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Paolo Laj Andrea I. Flossmann Wolfram Wobrock Sandro Fuzzi Giordano Orsi Loretta Ricci Stephan Mertes Alfons Schwarzenbck Jost Heintzenberg Harry Ten Brink 《Atmospheric Research》2001,58(4):256
We investigated the partitioning of trace substances during the phase transition from supercooled to mixed-phase cloud induced by artificial seeding. Simultaneous determination of the concentrations of H2O2, NH3 and black carbon (BC) in both condensed and interstitial phases with high time resolution showed that the three species undergo different behaviour in the presence of a mixture of ice crystals and supercooled droplets. Both H2O2 and NH3 are efficiently scavenged by growing ice crystals, whereas BC stayed predominantly in the interstitial phase. In addition, the scavenging of H2O2 is driven by co-condensation with water vapour onto ice crystals while NH3 uptake into the ice phase is more efficient than co-condensation alone. The high solubility of NH4+ in the ice could explain this result. Finally, it appears that the H2O2–SO2 reaction is very slow in the ice phase with respect to the liquid phase. Our results are directly applicable for clouds undergoing limited riming. 相似文献
44.
利用非金属矿制备白炭黑现状及发展前景 总被引:8,自引:0,他引:8
简术了白炭黑的用途和制备方法,综述了利用非金属矿制备白炭黑的方法和技术现状,对充分利用非金属矿制备白炭黑提供思路并展望其发展前景。 相似文献
45.
1993年5月4~6日在我国西北部地区发生了一次“黑风暴”。用改进的MM1和高分辨PBL参数化及40 km细网格控制试验能基本上模拟出“93.5”黑风暴的结构和演变。模拟结果表明,黑风暴发展时段,在PBL内与一个中尺度气旋性强涡旋相伴,在对流层内与一个垂直涡柱相伴。这个伸展至对流层顶的涡柱下(上)半部是与低(高)空强烈辐合(辐散)入(外)流相伴的气旋(反气旋)性涡柱。该黑风暴结构不同于一般锋面结构,其主要判别是:界面坡度陡,θe水平梯度大,斜压性强,PBL内暖心明显。该暖心结构与下垫面剧烈热力强迫有关。不 相似文献
46.
Sunil Bharati Richard L. Patience Steve R. Larter Guy Standen Iain J. F. Poplett 《Organic Geochemistry》1995,23(11-12)
The significance and validity of integrating data obtained from a variety of analytical techniques to understand, elucidate and model kerogen's complex chemical structure is reported here using degradative (open and closed system pyrolysis, chemical oxidation), non-degradative (13C CP/MAS NMR) and optical (incident white light and blue light) methods. Seven Cambrian Alum Shale samples, ranging in maturity from immature to post-mature with respect to petroleum generation, were studied and were chosen for their simple geological history, uniform organic matter type and high organic carbon content. The Alum Shale kerogens, which primarily consist of algal organic matter, liberate low molecular weight gaseous and aromatic compounds on pyrolysis and give mostly branched dicarboxylic acids on chemical oxidation. 13C NMR spectroscopy shows that the Alum Shale kerogens are anomalously rich in oxygen-bearing functional groups (such as C = O, ArCO, CHO, CHxO), most of which apparently remain intact within the kerogen macro-molecule (KMM) through the diagenetic and catagenetic stages. Fragments released by different degradative techniques are quantified and the aromaticity (fa), O/C and relative proportions of various carbon types estimated by 13C NMR. A synthesis of these data has allowed us to better understand the chemistry of the Alum Shale kerogen. 相似文献
47.
The broad X-ray iron line observed in many active galactic nuclei spectra is thought to originate from the accretion disc surrounding the putative supermassive black hole. We show here how to perform the analytical integration of the geodesic equations that describe the photon trajectories in the general case of a rotating black hole (Kerr metric), in order to write a fast and efficient numerical code for modelling emission line profiles from accretion discs. 相似文献
48.
研究了盐度对黄鳍鲷SparuslatusHouttuyn、平鲷Rhabdosargussarba(Forskal)、黑鲷Sparusmacrocephalus(Basilewsky)和真鲷Pagrsomusmajor(TemmincketSchlegel)4种鲷鱼精子活力的影响。对南海区4种鲷鱼精子的适盐性及其活力进行了比较,黄鳍鲷、平鲷、黑鲷和真鲷精子激活所需的最低盐度分别为8、10、>8、>10;激活的最适盐度则分别为21、22、25、25,与之相应的精子活动(涡动)时间分别为14.7、17.7、17.2、18.0min;在高盐条件(盐度40左右)下,黄鳍鲷精子的适应性最强,精子活力最好,其次是黑鲷、真鲷的精子,平鲷精子对高盐条件的适应性最差。 相似文献
49.
中奥陶世克拉道克阶(Caradocian)在全球范围内为海侵期,体现在全球范围广泛的黑色页岩沉积及笔石动物的大规模繁盛,湘黔地区这一时期地层发育完全,从碳酸盐台地-斜坡-外陆架盆地均有不同程度的响应。在台地区表现为碳酸盐台地的淹没,斜坡区表现为碳酸盐重力流及黑色页岩、粉砂岩沉积,形成碳酸盐与陆源碎屑的混合沉积,而在外陆架盆地区表现为黑色岩系大规模发育及笔石的大量繁盛。 相似文献
50.
Group velocities of Rayleigh and Love waves along the paths across the Black Sea and partly Asia Minor and the Balkan Peninsula are used to estimate lateral variations of the crustal structure in the region. As a first step, lateral variations of group velocities for periods in the range 10–20 s are determined using a 2D tomography method. Since the paths are oriented predominantly in NE–SW or N–S direction, the resolution is estimated as a function of azimuth. The local dispersion curves are actually averaged over the extended areas stretched in the predominant direction of the paths. The size of the averaging area in the direction of the best resolution is approximately 200 km. As a second step, the local averaged dispersion curves are inverted to vertical sections of S-wave velocities. Since the dispersion curves in the 10–20 s period range are mostly affected by the upper crustal structure, the velocities are estimated to a depth of approximately 25 km. Velocity sections along 43° N latitude are determined separately from Rayleigh and Love wave data. It is shown that the crust under the sea contains a low-velocity sedimentary layer of 2–3 km thickness, localized in the eastern and western deeps, as found earlier from DSS data. Beneath the sedimentary layer, two layers are present with velocity values lying between those of granite and consolidated sediments. Velocities in these layers are slightly lower in the deeps, and the boundaries of the layers are lowered. S-wave velocities obtained from Love wave data are found to be larger than those from Rayleigh wave data, the difference being most pronounced in the basaltic layer. If this difference is attributed to anisotropy, the anisotropy coefficient = (SH - SV)/Smean is reasonable (2–3%) in the upper layers, and exceeds 9% in the basaltic layer. 相似文献