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Brian Gulson Karen Mizon Michael Korsch Honway Louie Michael Wu Jenny Stauber J. Michael Davis Alan Taylor 《中国地球化学学报》2006,25(B08):62-62
This is a 4-year longitudinal study to evaluate changes to the environment and exposure of young children associated with the introduction of methylcyclopentadienyl manganese tricarbonyl (MMT) into Australia in 2000. The cohort includes 57 females and 56 males; age range of 0.29 to 3.9 years. Samples are collected every 6 months from children in residences located at varying distances from major traffic thoroughfares in Sydney. Environmental samples: air, house and day care dustfall, soil, dust sweepings and gasoline. Samples from children: blood, urine, handwipes prior to and after playing outdoors, and a 6-day duplicate diet. All samples are analyzed for a suite of 20 elements using ICP-MS. Results are presented for the first three 6-month sampling periods for Pb and Mn. For dustfall accumulation, there was no significant change over the 3 sampling periods (time) for Pb or Mn, and a positive relationship between ‘traffic exposure' (traffic volume and proximity to the road) and Pb but not Mn. For handwipes, Pb and Mn in wipes taken from children after playing outdoors were usually significantly greater than for wipes taken prior to playing. There was no significant association between Pb or Mn in handwipes with traffic exposure. Dustfall accumulation was a significant predictor for Pb in the handwipes, and dust sweepings were a significant predictor of Mn in handwipes. 相似文献
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Yoko Fujikawa Daisuke Yoneda Atushi Minami Hiroshi Yashima Toshio Tonokai Sotoji Tani Masami Fukui Tatuhide Hamasaki Masataka Sugahara 《中国地球化学学报》2006,25(B08):113-113
Biological iron and manganese removal utilizing indigenous iron and manganese oxidizing bacteria (IRB hereafter) in groundwater can also be applied to arsenic removal according to our pilot-scale test. The arsenic removal probably occurred through sorption and complexation of arsenic to iron and manganese oxides formed by enzymic action of IRB. We investigated the chemical properties of iron and manganese oxides in IRB floc and the valence state of arsenic sorbed to the floc to clarify the mechanisms of the arsenic [especially As (Ⅲ)] removal. The floc samples were collected from two drinking water plants using IRB (Jyoyo and Yamatokoriyama, Japan), and our pilot - scale test site where arsenic and iron removal using IRB is under way (Mukoh, Japan). The Jyoyo and Yamatokoriyama IRB floc samples were subjected to As (Ⅲ) and As(Ⅴ) sorption experiments. The elemental composition of the floc samples was measured. XANES spectra were collected on As, Fe and Mn K-edges at synchrotron radiation facility Spring 8 (Hyogo, Japan). FT-IR and the X-ray diffraction spectra of the samples were also obtained. The IRB floc contained ca. 35 % Fe, 0.3%-3.5% Mn and 2%-6% P. The samples were highly amorphous and contained ferrihidrites and hydrated iron phosphate. According to XANES analyses of IRB, As associated with IRB was in +5 valence state when As (Ⅲ) (or As (Ⅴ)) was added in laboratory sorption test, Fe in +3 valence state, and Mn a mixture of+3 and +4 valence states. Small shift was observed in the XANES spectra of IRB on As K-edge as the equilibration time of the sorption experiment was increased. Gradual oxidation of a small amount of As (Ⅲ) associated with IRB or change in arsenic binding with sorption site were the probable mechanism. 相似文献
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本文着重探讨了人造金刚石触媒中的锰含量测试方法,通过试验,对比分析,认为该方法能够准确的测定触媒中的锰含量。 相似文献
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广西凤凰山锰银氧化矿可选性试验研究 总被引:3,自引:0,他引:3
锰银氧化矿是公认的难选冶矿石类型,在当前经济技术条件下仍属于难以利用的矿种。采用强磁选方法优先回收银锰、磁选尾矿氰化浸银的试验流程,获得银回收率达到90%的良好效果。 相似文献
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大洋多金属结核中1nm锰矿相的相变及其主要控制因素研究 总被引:1,自引:3,他引:1
多金属结核样品在室温中放置或加热干燥后 ,其中的 1nm锰矿相会部分或全部地相变为 0 7nm锰矿相 ,这说明 0 7nm锰矿相可能不是多金属结核的原生锰矿相 ,而仅仅是 1nm锰矿相的相变产物。研究结果表明 :1nm锰矿相结构中的Cu2 + 、Co2 + 、Ni2 + 等金属阳离子的含量与其结构稳定性有正相关关系 ,即金属离子含量越高 ,其结构越稳定 ,1nm锰矿相越不易相变为 0 7nm锰矿相 ,反之亦然 ;另外 ,不同金属阳离子稳定 1nm锰矿相结构的能力也不同 ,结核中几种主要金属阳离子对 1nm锰矿相结构的稳定能力从大到小为 :Ni2 + >Cu2 + >Co2 + >Zn2 + >Ca2 + =Mg2 + 。 相似文献
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吉林省土壤中有效锰、铜、钼和锌含量的时空变化 总被引:5,自引:0,他引:5
选择吉林省的五个大豆种植区(敦化、桦甸、榆树、农安、白城)、四个水稻种植区(白城、九台、延吉、梅河口)及3个草场分布区(镇赉、洮南、大安),对其土壤中有效锰、铜、钼和锌的含量在过去20年的变化作了比较和分析。经研究表明:吉林省土壤中有效锰和有效铜含量较20年前有所增高,有效钼含量总体呈降低趋势,中部部分地区和东部地区土壤有效锌含量降低,其余地区含量增高。空间分布东部高于中西部。 相似文献
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痕量铁和锰的化学发光检测 总被引:5,自引:1,他引:5
评述了国内外有关铁、锰的化学发光分析进展。从发光体系、操作方式、最佳条件、干扰离子、检测限等各个方面对化学发光法测定铁、锰及其它们与其它组分同时测定中的应用进行分类评述。 相似文献