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991.
Samples from extremely acidic waters should be taken using the introduced syringe technique avoiding atmospheric contact to minimize CO2 evaporation from the samples. The syringe technique inclusive manual injection enables the determination of TIC in acid waters with high precision and accuracy. If a TOC analyser with a small sample volume is used, the vials should be filled directly inside the water sampler without air bubbles, covered with aluminium foil and transported at ambient water temperatures. If an autosampler is used, partial selection of the vials increases the stability of the results. Care should be taken that samples can be analysed within a short time. 相似文献
992.
Sunil Varma Jim Underschultz Tess Dance Robert Langford Joan Esterle Kevin Dodds Dominique van Gent 《Marine and Petroleum Geology》2009
Coal-fired power stations in Collie, Western Australia emit 10 million tonnes of CO2 per year. This study assesses the potential opportunities of geological storage of CO2 both within the Collie Basin and the onshore part of the adjacent Southern Perth Basin of Western Australia within 50 km of Collie town site through a desktop evaluation of existing data. The aquifers and coal formations within both basins have been evaluated for their suitability for storage based on geological, geographical and environmental criteria related to storage capacity, injectivity, proximity to sources of CO2, location of other natural resources and containment security. The study has concluded that there is limited scope for large-scale storage of CO2 within the Collie Basin. In addition the potential for storage within coals of either basin is not a viable solution. This assessment is based on published criteria for CO2 storage in sedimentary basins and coal-bearing formations. 相似文献
993.
Black carbon in marine particulate organic carbon: Inputs and cycling of highly recalcitrant organic carbon in the Gulf of Maine 总被引:2,自引:0,他引:2
D. Xanat Flores-Cervantes Desiree L. Plata John K. MacFarlane Christopher M. Reddy Philip M. Gschwend 《Marine Chemistry》2009,113(3-4):172-181
To increase our understanding of the roles of black carbon (BC), a highly sorptive and recalcitrant material, we measured BC concentrations and fluxes in marine particulate organic carbon (POC) out of the water column in the Gulf of Maine (GoM), a representative coastal area downwind of important BC sources of the Northeastern United States. Concentrations ranged from < 0.1 to 16 μg/L in the spring and late summer, typically contributing between 1 and 20% of the POC. Water-column export fluxes were near 10 gBC/m2∙yr. These observations suggest that (a) up to 50% of the “molecularly uncharacterized” POC in this region's seawater is combustion-derived BC, and (b) the “bioavailabilities” of hydrophobic pollutants like polycyclic aromatic hydrocarbons (PAHs) would be influenced substantially by sorption to BC. The observed BC spatial distributions imply that a large part of the BC was carried offshore by wind and that much of it is accumulated in the coastal sediments. On a global scale, these results suggest the GoM and other coastal areas with similar BC loadings accumulate significant amounts of highly recalcitrant organic carbon that remineralizes on geological time scales in the world's oceans. 相似文献
994.
Franck Touratier Catherine Goyet 《Deep Sea Research Part I: Oceanographic Research Papers》2009,56(10):1708-1716
Monthly observations accumulated over more than a decade at the DYFAMED time-series station allow us to estimate the temporal evolution of anthropogenic CO2 in the western Mediterranean Sea. This objective is reached by using recognized interpolation procedures to reconstruct the incomplete distributions of measured total dissolved inorganic carbon and total alkalinity. These reconstructed fields, associated with those available for dissolved oxygen and temperature, are used to estimate the distribution of anthropogenic CO2. This is done with the recently developed Tracer combining Oxygen, inorganic Carbon, and total alkalinity (TrOCA) approach. The main results indicate that (1) the concentrations of anthropogenic CO2 are much higher than those found in the Atlantic Ocean (the minimum concentration at the DYFAMED site is 50 μmol kg−1), and (2) the temporal trend for anthropogenic CO2 is decreasing, especially in the intermediate and the deep layers of the water column at the DYFAMED site. This decrease in anthropogenic CO2 is significantly correlated with a decrease in the dissolved oxygen and with an increase in both salinity and temperature. These trends are discussed in the light of recent published works that propose explanations for the observed increases in salinity and temperature that occurred in the western basin since the 1950s. We conclude that the decrease in anthropogenic CO2 probably resulted from an invasion of old water masses. Different hypotheses on the origin of these water masses are considered and several arguments indicate that the eastern Mediterranean transient (EMT) could have played an important role in the observed decrease in anthropogenic CO2 concentrations at the DYFAMED site. 相似文献
995.
Karine Granger Alain Mnesguen Sbastien Lefebvre Cdric Bacher Stphane Pouvreau 《Journal of Sea Research》2009,62(2-3):147
It is well known that temporal changes in bivalve body mass are strongly correlated with temporal variations in water temperature and food supply. In order to study the influence of the year-to-year variability of environmental factors on oyster growth, we coupled a biogeochemical sub-model, which simulates trophic resources of oysters (i.e. phytoplankton biomass via chlorophyll a), and an ecophysiological sub-model, which simulates growth and reproduction (i.e. gametogenesis and spawning), using mechanistic bases. The biogeochemical sub-model successfully simulated phytoplankton dynamics using river nutrient inputs and meteorological factors as forcing functions. Adequate simulation of oyster growth dynamics requires a relevant food quantifier compatible with outputs of the biogeochemical sub-model (i.e. chlorophyll a concentration). We decided to use the phytoplankton carbon concentration as quantifier for food, as it is a better estimator of the energy really available to oysters. The transformation of chlorophyll a concentration into carbon concentration using a variable chlorophyll a to carbon ratio enabled us to improve the simulation of oyster growth especially during the starvation period (i.e. autumn and winter). Once validated, the coupled model was a suitable tool to study the influence of the year-to-year variability of phytoplankton dynamics and water temperature on the gonado-somatic growth of the Pacific oyster. Four years with highly contrasted meteorological conditions (river inputs, water temperature and light) 2000, 2001, 2002 and 2003, were simulated. The years were split into two groups, wet years (2000 and 2001) and dry years (2002 and 2003). Significant variability of the response of oysters to environmental conditions was highlighted between the four scenarios. In the wet years, an increase in loadings of river nutrients and suspended particulate matter led to a shift in the initiation and the magnitude of the phytoplanktonic spring bloom, and consequently to a shift in oyster growth patterns. In contrast, in the dry years, an increase in water temperature—especially during summer—resulted in early spawning. Thus, the gonado-somatic growth pattern of oysters was shown to be sensitive to variations in river loadings and water temperature. In this context, the physiological status of oysters is discussed using a relevant indicator of energy needs. 相似文献
996.
Dissolved organic carbon (DOC) distributions along two Atlantic Meridional Transects conducted in 2005 in the region between 47°N and 34°S showed clear latitudinal patterns. The DOC concentrations in the epipelagic zone (0–100 m) were the highest (70–90 µM) in tropical and subtropical waters with stable mixed layers, and lowest (50–55 µM) at the poleward extremities of the transects due to deep convective mixing supplying low DOC waters to the surface. A decrease in DOC occurred with depth, and lowest DOC concentrations (41–45 µM) in the 100–300 m depth range were observed in the equatorial region due to upwelling of low DOC waters. A strong relationship between DOC and AOU was observed in the σ–t 26–26.5 isopycnal layer which underlies the euphotic zone and outcrops at the poleward extremities of the North and South Atlantic Subtropical Gyres (NASG and SASG) in the region ventilating the thermocline waters. Our observations reveal significant north–south variability in the DOC–AOU relationship. The gradient of the relationship suggests that 52% of the AOU in the σ–t 26–26.5 density range was driven by DOC degradation in the NASG and 36% in the SASG, with the remainder due to the remineralisation of sinking particulate material. We assess possible causes for the greater contribution of DOC remineralisation in the NASG compared to the SASG. 相似文献
997.
Dissolution of CO2 into deep subsurface brines for carbon sequestration is regarded as one of the few viable means of reducing the amount of CO2 entering the atmosphere. Ions in solution partially control the amount of CO2 that dissolves, but the mechanisms of the ion's influence are not clearly understood and thus CO2 solubility is difficult to predict. In this study, CO2 solubility was experimentally determined in water, NaCl, CaCl2, Na2SO4, and NaHCO3 solutions and a mixed brine similar to the Bravo Dome natural CO2 reservoir; ionic strengths ranged up to 3.4 molal, temperatures to 140 °C, and CO2 pressures to 35.5 MPa. Increasing ionic strength decreased CO2 solubility for all solutions when the salt type remained unchanged, but ionic strength was a poor predictor of CO2 solubility in solutions with different salts. A new equation was developed to use ion hydration number to calculate the concentration of electrostricted water molecules in solution. Dissolved CO2 was strongly correlated (R2 = 0.96) to electrostricted water concentration. Strong correlations were also identified between CO2 solubility and hydration enthalpy and hydration entropy. These linear correlation equations predicted CO2 solubility within 1% of the Bravo Dome brine and within 10% of two mixed brines from literature (a 10 wt % NaCl + KCl + CaCl2 brine and a natural Na+, Ca2+, Cl− type brine with minor amounts of Mg2+, K+, Sr2+ and Br−). 相似文献
998.
《China Geology》2022,5(3):359-371
To accelerate the achievement of China’s carbon neutrality goal and to study the factors affecting the geologic CO2 storage in the Ordos Basin, China’s National Key R&D Programs propose to select the Chang 6 oil reservoir of the Yanchang Formation in the Ordos Basin as the target reservoir to conduct the geologic carbon capture and storage (CCS) of 100000 t per year. By applying the basic theories of disciplines such as seepage mechanics, multiphase fluid mechanics, and computational fluid mechanics and quantifying the amounts of CO2 captured in gas and dissolved forms, this study investigated the effects of seven factors that influence the CO2 storage capacity of reservoirs, namely reservoir porosity, horizontal permeability, temperature, formation stress, the ratio of vertical to horizontal permeability, capillary pressure, and residual gas saturation. The results show that the sensitivity of the factors affecting the gas capture capacity of CO2 decreases in the order of formation stress, temperature, residual gas saturation, horizontal permeability, and porosity. Meanwhile, the sensitivity of the factors affecting the dissolution capture capacity of CO2 decreases in the order of formation stress, residual gas saturation, temperature, horizontal permeability, and porosity. The sensitivity of the influencing factors can serve as the basis for carrying out a reasonable assessment of sites for future CO2 storage areas and for optimizing the design of existing CO2 storage areas. The sensitivity analysis of the influencing factors will provide basic data and technical support for implementing geologic CO2 storage and will assist in improving geologic CO2 storage technologies to achieve China’s carbon neutralization goal.©2022 China Geology Editorial Office. 相似文献
999.
Clayton Munnings William Acworth Oliver Sartor Yong-Gun Kim Karsten Neuhoff 《Climate Policy》2019,19(1):92-107
Nearly every carbon price regulates the production of carbon emissions, typically at midstream points of compliance such as power plants, consistent with typical advice from the literature. Since the early 2010s however, policymakers in Australia, California, China, Japan and Korea have implemented carbon prices that regulate the consumption of carbon emissions, where points of compliance are further downstream, such as distributors or final consumers. This article identifies the pivot towards placing the point of compliance for carbon prices further downstream as an emerging international trend, describes the designs of different prices on carbon consumption around the world, and explains the various motivations of the policymakers implementing them. Findings reveal that policymakers tend to layer prices on carbon consumption on top of prices on carbon production in an effort to improve economic outcomes by addressing incomplete pass-through of the carbon price from producer to consumer, thereby facilitating more cost-effective abatement. Policymakers also use prices on carbon consumption to reduce emissions leakage or because large producers of carbon are not within their jurisdiction. The prevalence of prices on carbon consumption will likely increase as evidenced by proposals in China and Europe.
Key policy insights
The recent surge in the number of jurisdictions implementing prices on carbon consumption represents an emerging international trend.
Policymakers use prices on carbon consumption in an effort to improve economic outcomes and capture environmental benefits.
While this article offers insights that detail initial challenges and successes, whether these prices on carbon consumption actually achieve their intended goals is an academically rich topic that requires further research on individual policies.
1000.
Deforestation, the second largest source of anthropogenic greenhouse gas emissions, is largely driven by expanding forestry and agriculture. However, despite agricultural expansion being increasingly driven by foreign demand, the links between deforestation and foreign demand for agricultural commodities have only been partially mapped. Here we present a pan-tropical quantification of carbon emissions from deforestation associated with the expansion of agriculture and forest plantations, and trace embodied emissions through global supply chains to consumers. We find that in the period 2010–2014, expansion of agriculture and tree plantations into forests across the tropics was associated with net emissions of approximately 2.6 gigatonnes carbon dioxide per year. Cattle and oilseed products account for over half of these emissions. Europe and China are major importers, and for many developed countries, deforestation emissions embodied in imports rival or exceed emissions from domestic agriculture. Depending on the trade model used, 29–39% of deforestation-related emissions were driven by international trade. This is substantially higher than the share of fossil carbon emissions embodied in trade, indicating that efforts to reduce greenhouse gas emissions from land-use change need to consider the role of international demand in driving deforestation. Additionally, we find that deforestation emissions are similar to, or larger than, other emissions in the carbon footprint of key forest-risk commodities. Similarly, deforestation emissions constitute a substantial share (˜15%) of the total carbon footprint of food consumption in EU countries. This highlights the need for consumption-based accounts to include emissions from deforestation, and for the implementation of policy measures that cross these international supply-chains if deforestation emissions are to be effectively reduced. 相似文献