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21.
This study investigated the potential for the uranium mineral carnotite (K2(UO2)2(VO4)2·3H2O) to precipitate from evaporating groundwater in the Texas Panhandle region of the United States. The evolution of groundwater chemistry during evaporation was modeled with the USGS geochemical code PHREEQC using water-quality data from 100 groundwater wells downloaded from the USGS National Water Information System (NWIS) database. While most modeled groundwater compositions precipitated calcite upon evaporation, not all groundwater became saturated with respect to carnotite with the system open to CO2. Thus, the formation of calcite is not a necessary condition for carnotite to form. Rather, the determining factor in achieving carnotite saturation was the evolution of groundwater chemistry during evaporation following calcite precipitation. Modeling in this study showed that if the initial major-ion groundwater composition was dominated by calcium-magnesium-sulfate (>70 precent Ca + Mg and >50 percent SO4 + Cl) or calcium-magnesium-bicarbonate (>70 percent Ca + Mg and <70 percent HCO3 + CO3) and following the precipitation of calcite, the concentration of calcium was greater than the carbonate alkalinity (2mCa+2 > mHCO3− + 2mCO3−2) carnotite saturation was achieved. If, however, the initial major-ion groundwater composition is sodium-bicarbonate (varying amounts of Na, 40–100 percent Na), calcium-sodium-sulfate, or calcium-magnesium-bicarbonate composition (>70 percent HCO3 + CO3) and following the precipitation of calcite, the concentration of calcium was less than the carbonate alkalinity (2mCa+2 < mHCO3- + 2mCO3−2) carnotite saturation was not achieved. In systems open to CO2, carnotite saturation occurred in most samples in evaporation amounts ranging from 95 percent to 99 percent with the partial pressure of CO2 ranging from 10−3.5 to 10−2.5 atm. Carnotite saturation occurred in a few samples in evaporation amounts ranging from 98 percent to 99 percent with the partial pressure of CO2 equal to 10−2.0 atm. Carnotite saturation did not occur in any groundwater with the system closed to CO2. 相似文献
22.
Review of Earth Critical Zone Research 总被引:2,自引:0,他引:2
Since the Earth Critical Zone put forward by National Research Council of America in 2001, it has got a lot of attention and some significant progresses have been made. This paper summarized those Earth Critical Zone projects and related research plans organized and implemented by the United States of America, Germany, Australia, France, China and the European Union, as well as main scientific problems and future development direction in the study of Earth Critical Zone. According to research status of China, the four main research contents should be strengthened including structure, formation and evolution mechanism of Earth Critical Zone, the coulpling interaction mechanism between migration and transformation of material and multi-processes, sevice function and evolution features of Earth Critical Zone and its support and effect on sustainable development, model simulation of process and system of Earth Critical Zone. In addition, our country should actively conduct cooperation and communication with the advanced countries, and enhance our involvement in international key research plans. 相似文献
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山东省曹县地区土壤地球化学调查是按浅层土壤样品1点/4 km~2,深层土壤样品1点/16 km~2。测试N,P,K,Cu,Zn,B,Mo,Mn,F,As,Hg,Pb,Cr,Cd等14种指标。在统计这些指标的表层、深层土壤地球化学特征参数的基础上,对其与世界、全省同类参数的差异进行了分析,并分析了区内表层、深层土壤元素含量的相关性,认为该区表层土壤元素含量的显著特征是高F而低P,Zn,Mo。大部分元素在表层土壤中的含量继承了土壤母质的成分特征,但N,P,F,Hg等受人为活动和污染源的作用在表层土壤中明显富集。 相似文献
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金岭杂岩体由细粒黑云角闪闪长岩、中细粒黑云角闪闪长岩、中细粒黑云角闪二长闪长岩和细粒角闪二长闪长岩组成,是鲁西地区典型矽卡岩型富铁矿(金岭铁矿)控矿岩体。本次研究对细粒黑云角闪闪长岩和细粒角闪二长闪长岩进行了锆石LA‐ICP‐MS U‐Pb定年,其结果分别为129.2±3.2 Ma和132.8±1.2 Ma,表明该杂岩体的侵位时代为早白垩世。样品SiO2、K2O和Na2O含量分别介于54.17%~63.73%、1.92%~4.76%和3.10%~5.41%之间,K2O/Na2O为0.58~0.94,A/CNK为0.60~0.93,具有轻稀土富集,重稀土亏损的右倾型稀土配分模式,轻、重稀土分馏程度中等((La/Yb)N=9.94~23.49),Eu异常不明显(δEu=0.84~1.10),具中—弱负Ce异常(δCe=0.56~0.92)。样品以富集大离子亲石元素(Ba、K、U、Pb等)、亏损高场强元素(Nb、Ta、Ti)以及高Sr/Y为特征。金岭杂岩体为燕山晚期岩浆活动产物,属准铝质高钾钙碱性系列,岩浆主要来源于富集岩石圈地幔的部分熔融,并在岩浆上升侵位的过程中有地壳物质的同化混染。燕山晚期华北克拉通在古太平洋板块俯冲后后撤引起的板内伸展环境下,增厚陆壳减薄阶段,岩浆上侵就位形成金岭杂岩体。 相似文献
26.
Hydro-geochemistry of groundwater and surface water in Dschang town(West Cameroon): Alkali and alkaline-earth elements ascertain lithological and anthropogenic constraints
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Yemeli Elida Joelle Temgoua Emile Kengni Lucas Ambrosi Jean-Paul Momo-nouazi Mathieu Silatsa-Tedou Francis Brice Wamba Franck Robean Tchakam-Kamtchueng Brice 《地下水科学与工程》2021,9(3):212-224
This study focuses on the sources of alkali and alkaline-earth elements based on the geochemistry of groundwater and surface water in Dschang concerning environmental and anthropogenic constraints. A comprehensive set of 50 samples from groundwater and surface water were analyzed by ICPMS and processed by spatial interpolation in a GIS environment. The results highlight a geochemical anomaly at the center of the densely inhabited area subject to a profusion of open dumps discharges. This anomaly with the highest spatial contents of Be(Cs, Rb, Mg) suggests an anthropogenic source that demarcates with the lowest alkali and alkaline-earth elements on the peripheral area of Dschang. Other findings include lithological constraints with volcanic rocks being the main source compared to granitoid.The study points out good correlations between Be, Cs, Rb and Mg spatial distributions and physicochemical parameters of waters(K, EC, TDS), and inversely with the lowest p H. p H is established as the most functioning physico-chemical constraint of alkali and alkaline-earth mobility in Dschang. The p H lowest values within the geochemical anomaly also highlight the impact of human activities on water acidity, which later enhance elements mobility and enrichment. Despite low elements contents relative to WHO standards, our findings point out an example of anthropogenic impact on water geochemistry linked to solid waste pollution; it also demonstrates significant anthropogenic changes of environmental physicochemical parameters of prime importance in the mobility and distribution of elements in the study area.Similar assessments should be extended in major towns in Cameroon. 相似文献
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以二氧化氯作为一种新型的消毒剂和杀菌剂 ,以传统含氯制剂 (如漂白粉、二氯异氰尿酸钠、三氯异氰尿酸 )作为对照 ,比较其在治疗欧洲鳗细菌性疾病及改善养殖水质方面的显著特性 ,其作用活性与环境 (如 p H、温度、氨及有机物 )因子的关系。结果表明 ,二氧化氯 (Cl O2 )对爱德华氏菌、嗜水气单胞菌和柱状屈挠杆菌有很好的杀灭效果 ,能迅速治愈欧洲鳗的赤鳍病和肝肾病 ,且能有效改善养殖水体 ,水中生化需氧量比对照组下降 10 %~ 30 % ,化学耗氧量下降 5% ,溶氧量提高 8%~ 10 %。当二氧化氯体积分数为 8m L/m3时 ,其杀菌率均高达 90 %以上 ,为氯制剂的 1.8倍 ,且活性不受环境因子的影响 相似文献
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黄淮海地区乡村人—地—业协调发展格局与机制 总被引:8,自引:0,他引:8
乡村在社会中占有重要地位,但乡村衰败目前已成为世界性问题,因此,乡村振兴需破解乡村病问题。现有乡村研究主要关注乡村单一系统、乡村转型或乡村特定问题的研究,对乡村系统自身、乡村各子系统之间关系及其驱动乡村发展逻辑的研究则显匮乏。基于黄淮海地区县域数据,选取乡村人—地—业3个子系统,利用耦合协调度模型刻画了乡村内部系统耦合协调度的空间格局,并对人—地—业驱动乡村发展的内在逻辑进行了探讨。结果发现:① 黄淮海地区大部分县域乡村人—地—业发展处于高水平耦合阶段,在空间格局上形成了4条明显的高值轴带,且乡村系统发展水平呈逐年上升趋势。② 黄淮海地区乡村耦合协调水平整体较高,但大部分处于勉强协调或初级协调阶段,耦合协调水平较高的县域主要集中在经济较发达地区。③ 黄淮海地区乡村耦合协同关系可分为低协调水平—土地发展领先型、中协调水平—人口发展领先型和高协调水平—人业发展引领型3种类型,其中产业在黄淮海地区乡村协调发展中至关重要。④ 乡村人—地—业的协调发展可有效激活“四力”,为乡村可持续发展奠定了基础。本研究为理解乡村系统自身、破解乡村问题及实现乡村可持续发展提供了参考。 相似文献
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