质量传输和同位素交换:流动几何学和交换机制

耦合的质量传输和动力学限制的同位素交换模型综合考虑了平流、扩散、热液弥散 ,以及岩石与水之间的不平衡同位素交换等项因素。把耦合模型应用于 2个构造环境下的古热液系统 ,进而解释稳定同位素数据。对于造成环绕浅成侵入岩体分布的18O亏损环带的流体的流动几何学 ,以及浅部正断层流体流动的几何学 ,耦合模型提供了不同于单一同位素交换模型的解释。耦合模型也提供了关于同位素相对交换速率和同位素交换机制的信息。结果表明 ,断层带的动态重结晶促进了表面反应 ,进而便利了同位素交换 ;在化学不反应性和未变形的矿物中 ,同位素交换可能受制于固态条件下的扩散。     

Scale effects of eroded sediment transport in Wujiang River Basin,Guizhou Province,China

In recent years, research on spatial scale and scale transformation of eroded sediment transport has become a forefront field in current soil erosion research, but there are very few studies on the scale effect problem in Karst regions of China. Here we quantitatively extracted five main factors influencing soil erosion, namely rainfall erosivity, soil erodibility, vegetative cover and management, soil and water conservation, and slope length and steepness. Regression relations were built between these factors and also the sediment transport modulus and drainage area, so as to initially analyze and discuss scale effects on sediment transport in the Wujiang River Basin (WRB). The size and extent of soil erosion influencing factors in the WRB were gauged from: Advanced Spaceborne Thermal Emission and Reflection Radiometer Global Digital Elevation Model (ASTER GDEM), precipitation data, land use, soil type and Normalized Difference Vegetation Index (NDVI) data from Global Inventory Modeling and Mapping Studies (GIMMS) or Advanced Very High Resolution Radiometer (AVHRR), and observed data from hydrometric stations. We find that scaling effects exist between the sediment transport modulus and the drainage area. Scaling effects are expressed after logarithmic transformation by a quadratic function regression relationship where the sediment transport modulus increases before decreasing, alongside changes in the drainage area. Among the five factors influencing soil erosion, slope length and steepness increases first and then decreases, alongside changes in the drainage area, and are the main factors determining the relationship between sediment transport modulus and drainage area. To eliminate the influence of scale effects on our results, we mapped the sediment yield modulus of the entire WRB, adopting a 1 000 km2 standard area with a smaller fitting error for all sub-basins, and using the common Kriging interpolation method.     

The influence of grain-size analysis methods and sediment mixing on curve shapes and textural parameters: Implications for sediment trend analysis

To this day, deterministic physical models capable of explaining the evolution of grain-size distributions in the course of transport are still lacking. For this reason, various attributes of particle frequency distributions, in particular curve shapes and textural parameters, have for many decades been investigated for potential information about transport behaviour and size-sorting processes of sediments in numerous environments. Such approaches are essentially conceptual and hence rely heavily on the validity of the assumptions on which they are based. A factor which has to date been largely ignored in this context, is the fact that different methods of grain-size analysis (e. g. sieving, laser absorption and diffraction, settling velocity measurements), when applied to the same sample material, produce variable curve shapes, and hence incongruous textural data. This is illustrated by selected examples showing the differences between sieving and settling results, conversion of settling velocities into equivalent settling diameters (psi-phi-transformations), and the influences of particle shape, particle density, and water temperature. It is demonstrated that particle-size distributions are not only method-dependent but also dependent on the adopted post-processing procedure. As a result, only frequency curves generated by the same method and subsequently processed by identical computational procedures can be meaningfully compared. Furthermore, the computation of textural parameters from bi- or multimodal size distributions produces spurious results which are unrelated to the processes leading to the mixing of different size populations frequently observed in nature. In such cases, only the decomposition of such distributions into individual populations and the spatial comparison of such populations makes any sense. Because a physical explanation for the generation of size distributions is lacking, a particular curve shape of a grain-size population has no meaning on its own. Only a systematic comparison of progressively changing curve shapes (and associated textural parameters) of sediments collected on a closely spaced grid can yield data suitable for sediment trend analysis.     

黄河中游一次致洪暴雨过程的形成机理

利用常规观测资料、NCEP再分析资料等,对黄河中游2013年7月21-22日的致洪暴雨过程的形成机理进行分析。结果发现:1)地面辐合线的形成和维持是本次过程降水强度大和降水集中的主要原因。中尺度雨团和地面中尺度辐合线相对应,地面中尺度辐合线的形成和冷空气扩散补充相对应。第一次冷空气扩散,促使长武站附近地面中尺度辐合线的形成和维持;第二次冷空气补充,促使北洛河流域、无定河流域的地面中尺度辐合线形成并维持。2)暴雨过程发生前,其上空存在干暖盖的结构特征,是能量积累及位势不稳定层结结构建立的关键;暴雨发生过程中干空气侵入对中尺度对流云团起激发作用。3)暴雨、大暴雨发生过程中水汽的垂直输送明显,暴雨区上空1000-100 h Pa相对湿度均在90%以上。     

RELATIONSHIPS BETWEEN SPRING KUROSHIO SSTA AND SUMMER RAINFALL IN CHINA

Based on the data of SST and NCEP/NCAR reanalysis data, the relationship is analyzed of spring SSTA in the Kuroshio region with summer precipitation in China, summer 500 hPa field and water vapor transport, using the methods of Morlet wave, correlation and composite analysis. The results show that annual and interdecadal change of spring SST in the Kuroshio region is distinct. Spring SST displays a significantly increasing trend and there exist different periodic oscillations in the Kuroshio region, with the 23-year periodic oscillation being the most obvious. Troughs and ridges in the mid- and higher- latitudes turn deeper in high Kuroshio SSTA years. At the same time, the western Pacific subtropical high strengthens and stretches westwards. As a result, the warm / wet air from the west of the subtropical high locates in the mid- and lower- reaches of the Yangtze River and south China and summer rainfall in the above regions increases accordingly. Composite anomalous water vapor flux fields indicate that the vapor transport from the South China Sea and western Pacific and the vapor from the north converge over the mid- and lower- reaches of the Yangtze River and south China, which results in the increase of the summer rainfall in the mid- and lower- reaches of the Yangtze River and south China. On the contrary, the summer rainfall in the mid- and lower- reaches of the Yangtze River and south China decreases correspondingly in low Kuroshio SSTA years.     

中国西北干旱区戈壁下垫面夏季的热力输送

以敦煌戈壁站2004年6月和2008年8月的常规观测和超声观测为例,分析了西北干旱区戈壁下垫面夏季热力输送的一般过程及特征。首先评价了湍流通量的观测质量以及仪器观测的地表能量通量闭合问题,结果表明敦煌戈壁站的观测在白天总体较好。夏季地表能量通量的平均日变化显示,潜热通量整天都很小,可以忽略,白天到达地表的短波辐射以及地表向上的长波辐射非常强,地表净辐射主要转化为感热输送（敦煌戈壁站在中午时平均分别达380W·m-2以上和250W·m-2以上）;夜间土壤释放热量以平衡地表的辐射冷却,感热通量略低于0。白天时地表大气经常触发自由对流活动,影响动量通量的观测质量,并有效输送地表热力至上层大气中,有助于形成超厚大气边界层。分析了戈壁下垫面的动量粗糙度特征和热力粗糙度特征（敦煌戈壁站动量粗糙度约为0．6mm）,热力粗糙度基本小于动量粗糙度一个量级,这符合目前对干旱区戈壁下垫面热力输送特征的初步认识。     

江西2012年5月12日大暴雨过程水汽输送分析

利用NCEP 1°×1°再分析资料、常规气象观测资料和WRF中尺度数值模式,对2012年5月12日江西出现的大暴雨天气水汽输送的过程进行分析。结果表明,从大尺度分析,此次暴雨过程的水汽输送特征并不典型,比湿、水汽通量、水汽通量散度、整层水汽输送等均不能满足江西出现暴雨时应该达到的水汽条件;但模拟的中小尺度水汽指数能够满足江西发生暴雨的水汽条件。此次暴雨过程的水汽主要来自南海地区。暴雨出现的区域与整层水汽大值区的水平梯度最大处相吻合。当整层水汽输送值较小时,水汽输送主要集中在中低层,但当整层水汽输送值较大时,水汽输送的高度高度超过500 hPa高度层,仅分析500 hPa高度层以下的水汽输送对暴雨预报会造成一定的误差。     

嵌套网格空气质量预报模式系统的发展与应用

主要综述中国科学院大气物理研究所自主开发的嵌套网格空气质量预报模式系统(NAQPMS,Nested Air Quality Prediction Modeling System)的历史发展与应用情况.模式发展伊始为欧拉污染物输送实用模型,利用其研究东亚硫氧化物的跨国输送问题,得出中国对于周边国家的输送量不大的结论; 在系统中嵌入适合东亚的起沙机制模块,用来模拟沙尘发生、输送及沉降等过程,估算亚洲大陆沙尘气溶胶对海洋地区的输送与沉降通量,为研究海洋生物地球化学循环提供基础数据; 利用该系统研究沙尘及其土壤粒子对酸雨的中和作用,发现沙尘输送对东亚酸雨的分布影响很大; 发展城市尺度高分辨率气象和空气质量预报技术,使模式水平分辨率达到500 m,并应用于台北高浓度臭氧和PM10的模拟; 研究和集成区域及城市尺度大气污染预报理论和模拟技术,研制成目前的嵌套网格空气质量预报模式系统,以探讨不同尺度各种污染(如沙尘暴、城市光化学烟雾、酸雨、高浓度悬浮颗粒物等)的变化规律.在模式系统中初步建立资料同化模块,开展大气化学成分及沙尘输送模拟的资料同化研究.系统已经在北京、上海、深圳、郑州等城市环境监测中心实施空气质量的实时预报.未来,系统将集成到全球环境大气输送模式(GEATM),以实现从城市群到全球具有双向耦合功能的模式系统.     

COMPARISON OF AEROSOL CHARACTERISTICS OVER MAINLAND OF CHINA AND WESTERN PACIFIC AND ITS LONG-RANGE TRANSPORT

Based on the aerosol data obtained at Shangdianzi regional background monitoring station together withthe air trajectory analysis,the chemical constituents of the aerosol from the different sources are discussed andcompared with the aerosol samples collected over the western Pacific.The results show that the relative massconcentrations of the crustal and pollutant elements in the aerosol collected over the ocean are higher than thosebeing observed at Shangdianzi in particle size above 4.7 μm and below 0.65μm in diameter.The variationsof the enrichment factors of these elements in marine aerosol with particle size are different from those in shang-dianzi's samples.The former enrichment factors are evidently higher than the latter above 1.1 μm in diameter.On the basis of the comparative research,the long-range transport processes of aerosol particles are discussed.     

Satellite and ground observations for large-scale air pollution transport in the Yellow Sea region

Large-scale air pollution transport (LSAPT) in the Yellow Sea region and their inflow onto the Korean Peninsula were observed through satellite images and ground measurements. LSAPT includes regional continental air-masses saturated with pollutants originating from China and subsequently landing on or passing through the Korean Peninsula. It is also possible to identify the distribution and transport patterns of LSAPT over the Yellow Sea. The ground concentrations for PM10, PM2.5 and CO measured at Cheongwon, located in the centre of south Korea, were compared with NOAA satellite images. Notably, the episodes observed of the LSAPT show a PM2.5 to PM10 ratio of 74% of the daily maximum concentrations. However, cases of duststorms were clearly distinguished by much higher PM10 concentrations and a ratio of 30% of PM2.5 to PM10 for daily maximum concentrations. For the episode on January 27, 2006, the inflow of a regionally polluted continental air-mass into the central and southwestern regions of the Korean Peninsula was observed sequentially at various ground observatories as well as by satellite. The north airflow dissipated the clouds over Mt. Halla on Jeju Island and further downwind, reducing air pollution and creating a von Kármán vortex.