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161.
The shear viscosities and 1 bar heat capacities of glasses and melts along the 67mol% silica isopleth in the system SiO2-Al2O3-Na2O-TiO2 have been determined in the temperature ranges 780-1140 K and 305-1090 K respectively. Anomalous behaviour of both these properties is observed for compositions rich in TiO2 and/or Al2O3, an observation attributed to liquid-liquid phase separation followed by anatase crystallization. For samples which do not show anomalous behaviour, it is found that the partial molar heat capacity of the TiO2 component previously determined in Al-free compositions reproduces our heat capacities to within 1.3%. Viscosity data show that addition of TiO2 tends to increase viscosity and melt fragility at constant temperature. Furthermore, heat capacity and viscosity data may be combined within the framework of the Adam-Gibbs theory to extract values of the configurational entropy of the liquids and qualitative estimates of the variation of the average energy barrier to viscous flow. Configurational entropy at 900K is inferred to decrease upon addition of TiO2, in contrast to previous results from Al-free systems. The compositional limit separating normal from anomalous behaviour, as well as the data for homogenous melts have been used to constrain the structural role of Ti in these samples. Our data are consistent with a majority of Ti in five-fold coordination associated with a titanyl bond, in agreement with previous spectroscopic studies. Furthermore, we find no evidence for a Ti-Al interaction in our samples, and we are led to the conclusion that Al and Ti are incompletely mixed, a hypothesis consistent with the observed reduction of configurational entropy upon addition of TiO2, suggesting an important role of medium range order in controlling the variations in thermodynamic properties. 相似文献
162.
Regions and sustainable development: regional planning matters 总被引:1,自引:0,他引:1
This paper looks at how the term 'sustainable development' has been used in the process of regional plan making over the past decade. It emphasizes the differing geographies of these debates within England, in terms of how sustainable development has been used to justify different types of approach in different parts of the country. Both drawing on and challenging recent work on state theory, the paper argues the need to see regional planning as a part of a multi-scalar governance system, whose importance should not be underestimated. 相似文献
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基于图论的树状河系结构化绘制模型研究 总被引:5,自引:1,他引:5
结合树状河系自身的结构特点和图论的思想,提出了基于图论的河系结构化绘制模型的建立,利用图论的思想描述了河系的结构并建立其自动符号化模型,阐述了主流、流向自动确定和结构化绘制实现的详细算法,并对通用图形数据格式DXF文件记录的河系数据进行了测试。 相似文献
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The resolution of whole Earth seismic tomographic models 总被引:2,自引:0,他引:2
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Sensitivity kernels for finite-frequency surface waves 总被引:1,自引:1,他引:1