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311.
The photochemical instability of several related pteridines in seawater was investigated by aseptic incubation of solutions at 20–22°C under illumination from cool-white light of intensity 6 kerg cm−2 sec−1, and the chemical changes were spectrophotometrically monitored. All the pteridines showed markedly accelerated degradation from this illumination relative to their behaviour in total darkness.Pterin and lumazine were degraded very slowly with zero-order reaction kinetics, while the other pteridines photolysed rapidly (according to first-order kinetics) with decomposition rates increasing in the order dioxylumazine (2,4,6,7-tetrahydroxypteridine) < leucopterin < isoxanthopterin < xanthopterin < oxylumazine (2,4,6-trihydroxypteridine). Excepting leucopterin and dioxylumazine, the photolysis rates were attributable to the pH of seawater and not its salt content; this was also the case with oxylumazine which required the salt content of seawater for decomposition in darkness. Leucopterin and dioxylumazine (both 6,7-dihydroxylated pteridines) gave evidence of complexation with the major divalent cations (Ca2+, Mg2+) of seawater, by virtue of which their photolytic degradation rates were enhanced to magnitudes obtained in pH-10 buffer without seawater. It is proposed that such complexation produces structural forms of these pteridines analogous to their normal ionic forms at pH 10–12.The photolysis of the 6-hydroxylated pteridines (xanthopterin, oxylumazine) proceeded via intermediate formation of their corresponding 7-hydroxylated derivatives (leucopterin, dioxylumazine). 相似文献
312.
D. Jeff Ross Craig R. Johnson Chad L. Hewitt 《Estuarine, Coastal and Shelf Science》2006,67(4):695-707
The northern Pacific seastar, Asterias amurensis, was first collected in southeast Tasmania in 1986. Mistaken for the endemic asteroid Uniophora granifera, its true identity was not realised until 1992. It is now a conspicuous predator in soft sediment habitats in this region, and is considered a major threat to native assemblages and commercial species. We examined the structure of soft sediment assemblages at different spatial scales in southeast Tasmania, and correlated spatial variation in community composition with seastar abundances. We found that the structure of soft sediment assemblages is highly variable at a range of spatial scales from metres to tens of kilometres. Clear differences in the composition of assemblages and abundances of major taxa were detected between areas with and without seastars and between areas with low and high seastar densities. However, the nature of these patterns suggests that they are more likely due to differences in sediment characteristics than due to impacts of the seastar. Thus, spatial differences in soft sediment assemblages might have been erroneously attributed to seastars without detailed information on important physical factors such as sediment characteristics. A second survey, using larger sampling units (1 m2) but across a more limited spatial extent, targeted bivalves and heart urchins that were identified as important prey of the seastar in observations of feeding and in experimental studies. Large-scale patterns of abundance and size structure were consistent with seastar effects anticipated from small-scale experimental and feeding studies for some, but not all, species. While the field survey ultimately provided evidence about the presence or absence of seastar impacts at large-scales, the identification of key ecological variables in experimental and feeding studies proved crucial to both the design and interpretation of patterns observed in the large-scale surveys. Overall, this work highlighted the necessity to consider multiple lines of evidence rather than relying on a single ‘inferential’ test, in the absence of pre-impact data. 相似文献
313.
中国台湾地区地处欧亚板块与菲律宾海板块之间,地震活动频繁.本文报道了 我国台湾地区及其邻近海域1985~2002年间5.5级以上地震的条带内外频度比分 布,并着重研究了1999—2002年中发生的3次7.5级以上地震前的条带现象.其结 果表明:台湾地区近期发生的3次7.5级以上大地震前,5.5级以上地震呈条带分 布.这些条带符合条带内地震个数Nin≥6的条件,符合条带内、外频度比Nin/(Nin Nout)≥75%的条件,也符合条带长宽比大于5的要求,只是与板内地震条带相比,条 带的长度较短. 相似文献
314.
315.
李刚 《海洋地质与第四纪地质》2003,23(1):125-129
归一化层速度是对任意深度处的层速度进行归一化处理的一种速度形式,归一化处理的目的是把任意深度处的层速度转换为与深度无关的格式,归一化后层速度的横向变化主要取决于地层岩性,孔隙度等物性的变化,利用这一特点可以方便地利用已知钻井资料对其进行标定,比较简单地进行地层岩性,孔隙度等特性的预测。实际应用表明,其预测结果与钻井揭示吻合较好,预测效果令人满意。 相似文献
316.
夏、冬两季长江口及邻近海域悬浮物的分布特征及其沉积量 总被引:11,自引:0,他引:11
利用2001年7~8月 ,2002年1月两个航次的悬浮物浓度资料 ,并参考其它水文参数 ,简要分析长江口及邻近海域悬浮物的分布特征 :无论夏季还是冬季 ,长江入海悬浮物总是向东南方输运 ;冬季由于再悬浮作用显著 ,悬浮物浓度明显高于夏季 ,且南北分布范围也明显增大 ,垂向分布均匀。同时采用数值模拟的海流流速值和观测的悬浮物浓度值计算悬浮物的断面通量 ,并最终得计算区悬浮物夏、冬两季的沉积量 ,夏、冬季长江口及邻近海域悬浮物的沉积量分别为0.79×108t,1.44×108t。 相似文献
317.
Observations of wintertime nutrient concentrations in surface waters are scarce in the temperate and subarctic North Atlantic Ocean. Three new methods of their estimation from spring or early summer observations are described and evaluated. The methods make use of a priori knowledge of the vertical distribution of oxygen saturation and empirical relationships between nutrient concentrations and oxygen saturation. A south–north increase in surface water winter nutrient concentration is observed. Winter nitrate concentrations range from very low levels of about 0.5 μmol dm−3 at 33°N to about 13.5 μmol dm−3 at 60°N. Previous estimates of winter nitrate concentrations have been overestimates by up to 50%. At the Biotrans Site (47°N, 20°W), a typical station in the temperate Northeast Atlantic, a mean winter nitrate concentration of 8 μmol dm−3 is estimated, compared to recently published values between 11 and 12.5 μmol dm−3. It is shown that most of the difference is due to a contribution of remineralised nitrate that had not been recognized in previous winter nutrient estimates. Mesoscale variation of wintertime nitrate concentrations at Biotrans are moderate (less than ±15% of the regional mean value of about 8 μmol dm−3). Interannual variation of the regional mean is small, too. In the available dataset, there was only 1 year with a significantly lower regional mean winter nitrate concentration (7 μmol dm−3), presumably due to restricted deep mixing during an atypically warm winter. The significance of winter nitrate estimates for the assessment of spring-bloom new production and the interpretation of bloom dynamics is evaluated. Applying estimates of wintertime nitrate concentrations of this study, it is found that pre-bloom new production (0.275 mol N m−2) at Biotrans almost equals spring-bloom new production (0.3 mol N m−2). Using previous estimates of wintertime nitrate yields unrealistically high estimates of pre-bloom new production (1.21–1.79 mol N m−2) which are inconsistent with observed levels of primary production and the seasonal development of biomass. 相似文献
318.
319.
The ridge located between 31° S and 34°30′S is spreading at a rate of 35 mm yr−1, a transitional velocity between the very slow (≤20 mm yr−1) opening rates of the North Atlantic and Southwest Indian Oceans, and the intermediate rates (60 mm yr−1) of the northern limb of the East Pacific Rise, and the Galapagos and Juan de Fuca Ridges. A synthesis of multi-narrow beam,
magnetics and gravity data document that in this area the ridge represents a dynamically evolving system. Here the ridge is
partitioned into an ensemble of six distinct segments of variable lengths (12 to 100 km) by two transform faults (first-order
discontinuities) and three small offset (< 30 km) discontinuities (second-order discontinuities) that behave non-rigidly creating
complex and heterogeneous morphotectonic patterns that are not parallel to flow lines. The offset magnitudes of both the first
and second-order discontinuities change in response to differential asymmetric spreading. In addition, along the fossil trace
of second-order discontinuities, the lengths of abyssal hills located to either side of a discordant zone are observed to
lengthen and shorten creating a saw-toothed pattern. Although the spreading rate remains the same along the length of the
ridge studied, the morphology of the spreading segments varies from a deep median valley with characteristics analogous to
the rift segments of the North Atlantic to a gently rifted axial bulge that is indistinguishable from the shape and relief
of the intermediate rate spreading centers of the East Pacific Rise (i.e., 21°N). Like other carefully surveyed ridge segments
at slow and fast rates of accretion, the along-axis profiles of each ridge segment are distinctly convex upwards, and exhibit
along-strike changes in relief of 500m to 1500 between the shallowest portion of the segment (approximate center) and the
segment ends. Such spatial variations create marked along-axis changes in the morphology and relief of each segment. A relatively
low mantle Bouguer anomaly is known to be associated with the ridge segment characterized by a gently rifted axial bulge and
is interpreted to indicate the presence of focused mantle upwelling (Kuo and Forsyth, 1988). Moreover, the terrain at the
ends of each segment are known to be highly magnetized compared to the centers of each segment (Carbotte et al, 1990). Taken
together, these data clearly establish that these profound spatial variations in ridge segment properties between adjoining
segments, and along and across each segment, indicate that the upper mantle processes responsible for the formation of this
contrasting architecture are not solely related to passive upwelling of the asthenosphere beneath the ridge axis. Rather,
there must be differences in the thermal and mechanical structure of the crust and upper mantle between and along the ridge
segments to explain these spatial variations in axial topography, crustal structure and magnetization. These results are consistent
with the results of investigations from other parts of the ridge and suggest that the emplacement of magma is highly focused
along segments and positioned beneath the depth minimum of a given segment. The profound differences between segments indicate
that the processes governing the behavior of upwelling mantle are decoupled and the variations in the patterns of axis flanking
morphology and rate of accretion indicate that processes controlling upwelling and melt production vary markedly in time as
well. At this spreading rate and in this area, the accretionary processes are clearly three-dimensional. In addition, the
morphology of a ridge segment is not governed so much by opening rate as by the thermal structure of the mantle which underlies
the segment. 相似文献
320.