Parsivel~激光降水粒子谱仪及其在气象领域的应用

降水粒子特性是大气运动和云内微物理过程的综合结果,在云降水物理及人工影响天气领域有着重要的意义。传统的测量方法不适合对大量数据分析寻找规律,德国OTT公司的Parsivel激光降水粒子谱测量系统可以较好解决自动测量难题。该仪器是以激光测量为基础的粒子测量传感器,采用平行激光束和光电管阵列结合,当有降水粒子穿越采样空间时,自动记录遮挡物的宽度,通过穿越时间计算降水粒子的尺度和速度,根据各种参数的综合信息对降水粒子进行分类,并能够以数字形式显示瞬时降水强度、降水粒子总数、累积降水量、降水时的能见度和雷达反射因子,以图形方式显示降水粒子尺度谱、速度谱、降水粒子分类且自动生成天气现象代码,实现天气现象的自动识别。激光降水粒子谱仪主要用于气象水文观测。在雷达气象学领域可用于Z/R关系的拟合修正,比传统的用雨量筒观测数据拟合效果好得多;由降水粒子谱仪测量雨滴的降落速度,可以对天气雷达垂直向上测量的粒子径向速度谱进行校正。人工影响天气的效果检验一直是一个难题,自然降水粒子谱分布形式与人工催化以后的降水粒子谱型理论上应当具有较大的差别,人工增雨作业降水滴谱变化物理响应和降水强度时间变化响应都有明显的区别。如果能够实时检测到这些差别,就能够充分说明人工催化的有效性。未来如果能够进行联网观测记录区域性降水、降雹,就有充分证据表明人影作业的有效性,在定量化作业效果评估以及灾害损失评估等方面应用潜力巨大。利用该仪器已经对一年的自然降水过程进行了连续观测,并将所获得的降水粒子谱、雨滴浓度值随时间变化状况与卫星反演的云顶有效粒子半径时间变化趋势进行了对比,发现有较好的一致性。     

Octahedral cation ordering in olivine at high temperature. I: in situ neutron single-crystal diffraction studies on natural mantle olivines (Fa12 and Fa10)

Crystallographic determinations on natural olivine single crystals of mantle composition and origin, carried out by in situ neutron diffraction at high temperature, show that the octahedrally co-ordinated Fe²⁺ and Mg cations undergo two successive trends of cation ordering with increasing temperature. An initial slight preference of Fe²⁺ for site M1, up to a temperature of about 850?°C, is followed by a reverse-ordering reaction with a site preference exchange between the two cations. The cross-over between the two regimes of ordering, corresponding to a situation of complete disorder, occurs at about 900?°C. Above this temperature Fe²⁺ progressively and strongly segregates into site M2 up to 1300?°C, the practical limit of the experimental setup utilized in the experiments. Care was taken to ensure that no chemical changes occurred in the crystals (i.e. oxidation), as testified by Mössbauer spectroscopy determinations carried out before and after the heat treatment. The cation-ordering behaviour is reflected in temperature-dependent changes of geometrical and atomic displacement parameters occurring in the octahedral sites M1 and M2. A thermodynamical explanation of this behaviour is proposed in terms of a prevailing vibrational contribution to entropy.     

北大西洋-东亚和北亚型遥相关的机制及其对新疆夏季旱涝的影响

北大西洋-东亚和北亚（简称NAENA）型遥相关是夏季欧亚大陆对流层上层经向风异常的第二主导模态,对欧亚大陆多尺度气候变率有显著影响。本文在分析NAENA型维持的动力学机制的基础上,研究了该遥相关型对新疆夏季旱涝异常的影响及其可能机制。大气波列的涡度收支分析表明,气候态的旋转纬向风引起的扰动涡度平流可以被扰动旋转经向风引起的平均涡度平流所补偿。能量转换过程分析表明,该大气波列有效地从平均流中提取有效位能,通过斜压能量转换过程得以维持。大西洋海温异常三极子模态则是NAENA型维持的重要外强迫因子。回归分析表明NAENA型遥相关能通过促进南疆夏季降水,显著影响新疆的旱涝异常。NAENA型位于中亚的气旋性低压一方面增强了南疆地区的垂直上升运动,同时气旋性环流将更多的水汽输送到该地区,有利于水汽在对流层中低层的异常辐合,进而对南疆的降水有促进作用。     

2017年江西汛期设区市城区暴雨回波特征分析

使用江西WebGIS雷达拼图和自动站雨量、雷电监测、强天气监测等数据,以及MICAPS常规天气图资料,对2017年3—7月江西汛期11个设区市26次城区暴雨过程的雷达回波特征进行分析。结果表明:2017年江西汛期共出现52日暴雨过程,其中江西11个设区市所在地城区出现26次暴雨。在这26次城区暴雨个例中,有23次伴随出现短时强降水,有3次降水比较均匀。暴雨维持时间长短不一,最长的有15 h,最短只有3 h,平均是10 h。有5次出现大风天气,21次没有大风出现。雷达回波特征主要有3种:块状(强单体、超级单体)、带状(飑线、回波带)、絮状(絮带、絮团)。这3种回波形态特征,出现率最高的是絮状回波,即比较宽、嵌有中等强度的对流单体絮带状回波带,强度40～55 dBz,出现16次,概率62%;其次是窄而长、紧密排列由强单体组成的飑线回波带,强度50～60 dBz,出现8次,概率30%;块状(强单体、超级单体)回波强度最强,中心强度达到60～70 dBz,出现2次,概率8%。     

海河流域严重干旱500hPa信号场异常信号分析

基于严重少雨旬的定义,分析海河流域1961～2009年严重少雨旬的分布特征,进而对汛期40个典型严重少雨旬的500hPa信号场进行经验正交分解(EOF分析).结果表明:EOF第一模态的方差贡献率达到35.3％,远高于其他模态;第一模态呈现出2个负异常区和1个正异常区,在对应的环流背景下,海河流域受暖性高压控制,高纬冷空气及低纬暖湿气流难以到达流域上空交绥,持续高温少雨造成流域严重干旱.     

Likely effects of climate change on groundwater availability in a Mediterranean region of Southeastern Spain

Groundwater resources are typically the main fresh water source in arid and semi‐arid regions. Natural recharge of aquifers is mainly based on precipitation; however, only heavy precipitation events (HPEs) are expected to produce appreciable aquifer recharge in these environments. In this work, we used daily precipitation and monthly water level time series from different locations over a Mediterranean region of Southeastern Spain to identify the critical threshold value to define HPEs that lead to appreciable aquifer recharge in this region. Wavelet and trend analyses were used to study the changes in the temporal distribution of the chosen HPEs (≥20 mm day^?1) over the observed period 1953–2012 and its projected evolution by using 18 downscaled climate projections over the projected period 2040–2099. The used precipitation time series were grouped in 10 clusters according to similarities between them assessed by using Pearson correlations. Results showed that the critical HPE threshold for the study area is 20 mm day^?1. Wavelet analysis showed that observed significant seasonal and annual peaks in global wavelet spectrum in the first sub‐period (1953–1982) are no longer significant in the second sub‐period (1983–2012) in the major part of the ten clusters. This change is because of the reduction of the mean HPEs number, which showed a negative trend over the observed period in nine clusters and was significant in five of them. However, the mean size of HPEs showed a positive trend in six clusters. A similar tendency of change is expected over the projected period. The expected reduction of the mean HPEs number is two times higher under the high climate scenario (RCP8.5) than under the moderate scenario (RCP4.5). The mean size of these events is expected to increase under the two scenarios. The groundwater availability will be affected by the reduction of HPE number which will increase the length of no aquifer recharge periods (NARP) accentuating the groundwater drought in the region. Copyright © 2016 John Wiley & Sons, Ltd.     

运用STOMP数值模拟器进行多空介质中尿素水解以及方解石沉淀数值模拟

遍布于美国能源部所辖野外场地的地下放射性核素和痕量金属污染对美国能源部的长期监管职能提出了最严峻的挑战。目前较有前景的一个原地固化污染物方法是利用尿素酶催化尿素水解,进而推动方解石沉淀及与之共同沉淀。运用STOMP数值模拟器实施一系列反应性溶质数值模拟来研究系统中水流、运移、反应与反应导致的介质性质变化之间的紧密的非线性耦合,并在研究中系统性增加反应系统的复杂度和物理-化学的非均质性以考察模拟效果。通过调整反应速率表达式中尿素酶浓度和沉淀反应常数,对尿素水解和方解石沉淀速率进行了敏感度分析。结果显示:尿素水解速率是矿物沉淀总量的决定性因素,沉淀物的空间分布既取决于水解速率也取决于沉淀速率;在一维水流柱6个空隙体积的时间段模拟中,观察到了5%的最大空隙度减少;当二维模拟中考虑一个低渗透性包裹体时,被改变的流场重新对生成的沉淀组成物进行了分布,形成了扭曲的反应锋面。模拟结果也显示沉淀在低渗透性区域边界上形成,这说明位于这个区域里面的污染物可能被囊裹而从流线中被隔离起来。     

北大西洋涛动和南半球环状模不同位相配置对我国南方夏季降水的协同影响

利用我国气象台站观测资料和再分析格点数据,诊断研究了前期春季（4-5月份）北大西洋涛动（North Atlantic Oscillation,NAO）和南半球环状模（Southern Annular Mode,SAM）在不同位相配置下对我国南方夏季降水异常变化的协同影响作用.分析结果表明,在剔除ENSO最强信号影响后,我国南方夏季降水异常分布显著地依赖于前期春季两个较为独立的年际变率主模态（NAO和SAM）位相的不同配置,即降水异常型主要表现为两个因子单独作用的叠加效果.当前春SAM正位相偏强而NAO负位相偏强时,二者的影响呈现协同正效应,我国南方夏季（6-7月份）降水表现为全区正异常,特别在长江中下游及其以南附近地区最为显著;反之,当前春SAM呈偏强的负位相而NAO偏强的正位相配置时,二者的影响呈现协同负效应,对应我国夏季长江中下游地区降水表现为显著负异常.对其可能的影响机理研究表明,在SAM与NAO位相相反情况下,二者均会通过海气相互作用过程影响到热带大西洋北部海温的异常变化,进而形成协同作用,增强北大西洋海温三极子模态异常信号,从而通过欧亚大陆的遥相关波列对东亚夏季风和我国南方降水产生显著影响.相比之下,当SAM与NAO同位相时,可能表现为抵消效应,不利于北大西洋海温三极子发展,从而削弱对我国南方夏季降水的影响,此方面还有待进一步研究.

     

On the origin of oriented rutile needles in garnet from UHP eclogites

Although oriented rutile needles in garnet have been reported from several ultrahigh‐pressure (UHP) rocks and considered to be important UHP indicators, their crystallographic features including growth habit and lattice correspondences with garnet host have never been properly characterized. This paper presents a detailed analytical electron microscopic (AEM) study on evenly distributed oriented rutile needles in garnet of two eclogitic rocks from Sulu. Some garnet in one UHP diamondiferous quartzofeldspathic rock from the Saxonian Erzgebirge, and in one high‐pressure (HP) felsic granulite from Bohemia also contain a few unevenly distributed oriented rutile needles. They have also been studied for the purpose of comparison. Despite different distribution patterns, AEM revealed that all rutile needles are oriented along the 〈111〉 directions of garnet with their lateral sides surrounded by the {110} planes of garnet, and that the growth directions of most needles are close to the normal of the {101} planes of rutile. No other specific crystallographic orientation relationships between rutile and garnet host were observed, and there is no pyroxene associated with rutile, as necessitated by the precipitation reaction of rutile in garnet as previously proposed. A simple solid‐state precipitation scenario for the formation of the rutile needles in garnet in these two eclogitic rocks is not justified. Three alternative mechanisms are considered for the formation of oriented rutile needles: (i) the rutile needles may be inherited from precursor minerals; (ii) the rutile needles may be formed by a dissolution–reprecipitation mechanism; and (iii) the rutile needles may be formed by cleaving and healing of garnet with rutile deposition. None of these mechanisms can fully explain the observations, although the first one is less likely and the third one is preferred. This study presents an example where the presence of oriented/aligned inclusions in minerals does not necessarily imply a precipitation origin.     

洞穴滴水、石笋中元素及元素比值对气候环境变化响应的研究进展

滴水/石笋元素是除δ18O和δ13C,研究气候环境变化的又一重要代用指标。外界气候环境变化通过改变表层岩溶带和岩溶含水层中的水文环境,甚至洞穴环境,进而影响元素的溶解、运移和沉淀过程,从而使得滴水/石笋中元素表现一定的变化规律。本文通过分析影响洞穴滴水元素及元素比值变化的因素：元素来源、水—岩相互作用和滞留时间、差异性淋滤、先期碳酸盐沉淀及分配系数的基础上,从元素对岩溶区“二元结构”和极端天气/气候事件响应的角度,探讨了滴水/石笋中元素的气候环境指示意义。取得了以下认识：① 强降水带来的冲刷作用和溶解作用,促进土壤和基岩中元素、胶体和天然有机质（NOM：Natural Organic Matter）等物质在短时间内快速溶解和运移,使滴水中元素含量增加;但随着降水增多带来的稀释作用,使得滴水/石笋中Mg,Sr和Ba等元素含量降低,因此,单一元素的解译较为复杂;② 基岩/溶液中元素溶解和沉积的差异,导致元素相对含量的变化,使得元素X/Ca值对外界环境的响应具有一致性,尤其是Mg/Ca和Sr/Ca值：在干旱条件下,降水减少导致方解石先期沉积（PCP：Prior Calcite precipitation）作用增强,使Mg/Ca和Sr/Ca值增大。但目前存在着一些问题：① Mg/Ca和Sr/Ca值变化对强降水事件的响应并不明显,可能与新、老水混合及元素溶解过程中的溶解比例差别不大有关;② 多源、多期混合水源会导致洞穴滴水元素对极端事件响应减弱;③ Mg/Ca和Sr/Ca的变化为解释δ18O的“雨量效应”及“源效应”提供了见解,但元素变化能否反映季风强度的变化,仍有待进一步的研究。基于以上认识,笔者提出开展更加系统的大气—土壤—包气带—洞穴的监测;开展更高分辨率、更长时间尺度的洞穴监测;开展多区域、多洞穴系统对比研究来更加深入地开展洞穴石笋元素研究。