Key Laboratory of Loess and
Quaternary Geology, Institute of Earth Environment, Chinese Academy of Sciences (Grant No SKLLQG0502) and State Key Laboratory
of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences 相似文献
972.
《中国科学D辑(英文版)》2008,(Z2)
The quality of the Ordovician carbonate reservoir beds in the Tarim Basin is closely related to the development of secondary pores,fractures and cavities. Karstification is important in improving the properties of reservoir beds,and karstification related to unconformity has caught wide attention. Compared with the recent research on the unconformity karst reservoir bed improvement,this paper shows a new way of carbonate reservoir bed transformation. Based on field survey,core and slices observation,transformation of Ordovician carbonate reservoir beds by faulting can be classified into three types: (1) Secondary faults and fracturs generated by faulting improved carbonate reservoir bed properties,which were named the Lunnan or Tazhong82 model; (2) upflow of deep geothermal fluids caused by faulting,with some components metasomatizing with carbonate and forming some secon-dary deposit,such as fluorite. It can improve carbonate reservoir bed properties obviously and is named the Tazhong 82 model; and (3) the faulting extending up to the surface increased the depth of supergene karstification and the thickness of reservoir bed. It is named the Hetianhe model. Trans-formation effect of carbonate reservoir beds by faulting was very significant,mainly distributed on the slopes or on the edge or plunging end of the uplift. 相似文献
973.
通过对东北太平洋胡安·德富卡隆起西翼沉积柱样中的碳酸盐含量和浮游有孔虫氧同位素测试以及浮游有孔虫丰度、溶解指数和粗组分的统计,发现在晚第四纪约65 ka以来碳酸盐含量变化幅度大(0 4%~77 2%),相差非常悬殊,但其变化未呈现出冰期时溶解作用减弱、间冰期时溶解作用强烈这样明显的旋回性。粗组分分析结果显示,地层中有明显的浊流沉积发育。另外,碳酸盐含量和浮游有孔虫丰度分析结果揭露了研究区的 CCD在3 500 m左右。研究认为,在约65 ka来水深浅于3 500 m的区域碳酸盐含量的无规律性变化应与浊流沉积影响有直接的关系,而水深深于3 500 m的区域碳酸盐含量主要受控于深海碳酸盐的溶解作用。 相似文献
974.
975.
Influence of partial confinement and Holocene river formation on groundwater flow and dissolution in the Florida carbonate platform
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Much of what is known about groundwater circulation and geochemical evolution in carbonate platforms is based on platforms that are fully confined or unconfined. Much less is known about groundwater flow paths and geochemical evolution in partially confined platforms, particularly those supporting surface water. In north‐central Florida, sea level rise and a transition to a wetter climate during the Holocene formed rivers in unconfined portions of the Florida carbonate platform. Focusing on data from the Santa Fe River basin, we show river formation has led to important differences in the hydrological and geochemical evolution of the Santa Fe River basin relative to fully confined or unconfined platforms. Runoff from the siliciclastic confining layer drove river incision and created topographic relief, reorienting the termination of local and regional groundwater flow paths from the coast to the rivers in unconfined portions of the platform. The most chemically evolved groundwater occurs at the end of the longest and deepest flow paths, which discharge near the center of the platform because of incision of the Santa Fe River at the edge of the confining unit. This pattern of discharge of mineralized water differs from fully confined or unconfined platforms where discharge of the most mineralized water occurs at the coast. Mineralized water flowing into the Santa Fe River is diluted by less evolved water derived from shorter, shallower flow paths that discharge to the river downstream. Formation of rivers shortens flow path lengths, thereby decreasing groundwater residence times and allowing freshwater to discharge more quickly to the oceans in the newly formed rivers than in platforms that lack rivers. Similar dynamic changes to groundwater systems should be expected to occur in the future as climate change and sea level rise develop surface water on other carbonate platforms and low lying coastal aquifer systems. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
976.
正20141538 Cao Qing(School of Earth Sciences and Engineering,Xi’an Petroleum University,Xi’an 710065,China);Zhao Jingzhou Characteristics and Significance of Fluid Inclusions from Majiagou Formation,Yichuan Huangling Area,Ordos Basin(Advances in Earth Science,ISSN1001-8166,CN62-1091/P,28(7),2013,p.819-828,7 illus.,3 tables,43 refs.) 相似文献
977.
H. MIZUOCHI M. SATISH‐KUMAR Y. MOTOYOSHI K. MICHIBAYASHI 《Journal of Metamorphic Geology》2010,28(5):509-526
Calcite–dolomite solvus geothermometry is a versatile method for the estimation of metamorphic temperature because of its simplicity. However, in medium‐ to high‐grade metamorphic rocks the accuracy of estimating temperature by the integration of unmixed dolomite and calcite is hampered by the heterogeneous distribution of unmixed dolomite, difficulties in distinguishing between preexisting and exsolved dolomite and demarcating grain boundaries. In this study, it is shown that calcite–dolomite solvus thermometry can be applied to calcite inclusions in forsterite and spinel for the estimation of peak metamorphic temperature in granulite facies marbles from Skallevikshalsen, East Antarctica. The marbles are comprised of a granoblastic mineral assemblage of calcite + dolomite + forsterite + diopside + spinel + phlogopite ± apatite, characteristic of granulite facies metamorphic conditions. Forsterite, spinel and apatite frequently contain ‘negative crystal’ inclusions of carbonates that display homogeneously distributed dolomite lamellae. On the basis of narrow ranges of temperature (850–870 °C) recorded from carbonate inclusions compared with the range from matrix carbonate it is regarded that the inclusion carbonates represent a closed system. Furthermore, this estimate is consistent with dolomite–graphite carbon isotope geothermometry, and is considered to be the best estimate of peak metamorphic temperature for this region. Matrix calcite records different stages of retrograde metamorphism and re‐equilibration of calcite that continued until Mg diffusion ceased at ~460 °C. Electron backscattered diffraction (EBSD) results together with morphological features of unmixed coarse tabular dolomite suggest anisotropic diffusion and mineral growth are influenced by crystallographic orientation. Identification of sub‐grain boundaries and formation of fine‐grained unmixing in calcite rims suggest the presence of grain boundary fluids in the late retrograde stages of metamorphic evolution. These results, thus, demonstrate the usefulness of carbonate inclusion geothermometry in estimating the peak metamorphic temperatures of high‐grade terranes and the application of EBSD in understanding the unmixing behaviour of minerals with solid solutions. 相似文献
978.
碳酸盐矿物是火山岩储层内重要的矿物成分,长岭断陷火山岩储层内的自生碳酸盐矿物主要是方解石.本文通过对营城组储层内方解石矿物的碳氧同位素特征分析,探讨储层内碳酸盐矿物成因.研究表明,长岭断陷火山岩储层内方解石δ13 CV-PDB值范围为-12.7‰~0.4‰,δ18OV-SMOw值范围为3.8‰~12‰,具有高δ18O值.与方解石平衡的CO2碳同位素计算值范围较宽,为-16.0‰~2.2‰,表明其形成物质的多源性.在δ18 O-δ13C图解中显示,形成碳酸盐矿物的CO2来源于幔源-岩浆无机成因的CO2和有机质演化过程中产生的CO2,以无机成因CO2源为主.这些无机成因CO2、有机成因CO2和沉积有机质热演化产生的有机酸溶于流体,形成酸性流体.火山岩储层中碳酸盐矿物的形成实质就是这种酸性流体与储层围岩反应的结果. 相似文献
979.
980.
应用野外工作和室内研究相结合的方法,从储层的岩石学和储集空间等角度对塔中地区储层特征进行了研究。研究表明,研究区内良里塔格组灰岩段岩性主要为颗粒灰岩、骨架礁灰岩、藻粘结灰岩、泥晶灰岩、岩溶角砾岩等,其中颗粒灰岩大多经历了多期多成因成岩作用改造,裂缝较为发育;泥晶灰岩中多期压溶作用和白云石化作用较为常见;藻粘结灰岩受成岩作用改造相对最弱。宏观储集空间主要包括大型溶洞、孔洞及裂缝,其中孔洞多呈孤立、稀疏并沿裂缝分布;构造缝是裂缝的主要类型。微观储集空间主要包括溶孔和微裂缝,其中溶孔主要发育在亮晶颗粒灰岩中,可细分为粒内溶孔、粒间溶孔、晶间溶孔、铸模孔、溶蚀骨架孔、残余粒间孔及沿裂缝扩溶形成的溶孔,粒间溶孔所占比例最高。埋藏期溶蚀作用发育期次多,规模大,分布广泛,对储层物性的改善和油气聚集的影响最为明显。 相似文献