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41.
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Margaret C. Graham John G. Farmer Ian W. Oliver Angus B. MacKenzie Robert M. Ellam 《中国地球化学学报》2006,25(B08):112-112
Natural uranium has three isotopes, ^238U, ^235U and ^234U, with natural abundances of 99.27 atom %, 0.72% and 0.0055%, respectively. Only ^235U is fissile and the production of nuclear fuel and nuclear weapons involves enrichment of uranium in ^235U. This process also results in separation of ^234U from ^238U, leaving depleted uranium (DU), with typical ^234U/^238U and ^235U/^238U activity ratios of about 0.19 and 0.013, respectively, as a waste product. The high density, high melting and boiling points and chemical stability of uranium and the availability of DU in relatively pure form mean that DU has many uses, including armour-piercing munitions. Such munitions have been developed in the UK since the 1960s and testing has been carried out by the Ministry of Defence (MoD) at firing ranges such as Dundrennan, SW Scotland and Eskmeals, NW England. The firing of DU munitions can result in the dispersion of DU and its combustion products (oxides) as aerosols or as larger fragments, with the potential for human exposure either directly at the site of detonation or via post-depositional migration in the environment. The aim of this work was to investigate the potential environmental mobility of DU by characterizing the associations of U in soil porewaters with increasing distance from a firing site. To this end, several soil cores located down-wind of the firing site at Dundrennan, near Kirkcudbright, SW Scotland, were collected in May 2006. These were sectioned on-site into 1- or 2-cm depth intervals and porewaters were isolated by centfifugation (10 minutes; 8873 g) on return to the laboratory. Following filtration through 0.2-micron cellulose nitrate filters, the porewaters were analyzed by ICP-QMS (U concentration) and ICP-OES (Fe, Al, Ca, Mg, Mn concentrations). Sub-samples were also subjected to centrifugal ultrafiltration (100, 30, and 3 kD) and to gel electrophoretic fractionation (agarose; 0.045 M Tris-borate; 20 mA, 30 minutes). Results showed that U was present at up to 4 μg/L in the soil porewater and that the associations of U varied with sample location and soil depth. 相似文献
43.
Yoko Shimamoto Yoshio Takahashi 《中国地球化学学报》2006,25(B08):114-114
Although inorganic species are predominant in natural systems, but there are many kinds of organoarsenic species such as methylated and phenylated arsenic compounds. Phenylarsonic acid (PA) is a degradation product of organoarsenics used for chemical warfare agents, which has been detected in well water at the disposal site of the agents in Japan. There are few reports studying behavior of PA in soil. In this study, PA was adsorbed onto ferrihydrite and its chemical forms were determined using high performance liquid chromatography connected to inductivity-coupled plasma mass spectrometry (HPLC-ICP-MS). 100 mg/kg of PA was mixed with 0.03 g of 2-line ferrihydrite. For each suspension, pH was adjusted by HNO3 or NaOH. Each sample was incubated for more than 19 hours and the final pH was measured. After filtration, the chemical form of arsenic in the filtrate was measured using HPLC-ICP-MS. In addition, ferrihydrite separated by filtration was dissolved by 3 ml of 0.5 M HCI and the arsenic species in the solution was detected by HPLC-ICP-MS (column: Tosoh TSKgel SuperlC-AP, eluent: 0.01 M HNO3). It was verified that PA is not degraded by heating in 0.5 M HCl solution. At pH 3.1, any arsenic compounds were not detected from the solution, because almost all arsenic species were adsorbed onto ferrihydrite at lower pH. At pH= 12, however, 7%-10% of inorganic arsenic was detected in the solution. In solid phase, there are some problems to determine the precise ratio of inorganic and organic species. When the solution includes Fe ion at 0.01 M level, the retention time of arsenic species drifted compared to those in standard solution, which makes it difficult to determine precisely the arsenic species adsorbed on ferrihydrite. Therefore, more study is needed to determine the ratio of inorganic and organic species in the system. 相似文献
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Rajasekhar Balasubramanian Chanbasha Basheer Kang Lisa Siao Wei See 《中国地球化学学报》2006,25(B08):183-183
Microorganic pollutants such as polycylic aromatic hydrocarbons (PAHs), organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs) and total petroleum hydrocarbons (TPHs) are known to be present in urban ambient air. These organic compounds are prone to atmospheric transport and deposition over long distances, thus enabling them to accumulate even in regions remote from their sources. Deposition from the atmosphere can be via direct deposition and exchange with crops that may be directly or indirectly ingested by humans. It can also take place via wet and dry deposition and air-water exchange. Following their deposition, these microorganic pollutants tend to accumulate in soils, sediments and in human and ecological food chains. There are many reports in the literature on the atmospheric concentrations of microorganic pollutants, but there are few reports and data in Asia. This study was performed in Singapore to determine the relative amounts of persistent organic pollutants and TPHs in ambient aerosols. One of the important sources of these organic compounds in Southeast Asia is thought to be biomass burning (vegetation fires). Hence, air sampling was conducted during both smoke haze and non-haze periods. The data obtained from this study will be presented and discussed. 相似文献
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Sivaji Patra Congqiang LIU Siliang LI Fushun WANG Baoli WANG 《中国地球化学学报》2006,25(B08):269-270
Geochemical cycling has received wide attention due to the need to understand the pathways of pollutants through our present environment. In this regard the Yangtze River plays a significant role in putting those pollutants into the East China SeafWorld Oceans. The Yangtze River is of high sedimentation rate and water discharge. The watershed covers variable climate regions from temperate to subtropical and from semiarid to humid. Twenty three (23) sampling locations at the estuary have been selected for understanding the dynamic relationships. The elements (Cl^-, SO4^2-, Na^+, K^+, and Ca^2+) show conservative behavior during mixing of fresh water with saline water whereas Mg^2+, Mn^2+ show a non-conservative pattern . The relationships between Na^+/SO4^2- and Cl^-/SO4^2- molar ratios show a mixing of more than two water sources. 相似文献
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苦竹岽锡矿位于密坑山杂岩体北西部边缘与侏罗系上统鸡笼嶂组火山岩接触部位,明显受近东西向、南北向断裂带和接触带三者控制,为岩浆期后高中温气化热液微细脉浸染型矿床。在矿山探(采)过程中,进一步分析研究了锡矿的控矿因素和矿体的变化规律,指导矿山探(采)工程的布置,收到良好的效果,对今后矿山的探(采)工作具有较大的现实意义。 相似文献
50.
针对航天INSAR主、辅影像数据的特点,提出了加大匹配窗口、加大锚点间隔的匹配策略,以提高匹配的可靠性和速度.在匹配过程中,综合利用轨道参数和强度影像金字塔进行粗匹配,并对强度影像采用相关系数与最小二乘相结合的双向匹配方案,实现了自动、快速、高可靠性和高精度的航天INSAR复影像匹配.最后总结了航天INSAR复影像匹配的特点. 相似文献