No evidence for a decrease of nuclear decay rates with increasing heliocentric distance based on radiochronology of meteorites

It has been argued that the decay rates of several radioactive nuclides are slightly lower at Earth’s aphelion than at perihelion, and that this effect might depend on heliocentric distance. It might then be expected that nuclear decay rates be considerably lower at larger distances from the sun, e.g., in the asteroid belt at 2–3 AU from where most meteorites originate. If so, ages of meteorites obtained by analyses of radioactive nuclides and their stable daughter isotopes might be in error, since these ages are based on decay rates determined on Earth. Here we evaluate whether the large data base on nuclear cosmochronology offers any hint for discrepancies which might be due to radially variable decay rates. Chlorine-36 (t_1/2 = 301,000 a) is produced in meteorites by interactions with cosmic rays and is the nuclide for which a decay rate dependence from heliocentric distance has been proposed, which, in principle, can be tested with our approach and the current data base. We show that compilations of ³⁶Cl concentrations measured in meteorites offer no support for a spatially variable ³⁶Cl decay rate. For very short-lived cosmic-ray produced radionuclides (half-lives < 10–100 days), the concentration should be different for meteorites hitting the Earth on the incoming vs. outgoing part of their orbit. However, the current data base of very short-lived radionuclides in freshly fallen meteorites is far from sufficient to deduce solid constraints. Constraints on the age of the Earth and the oldest meteorite phases obtained by the U–Pb dating technique give no hints for radially variable decay rates of the α-decaying nuclides ²³⁵U or ²³⁸U. Similarly, some of the oldest phases in meteorites have U–Pb ages whose differences agree almost perfectly with respective age differences obtained with “short-lived” radionuclides present in the early solar system, again indicating no variability of uranium decay rates in different meteorite parent bodies in the asteroid belt. Moreover, the oldest U–Pb ages of meteorites agree with the main-sequence age of the sun derived from helioseismology within the formal ∼1% uncertainty of the latter. Meteorite ages also provide no evidence for a decrease of decay rates with heliocentric distance for nuclides such as ⁸⁷Rb (decay mode β⁻) ⁴⁰K (β⁻ and electron capture), and ¹⁴⁷Sm (α).     

太阳系~(53)Mn-~(53)Cr同位素体系

短周期放射性核素的初始丰度和分布情况,已成为陨石学和天体化学的重要研究领域之一。已有研究证实地外天体中53 Cr的放射性母体为53 Mn。53 Mn的半衰期为3.7±0.4Ma,可对太阳系形成之后的20Ma内发生的事件进行精确定年。本文系统总结了已报道的碳质球粒陨石、普通球粒陨石、顽辉石球粒陨石和分异陨石中的53 Mn-53 Cr同位素体系数据,依据55 Mn/52 Cr值和53 Cr异常探讨了太阳系形成时53 Mn和53 Cr的初始分布情况、太阳系初始的53 Mn/55 Mn值,讨论了陨石中普遍存在的54 Cr/52 Cr值异常和碳质球粒陨石全岩的54 Cr和53 Cr异常值之间的正相关关系对53 Mn-53 Cr体系定年影响。     

GGR Biennial Critical Review: Analytical Developments Since 2012

Advances in the chemical, crystallographic and isotopic characterisation of geological and environmental materials can often be ascribed to technological improvements in analytical hardware or to innovative approaches to data acquisition and/or its interpretation. This biennial review addresses key laboratory methods that form much of the foundation for analytical geochemistry; again, this contribution is presented as a compendium of laboratory techniques. We highlight advances that have appeared since January 2012 and that are of particular significance for the chemical and isotopic characterisation of geomaterials. Prominent scientists from the selected analytical fields present publications they judge to be particular noteworthy, providing background information about the method and assessing where further opportunities might be anticipated. In addition to the well‐established technologies such as thermal ionisation mass spectrometry and plasma emission spectroscopy, this publication also presents new or rapidly growing methods such as electron backscattered diffraction analysis and atom probe tomography – a very sensitive method providing atomic scale information.     

Altitude-dependent distribution of ~(137)Cs in the environment:a case study of Aragats massif,Armenia

This paper considers the distribution of technogenic 137Cs and naturally occurring radionuclides:238 U,232 Th and40 R concentrations in soils and 137Cs in atmospheric dry depositions by altitudinal belts of the Aragats mountain massif,Republic of Armenia.Undisturbed soil samples were collected at altitudes from 1000 to 3200 m.For the determination of geochemical variability,two soil sampling campaigns were undertaken.Atmospheric dry depositions were sampled from five stations at1100-3200 m collected onto organic fiber filters between June and December 2016.137Cs activity was measured using a high-purity Germanium detector coupled to a multichannel analyzer(Canberra).Results indicated that specific activity of 137Cs in soils at 1000 m is495-528 Bq m^-2,andat3200 mis10,500-11,470 Bq m^-2.No correlation observed for 137Cs versus naturally occurring radionuclides,which varies in distribution by altitude.Specific activities of 137Cs in dry atmospheric depositions varies from 1.06 at 846 m to2.37 Bq m^-2 per quarter at 3200 m and increases as the altitude increases.Activities of 137Cs in soil and dry atmospheric deposition correlated significantly,and 137Cs activity in soils and atmospheric dry depositions decrease as the absolute altitude decreases.The 50-year effective dose from exposure to 137Cs fallout varies with altitude from 0.007 to 1.42 m Sv.     

Forty years of anthropogenic radionuclides in surface seawater. Italian and Japanese data

The concentrations of man made radionuclides in surface seawater since early ′60s are here reported as measured in Italy and Japan. Most of the data refers to⁹⁰Sr and¹³⁷Cs, but occasionally the concentrations of⁸⁹Sr and¹³⁴Cs in some Italian samples are also given. The main sources of man made radionuclides were the global fallout produced by the nuclear weapon tests and the Chernobyl accident. The respective contributions to the contamination of surface seawater around both countries are discussed.     

Effects of gradient,distance, curvature and aspect on steep burned and unburned hillslope soil erosion and deposition

Wildfire denudes vegetation and impacts chemical and physical soil properties, which can alter hillslope erosion rates. Post‐wildfire erosion can also contribute disproportionately to long‐term erosion rates and landscape evolution. Post‐fire hillslope erosion rates remain difficult to predict and document at the hillslope scale. Here we use ²¹⁰Pb_aex (lead‐210 mineral‐adsorbed excess) inventories to describe net sediment erosion on steep, convex hillslopes in three basins (unburned, moderately and severely burned) in mountainous central Idaho. We analyzed nearly 300 soil samples for ²¹⁰Pb_aex content with alpha spectrometry and related net sediment erosion to burn severity, aspect, gradient, curvature and distance from ridgetop. We also tested our data against models for advective, linear and non‐linear diffusive erosion. Statistically lower net soil losses on north‐ versus south‐facing unburned hillslopes suggest that greater vegetative cover and soil cohesion on north‐facing slopes decrease erosion. On burned hillslopes, erosion differences between aspects were less apparent and net erosion was more variable, indicating that vegetation influences erosion magnitude and fire drives erosion variability. We estimated net soil losses throughout the length of unburned hillslopes, including through a footslope transition to concave form. In contrast, on burned hillslopes, the subtle shift from convex to concave form was associated with deposition of a post‐fire erosion pulse. Such overall patterns of erosion and deposition are consistent with predictions from a non‐linear diffusion equation. This finding also suggests that concave sections of overall convex hillslopes affect post‐disturbance soil erosion and deposition. Despite these patterns, no strong relationships were evident between local net soil losses and gradient, curvature, distance from ridgetop, or erosion predicted with advection or diffusion equations. The observed relationship between gradient and erosion is therefore likely more complex or stochastic than often described theoretically, especially over relatively short timescales (60–100 years). Copyright © 2016 John Wiley & Sons, Ltd.