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941.
A three-dimensional model of the global ammonia cycle 总被引:16,自引:0,他引:16
Using a three-dimensional (3-D) transport model of the troposphere, we calculated the global distributions of ammonia (NH3) and ammonium (NH
4
+
), taking into account removal of NH3 on acidic aerosols, in liquid water clouds and by reaction with OH. Our estimated global 10°×10° NH3 emission inventory of 45 Tg N-NH3 yr– provides a reasonable agreement between calculated wet NH
4
+
deposition and measurements and of measured and modeled NH
4
+
in aerosols, although in Africa and Asia especially discrepancies exist.NH3 emissions from natural continental ecosystems were calculated applying a canopy compensation point and oceanic NH3 emissions were related to those of DMS (dimethylsulfide). In many regions of the earth, the pH found in rain and cloud water can be attributed to acidity derived from NO, SO2 and DMS emissions and alkalinity from NH3. In the remote lower troposphere, sulfate aerosols are calculated to be almost neutralized to ammonium sulfate (NH4)2SO4, whereas in the middle and upper troposphere, according to our calculations, the aerosol should be more acidic, as a result of the oxidation of DMS and SO2 throughout the troposphere and removal of NH3 on acidic aerosols at lower heights. Although the removal of NH3 by reaction with the OH radical is relatively slow, the intermediate NH2 radical can provide a substantial annual N2O source of 0.9
–0.4
+0.9
Tg, thus contributing byca. 5% to estimated global N2O production. The oxidation by OH of NH3 from anthropogenic sources accounts for 10% of the estimated total anthropogenic sources of N2O. This source was not accounted for in previous studies, and is mainly located in the tropics, which have high NH3 and OH concentrations. Biomass burning plumes, containing high NO
x
and NH3 concentrations provide favourable conditions for gas phase N2O production. This source is probably underestimated in this model study, due to the coarse resolution of the 3-D model, and the rather low biomass burning NH3 and NO
x
emissions adopted. The estimate depends heavily on poorly known concentrations of NH3 (and NO
x
) in the tropics, and uncertainties in the rate constants of the reactions NH2 + NO2 N2O + H2O (R4), and NH2 + O3 NH2O + O2 (R7). 相似文献
942.
San-Shyan Lin J. L. Hong Wei F. Lee Y. H. Chang 《Soil Dynamics and Earthquake Engineering》2004,24(11):829-838
A procedure that uses the structural damping (SD) concept for estimating the capacity of a pile based on the Statnamic (STN) pile load test results, formerly used by the authors for short piles, is extended in this paper for the STN tested long piles. Similar to segmental unloading point method procedures for long piles, the shaft length is divided into several segments and each segment is assumed to behave as a mass of a single degree of freedom. The SD concept is then applied to each segment to consider the displacement related soil damping instead of the velocity dependent damping. Instrumented strain gauge data at different levels of the shaft are required for the interpretation method. Three case studies are presented in this paper to study the validity and applicability of the present method. The predicted results are also compared to the available test or analytical data. 相似文献
943.
944.
945.
利用算子运算的方法,对求定外空扰动引力的Bjerhammar方法、虚拟点质量方法以及虚拟单层密度方法进行了系统地归纳;利用Possion核的再生特性及球谐函数的正交性质,给出了它们之间的换算关系;最后从两个方面分析了实用计算中各种方法的优劣。 相似文献
946.
947.
GIS中DEM产品精度的分析和评价 总被引:8,自引:1,他引:8
从视觉上和统计上,对3个目前国内主流的GIS软件的DEM产品作了精度分析,给出了其DEM的精度评价结果,对实际生产有一定的参考价值,有助于对软件的DEM产品质量形成一定的认识。 相似文献
948.
949.
950.
Measuring Seismic Waves Induced by Large Earthquakes with GPS 总被引:4,自引:0,他引:4
Independent GPS position solutions at 1-sec interval, derived from the International GPS Service (IGS) data and orbit÷clock products, clearly show seismic waves generated by the magnitude 7.9 Denali Fault, Alaska earthquake of November 3, 2002. Surface seismic waves with periods of about 20 sec and amplitudes of up to 20 cm were detected up to 4,000 km from the epicenter. This confirms the previous findings reported by Larson et al. (2003); we use additional station data along with different processing software and strategies. The seismic waves from the May 26, 2003 magnitude 7.0 Japanese earthquake were also observed in the 1-sec position solution series at station MIZU, about 80 km from the epicenter. This earthquake, however, could not be detected by GPS at station USUD, about 410 km away. Similarly, the Algerian May 21, 2003 earthquake of magnitude 6.8 could not be detected by GPS at the nearest IGS station located approximately 800 km from the epicenter. 相似文献