对流层氮氧化物光化学转化特征研究

应用大气光化学模式研究了日间影响NOx光化学转化率的主要物理化学因子.探讨了在不同NMHC/NOx比值时,NOx光化学特征及其转化产物的变化规律.结果表明,影响NOx转化率的主要因子是阳光辐射强度和NMHC/NOx比值.但在NMHC/NOx比值很低时,光强的增加并不能显著提高NOx转化率.温度和初始臭氧浓度对NOx转化率的影响次之.相对湿度对NOx转化率的影响较小.在不同NMHC/NOx比值下,NOx转化特征和产物有很大区别.NMHC/NOx比值高时,产物中PAN＞HNO3.NMHC/NOx比值中(低)时,产物主要是HNO3,PAN等有机氮不到10%(1%).最后初步比较了模拟和观测的NOy组成.     

城市适应气候变化能力评价—以朝阳市为例

利用朝阳市1961—2016年气温、降水资料和2007—2016年社会经济资料,采用层次分析法（AHP）构建了基于气候系统和城市系统的城市适应气候变化能力评价指标体系,根据综合指数评价结果将适应能力分为五个等级,定量评估了2007—2016年朝阳市气候系统危险度、城市系统适应度以及城市适应气候变化能力动态变化。结果表明：2007—2016年朝阳市气候系统危险度显著增加,危险度由“较低”水平至“一般”水平,气候系统危险度的增加主要是由气象灾害和极端气候危险度增加造成的;随着经济发展和城市公共服务不断完善,朝阳市城市系统适应度稳步提升,由“低”水平提高至“高”水平;在气候系统和城市系统共同作用下,朝阳市城市适应气候变化能力显著提高,年增加率为0.029,综合能力由“较低”水平提升至“较高”水平。     

THERMAL FORCING IMPACTS OF THE EASTERLY VORTEX ON THE EAST-WEST SHIFT OF THE SUBTROPICAL ANTICYCLONE OVER WESTERN PACIFIC OCEAN

By employing the NCEP/NCAR reanalysis data sets(1 000 to 10 hPa,2.5°× 2.5°),the thermal forcing impacts are analyzed of an easterly vortex(shortened as EV) over the tropical upper troposphere on the quasi-horizontal movement of the Western Pacific Subtropical Anticyclone(shortened as WPS A) during 22-25 June 2003.The relevant mechanisms are discussed as well.It is shown that the distribution and intensity of the non-adiabatic effect near the EV result in the anomalous eastward retreat of the WPSA.The WPSA prefers extending to the colder region,i.e.,it moves toward the region in which the non-adiabatic heating is weakening or the cooling is strengthening.During the WPSA retreat,the apparent changes of non-adiabatic heating illustrate the characteristics of enhanced cooling in the east side of the EV.Meanwhile,the cooling in the west side exhibits a weakened eastward trend,most prominently at 300 hPa in the troposphere.The evidence on the factors causing the change in thermal condition is found:the most important contribution to the heating-rate trend is the vertical transport term,followed in turn by the local change in the heating rate term and the horizontal advection term.As a result,the atmospheric non-adiabatic heating generated by the vertical transport and local change discussed above is mainly connected to the retreat of the WPSA.     

华北平原冬麦田土壤CH4的吸收特征研究

利用静态箱/气相色谱(GC)法,对华北平原冬小麦拔节—成熟期间麦田土壤CH4气体通量进行了测定,得出华北平原典型冬麦田土壤是大气CH4的弱吸收汇。试验期间土壤CH4通量存在明显的季节变化和日变化,麦田拔节—成熟期间土壤CH4通量日平均值为-18.3μg.m-2.h-1,波动范围为-4.3~-24.4μg.m-2.h-1;在土壤CH4通量的日变化中,观测到麦田土壤在午间和夜间都有一个吸收峰,峰值出现的时间因生育期不同而有所不同。试验期间CH4通量日平均值与土壤温度关系不明显,而与土壤水分呈负相关(α=0.01);日变化中土壤CH4通量与地表温度的相关性较差,而与5 cm地温相关密切。麦田拔节—成熟期间土壤CH4通量日平均值随NH4 -N施用量的增加呈递减规律,农田秸秆还田后不利于土壤对CH4的吸收。     

The Effects of Line-Wing Cutoff in LBL Integration on Radiation Calculations

There are three basic methods in radiative transfer calculations, i.e., line-by-line (LBL) integration, correlated k-distribution method, and band model. The LBL integration is the most accurate of all, in which, there are two quadrature algorithms named in this paper as integration by lines and by sampling "points when calculating atmospheric transmittance in the considered wavenumber region. Because the LBL integration is the most expensive of all, it is necessary and important to save calculation time but increase calculation speed when it is put into use in the daily operation in atmospheric remote sensing and atmospheric sounding. A simplified LBL method is given in this paper on the basis of integration by lines, which increases computational speed greatly with keeping the same accuracy. Then, we discuss the effects of different cutoff schemes on atmospheric absorption coefficient, transmittance, and cooling rate under both of accurate and simplified LBL methods in detail. There are four cutoff schemes described in this paper, i.e., CUTOFFs 1, 2, 3, and 4. It is shown by this numerical study that the way to cut off spectral line-wing has a great effect on the accuracy and speed of radiative calculations. The relative errors of the calculated absorption coefficients for CUTOFF 2 are the largest under different pressures, while for CUTOFF 1, they are less than 2% at most of sampling points and for CUTOFFs 3 or 4, they are ahnost less than 5% in the calculated spectral region, however, the calculation time is reduced greatly. We find in this study that the transmittance in the lower atmosphere is not sensitive to different LBL methods and different cutoff schemes. Whereas for the higher atmosphere, the differences of transmittance results between CUTOFF 2 and each of other three cutoff schemes are the biggest of all no matter for the accurate LBL or for the simplified LBL integrations. By comparison, the best and optimized cutoff scheme is given in this paper finally.     

Earth System Model FGOALS-s2: Coupling a dynamic global vegetation and terrestrial carbon model with the physical climate system model

Earth System Models （ESMs） are fundamental tools for understanding climate-carbon feedback. An ESM version of the Flexible Global Ocean-Atmosphere-Land System model （FGOALS） was recently developed within the IPCC AR5 Coupled Model Intercomparison Project Phase 5 （CMIP5） modeling framework, and we describe the development of this model through the coupling of a dynamic global vegetation and terrestrial carbon model with FGOALS-s2. The performance of the coupled model is evaluated as follows. The simulated global total terrestrial gross primary production （GPP） is 124.4 PgC yr-I and net pri- mary production （NPP） is 50.9 PgC yr-1. The entire terrestrial carbon pools contain about 2009.9 PgC, comprising 628.2 PgC and 1381.6 PgC in vegetation and soil pools, respectively. Spatially, in the tropics, the seasonal cycle of NPP and net ecosystem production （NEP） exhibits a dipole mode across the equator due to migration of the monsoon rainbelt, while the seasonal cycle is not so significant in Leaf Area Index （LAI）. In the subtropics, especially in the East Asian monsoon region, the seasonal cycle is obvious due to changes in temperature and precipitation from boreal winter to summer. Vegetation productivity in the northern mid-high latitudes is too low, possibly due to low soil moisture there. On the interannual timescale, the terrestrial ecosystem shows a strong response to ENSO. The model- simulated Nifio3.4 index and total terrestrial NEP are both characterized by a broad spectral peak in the range of 2-7 years. Further analysis indicates their correlation coefficient reaches -0.7 when NEP lags the Nifio3.4 index for about 1-2 months.     

基于MODIS的春、夏季中国近海气溶胶对于云参数的影响差异研究

通过分析中国近海MODIS数据中气溶胶参数与云参数的相互关系,讨论了该区域气溶胶的间接效应及其对于云的可能影响.结果表明,在中国近海,气溶胶具有明显的间接效应,而且由于气溶胶种类和水汽的季节变化,使得气溶胶的间接作用具有很强的时间变化特征.在夏季,由于人为气溶胶占主导,它作为有效的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）有正相关、与云滴有效半径（CER）有负相关性、与云光学厚度（COT）也存在着正相关,气溶胶的间接效应明显;在春季,由于沙尘气溶胶盛行,同时沙尘并不是很好的云凝结核,使得气溶胶光学厚度（AOT）分别与云凝结核数（CCN）的正相关减弱、与云滴有效半径（CER）则由夏季的负相关变为正相关、与云光学厚度（COT）存在弱的负相关,气溶胶的间接效应不明显.     

时空投影模型(STPM)的次季节至季节(S2S)预测应用进展

随着数值天气预报技术和季节动力预报系统的发展,短期天气预报及长期气候预测的能力持续提高,然而介于两者之间的次季节至季节(S2S,两周至三个月)预测技巧偏低,成为当今气象学界和业务服务的难题。南京信息工程大学国家特聘专家李天明教授团队于2012年研发了基于时空投影技术的统计预报模型(STPM),成功地对中国大陆降水和气温距平,以及区域极端降水、夏季高温、冬季低温和西太平洋台风群发事件等高影响天气进行提前10~30 d的预报,并在国家气候中心及多个省份开展了业务应用。STPM也成功应用于台湾春雨预报、南海季风爆发和ENSO预测等季节至年际变化的预测。本文对S2S预测的理论基础、STPM的发展和应用进行了完整的介绍,并讨论了S2S预测业务中所面临的挑战和未来展望。     

海岸线熏烟扩散模式

该文导出一个无需作常涡扩散系数或“面源”假设的海岸线熏烟扩散模式。根据二维理论和观测资料对热力内边界层（TIBL）高度公式进行了简化。分析和预测结果表明:在海岸线附近,应尽可能将高污染源设置在远离海岸或靠近海岸线处,避免设置在有效源高度与当地TIBL高度相等的地点附近。     

基于概率加权估计的中国极端气温时空分布模拟试验

引入一种计算简便、有效性高,并可代替极大似然法的优良参数估计方法--概率加权法(PWM),利用Gumbel分布对中国极端气温时空变化特征作"当前"与"未来"气候的模拟试验.结果表明,这种方法具有较高的拟合优度.利用适应性较强的Weibull分布拟合中国逐日高(低)气温的原始分布,在此基础上,借助于蒙特卡洛随机模拟产生未来平均气候情景下的极端高(低)气温统计概率特征.模拟试验表明,在未来气候条件下,若平均气温升高1.0℃,中国各大区域极端高(低)气温的概率有一定的变动规律可寻.