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191.
泥炭地(peatland)是一类储碳效率很高的特殊陆地生态系统,其碳储量约占全球土壤碳库的近1/3,对全球碳循环有着举足轻重的作用。有证据表明在过去20余年,北半球大范围的天然水体中溶解有机碳的浓度呈显著增升趋势。普遍认为与全球变化背景下北方泥炭地大规模释放溶解有机碳有关,但其驱动机制尚不十分清楚。已经提出的具有代表性... 相似文献
192.
中国环境污染源的区域差异及其社会经济影响因素——基于339个地级行政单元截面数据的实证分析 总被引:10,自引:2,他引:10
基于2012年环境污染物排放和社会经济截面数据,选取化学需氧量、二氧化硫及污染源结构指标,定量研究中国339个地级行政单元环境污染源的空间分异和集聚效应,解析环境污染源及排放空间格局的影响因素,并提出污染防控措施与综合治理建议。结果表明:① 环境污染源结构区域差异显著,水环境污染源以农业源主导型、城镇生活源主导型、城镇生活和农业源复合型为主,三者比重分别为35.40%、33.92%和25.66%,农业源主导型排放强度最高,主要分布于华北和东北地区;大气环境污染源以工业源绝对主导型为主,其比重为74.63%,分布于除青藏高原区的广大区域。② 农业源主导使水污染物集聚式排放加剧,工业源主导则促进了大气污染物集聚式排放,特别在环渤海及其经济腹地区域,污染源结构强化了污染物排放的空间集聚效应。③ 人口规模、城镇化水平和经济增长速度是污染物排放的主要驱动因素,其中以人口规模影响最为显著;经济发展水平在区域模型中呈现不同的影响效应,对工业源主导型区域的大气污染物排放呈正向影响,而对城镇生活源主导型区域的水体污染物排放具有抑制作用;工业化程度对工业源绝对主导型区域的大气污染物排放正向影响显著。 相似文献
193.
This paper examines the impact of contrasting antecedent soil moisture conditions on the hydrochemical response, here the changes in dissolved nitrogen (NO3?, NH4+ and dissolved organic nitrogen (DON)) and dissolved organic carbon (DOC) concentrations, of a first‐order stream during hydrological events. The study was performed in the Hermine, a 5 ha forested watershed of the Canadian Shield. It focused on a series of eight precipitation events (spring, summer and fall) sampled every 2 or 3 h and showing contrasted antecedent moisture conditions. The partition of the eight events between two groups (dry or wet) of antecedent moisture conditions was conducted using a principal component analysis (PCA). The partition was controlled (first axis explained 86% of the variability) by the antecedent streamflow, the streamflow to precipitation ratio Q/P and by the antecedent groundwater depth. The mean H+, NO3?, NH4+, total dissolved nitrogen and DOC concentrations and electrical conductivity values in the stream were significantly higher following dry antecedent conditions than after wetter conditions had prevailed in the Hermine, although the temporal variability was high (17 to 138%). At the event scale, a significantly higher proportion of the changes in DON, NO3?, and DOC concentrations in the stream was explained by temporal variations in discharge compared with the seasonal and annual scales. Two of the key hydrochemical features of the dry events were the synchronous changes in DOC and flow and the frequent negative relationships between discharge and NO3?. The DON concentrations were much less responsive than DOC to changes in discharge, whereas NH was not in phase with streamflow. During wet events, the synchronicity between streamflow and DON or NO3? was higher than during dry events and discharge and NO3? were generally positively linked. Based on these observations, the hydrological behaviour of the Hermine is conceptually compatible with a two‐component model of shallow (DON and DOC rich; variable NO3?) and deep (DON and DOC poor; variable NO3?) subsurface flow. The high NO3? and DOC levels measured at the early stages of dry events reflected the contribution from NO3?‐rich groundwaters. The contribution of rapid surface flow on water‐repellent soil materials located close to the stream channel is hypothesized to explain the DOC levels. An understanding of the complex interactions between antecedent soil moisture conditions, the presence of soil nutrients available for leaching and the dynamics of soil water flow paths during storms is essential to explain the fluxes of dissolved nitrogen and carbon in streams of forested watersheds. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
194.
Temporal and spatial variations in the discharge and dissolved organic carbon of drip waters in Beijing Shihua Cave,China 总被引:1,自引:0,他引:1
To detect the causal relationship between cave drip waters and stalagmite laminae, which have been used as a climate change proxy, three drip sites in Beijing Shihua Cave were monitored for discharge and dissolved organic carbon (DOC). Drip discharges and DOC were determined at 0 to 14‐day intervals over the period 2004–2006. Drip discharges show two types of response to surface precipitation variations: (1) a rapid response; and (2) a time‐lagged response. Intra‐annual variability in drip discharge is significantly higher than inter‐annual variability. The content of DOC in all drip waters varies inter‐ and intra‐annually and has good correlation with drip water discharge at the rapid response sites. High DOC was observed in July and August in the three years observed. The flushing of soil organic matter is dependent upon the intensity of rain events. The DOC content of drip water increases sharply above a threshold rainfall intensity (>50 mm d?1) and shows several pulses corresponding with intense rain events (>25 mm d?1). The DOC content was lower and less variable during the dry period than during the rainy period. The shape of DOC peak also varies from year to year as it is influenced by the intensity and frequency of rainfall. The different drip sites show marked differences in DOC response, which are dominated by hydrological behaviour linked to the recharge of the soil and karst micro‐fissure/porosity network. The results explain why not all stalagmite laminae are consistent with climate changes and suggest that the structure of the rainy season events could be preserved in speleothems. Copyright © 2008 John Wiley & Sons, Ltd. 相似文献
195.
Preliminary study on the dissolved and colloidal organic carbon in the Zhujiang River estuary 总被引:3,自引:0,他引:3
INTRODUCTIONEstuariescompriseamajorbiogeochemicalinterfaceconnectingthelandandthesea (Man toura,1 987) .Thebehaviorandfateofaparticularriver bornesubstanceintroducedintoanestuaryisdeterminedtoalargeextentbythebiogeochemicalpropertiesofthesubstanceaswellasp… 相似文献
196.
A VERTICAL DISTRIBUTION MODEL OF NUTRIENTS AND DISSOLVED OXYGEN IN THE SOUTHERN TAIWAN STRAIT 总被引:3,自引:0,他引:3
Sinoe vertical transport of nutrients and dissolved oxygen are quite important in the water col-umn and have drawn serious attention these recent years, a one-dmension numerical model is tried to simulate the vertical distribution of nutrients and dissolved oxygen in June at two research sites in the southemTaiwan Strait. Physical transport parameters are calibrated by temperature simulation, and thenare used to simulate the profiles of NO_3, PO_4 and dissolved oxygen. The simulation was generally success-ful for both stations. The importance of various factors, such as upwelling tidal current andbiogeochemical activities, which influence the vertical distribution of nutrients and dissolved oxygen, is revealed by analysis of the modeling results. Some important rates, fluxes and ratios are also estimated anddiscussed on the basis of simulation. 相似文献
197.
A Lagrangian tracer model is set up for Hangzhou Bay based on Coupled Hydrodynamical Ecological model for Regional Shelf Sea
(COHERENS). The study area is divided into eight subdomains to identify the dominant physical processes, and the studied periods
are March (the dry season) and July (the wet season). The model performance has been first verified by sea-surface elevation
and tidal current observations at several stations. Eight tracer experiments are designed and Lagrangian particle tracking
is simulated to examine the impact of physical processes (tide, wind and river runoff) on the transport of passive tracer
released within the surface layer. Numerical simulations and analysis indicate that: (1) wind does not change the tracer distribution
after 30 days except for those released from the south area of the bay during the wet season; (2) the tide and the Qiantang
River runoff are important for particle transport in the head area of the bay; (3) the Changjiang River runoff affects the
tracer transport at the mouth of the bay, and its impact is smaller in the dry season than in the wet season.
Supported by the Natural Science Foundation of China (No.40576080); National High Technology Research and Development Program
of China (863 Program, No. 2007AA12Z182) 相似文献
198.
199.
200.
An Overview of Dissolved and Suspended Matter Fluxes in the Loire River Basin: Natural and Anthropogenic Inputs 总被引:7,自引:0,他引:7
Cécile Grosbois Philippe Négrel Daniel Grimaud Christian Fouillac 《Aquatic Geochemistry》2001,7(2):81-105
The spatial and temporal distributions of major elements were investigated in the surface waters and in associated suspended matter at two sites of the upper Loire basin (Orleans and Brehemont) between 1995 and 1998.According to geochemical and isotopic patterns, the dissolved load appears to result from a process of mixing rainwater inputs, weathering processes of carbonate and silicate bedrock, and agricultural and urban inputs. Natural inputs influence 60% of water chemical composition at both sites. Annual dissolved fluxes were estimated to be 1300 103 t/y at Orleans and 1620 103 t/y at Brehemont. Major elements are transported mainly in the dissolved fraction. After correcting for atmospheric and anthropogenic inputs, the silicate specific export rate was calculated to be 11 t/y/km2 throughout the basin and the carbonate specific export rate to be from 47 t/y/km2 at Orleans to 23 t/y/km2 at Brehemont.The suspended load appears to result from at least two particle reservoirs: a silicate reservoir and a carbonate reservoir. The silicate reservoir has a detrital origin, mainly during periods of high flow, while the carbonate reservoir has a detrital origin during periods of high flow and an authigenic origin during periods of low flow. Of the total annual flow of suspended matter, this authigenic material represents 16% at Orleans, 25% at Brehemont and 37% in the fluvial part of the estuary. After correcting authigenic inputs, the specific export rate due to mechanical weathering was estimated to be 8 t/y/km2 throughout the Loire basin. 相似文献