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111.
Yunchao HAO Zhigang GUO Dejiang FAN 《中国地球化学学报》2006,25(B08):13-13
In the East China Sea (ECS), there are some mud areas, including the south coastal mud area, the north coastal mud area, and the mud area to the southwest of Cheju Island. X-ray fluorescence (XRF) techniques and Thermal Ionization Mass Spectrometry (TIMS) were used to study the high-resolution sedimentary record of Pb concentrations and Pb stable isotopic compositions in the past one hundred and fifty years in the coastal mud of the ECS. Pb concentrations of a ^210Pb dating S5 core in the study area have increased rapidly since 1980, and reached the maximal value with 65.08 μg/g in 2000, corresponding to the fast economic development of China since the implementation of the "Reform and Open Policy" in 1978; ^206Pb/^207Pb ratios generally had stabilized at 1.195 from 1860 to 1966, and decreased gradually from 1966 to 2000, indicating that the anthropogenic source Pb contribution to the ECS has increased gradually since 1966, especially since 1980. Pb concentrations decreased distinctly from 2000 to 2003 and ^206Pb/^207Pb ratios increased from 2001 to 2003, corresponding closely to the ban of lead gasoline from 2000 in China. From 1950 to 2003, there occurred four distinct decrease events of ^206Pb/^207Pb, possibly responding to the Changjiang River (Yangtze River) catastrophic floods in 1998, 1991, 1981 and 1954; from 1860 to 1966, there were two decrease periods of ^206Pb/^207Pb, which may respond to the catastrophic floods of Changjiang River in 1931 and 1935, and 1870. As a result of the erosion and drowning by the catastrophic floods, the anthropogenic lead accumulated in soil and water environments over a long period of time was brought into the Changjiang River, then part of them was finally transported into the ECS, which leads to changes in Pb stable isotopic composition. 相似文献
112.
Wei ZHANG Congqiang LIU Zhiqi ZHAO 《中国地球化学学报》2006,25(B08):172-172
Boron has two stable isotopes (^10B and ^11B) with relative abundances of about 20% and 80%, respectively. Boron isotopic ratios in natural materials show a huge range of variations, from -70‰ to +60‰, when expressed with the classical δ^11B notation. Most of these isotopic variations occur at the surface of the Earth. Hence, boron isotopic composition can be used as a sensitive tracer in geochemical study, for instance, to identify the different sources of contamination and factors controlling the salinity of groundwater. During the last decade, boron isotopes have been used to discriminate between the influences of seawater intrusion and anthropogenic discharge. But few of those researches can precisely identify the different sources of contamination. We measured the boron concentrations and boron isotopic ratios of groundwater samples collected in Guiyang City, as well as the major ions. The results indicate that the major ion composition of the groundwater in the investigated area is mainly controlled by the interactions between water and the dominant rock i.e. carbonates. All the water compositions are characterized by high concentrations of Ca^2+, Mg^2+, HCO3^-, SO4^2-, and NO3^-, which are the dominant contaminants. Both dissolved boron concentrations and isotopic ratios show large variations among the ground waters, from 2 μg/L to 90 μg/L and from -6‰ to +26‰, respectively. The boron concentrations and isotopic ratios indicate that the river across the studied city has been seriously contaminated by urban discharge. Boron concentrations of fiver water samples varied from 20 μg/L to 140 μg/L, with an average δ^11B value of +2.0‰. Using boron isotopic compositions and different geochemical indices allowed us to clearly identify and distinguish the two major sources of contamination, agricultural activity and urban wastewater. Both of the two sources are characterized by high boron concentrations but their boron isotopic compositions significantly differ. 相似文献
113.
Houyi ZHENG Congqiang LIU Zhongliang WANG 《中国地球化学学报》2006,25(B08):174-174
Bedrock weathering and atmospheric deposition are the two primary sources of base cations (K^+, Na^+, Ca^2+ and Mg^2+) to forest ecosystems. Therefore, the key problem is to understand the relative inputs from these two sources and the cycling in the ecosystem. This study focuses on the effects of acid deposition on cation cycling in a small-forested karstic catchment in Guizhou Province. Sr isotope ratios were used as a tracer for understanding the transport process between the different cation pools: rock, soil, surface water, atmospheric deposition and plant. The samples of wet deposition, total deposition, throughfall, surface and ground waters, vegetation, and soil were monthly collected. The exchangeable Sr^2+ and Ca^2+ in soil samples were extracted by using 1 M ammonium acetate. The leaf-tissue samples were ashed at 550℃, and the residue was digested in ultrapure HClO4 and HNO3. All water samples were filtrated through 0.45 μm aperture filter paper. Base cation concentrations and Sr isotopic composition were analyzed for all the samples. The results show that acid deposition (average pH 4.9) frequently occurred in the studied region. Cation abundance follows an increasing manner from rainwater, throughfall, to surface water or ground water samples, suggesting that acid deposition at first eiuviates Ca^2+ , Mg^2+ and Sr^2+ from leaf, then the exchangeable cations from soil, and at last cations accumulate in surface water or ground water. 相似文献
114.
Hydrogen isotope of individual n-alkanes from modern sediments and their application to environments
Zhongping LI Liwu LI Li DU 《中国地球化学学报》2006,25(B08):207-207
Hydrogen isotopes are commonly fractionated to a much greater extent and as a result display larger variations in δ values, In terms of the hydrogen isotope ratios of individual n-alkanes of 16 samples of modern sediments selected from four different locations in the southern part of Gansu, China, the δD values for most of the n-alkanes varied from -150‰-300‰, Variations in δD also occurred between different ranges of n-alkanes, effects of environmental changes on the hydrogen isotopic compositions of individual n-alkanes have been detected. Besides the δD values of n-alkanes, the δD values of lipids including pristane (Pr), phytane (Ph) were also examined, by the combination of D/H ratios with molecular fingerprinting, Our results further support the notion that hydrogen isotopes of n-alkanes from modern sediments can act as paleoclimatic and paleoenvironmental proxies and provide invaluable new sources of information in the research of paleoenvironment reconstruction. 相似文献
115.
从分析大湾铀矿田各矿床(点)的铀镭平衡系数变化特征出发,结合放射性同位素比值特征分析铀镭迁移富集行为,指出了各矿床(点)氧化带的深度,以了解各铀矿床(点)潜在的工业价值. 相似文献
116.
库车坳陷侏罗系煤成气动力学模拟研究 总被引:1,自引:0,他引:1
应用黄金管—高压釜封闭体系热模拟实验与GC、GC-IRMS分析技术,结合KINETICS专用软件,对库车坳陷侏罗系煤成气进行了动力学模拟研究。库车坳陷侏罗系煤具有高的产气性,在高演化阶段主要产甲烷气;侏罗系煤热解气甲烷碳同位素为-36‰~-25‰,乙烷碳同位素为-28‰~-16‰;甲烷、C2-C5气态烃的生成活化能分别为(47~64k)calm/ol、(55~72k)calm/ol,频率因子各为5.265×1013s-1、5.388×1018s-1。在此基础上,进一步探讨了克拉2气田天然气的成因。研究认为,克拉2气田天然气属阶段捕获的煤成气,主要聚集了5~1Ma时期的天然气,其成熟度Ro分布范围为1.3%~2.5%。 相似文献
117.
118.
ZHANG Jian-min ZHAO Yong-zhong XU Jing HUANG Juan The Logging Company Jilin Petroleum Group Co. Ltd Songyuan Jilin China 《吉林大学学报(地球科学版)》2006,(Z2)
吉林油田同位素吸水剖面测井采用~(113)In同位素追踪技术,根据同位素追踪过程解释基本可以判断配水层段吸水情况。但是在注水井存在沾污、大孔道以及串槽等影响时,吸水面积确定比较困难。在同位素测井中增加井温、流量参数,通过多参数综合解释,不仅可以对沾污影响进行合理校正,确定准确的小层吸水量,而且能够正确判断各级封隔器、配水器的工作情况,在地层存在大孔道的情况下,确定地层的吸水面积。吸水剖面综合解释方法在吉林油田已普遍应用,见到明显的效果。 相似文献
119.
120.