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91.
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93.
G. P. Ayers R. W. Gillett J. M Cainey A. L. Dick 《Journal of Atmospheric Chemistry》1999,33(3):299-319
Datasets on aerosol composition in Southern Ocean air at Cape Grim and Macquarie Island, and rainwater composition at Cape Grim, have been analysed for sea-salt components in order to test the validity of the multiphase autocatalytic halogen activation process proposed initially by Sander and Crutzen (1996) and developed fully for clean marine air by Vogt et al. (1996). Four distinct datasets from the two locations were analysed. All four datasets provided consistent evidence in support of three predictions of the autocatalytic model: (1) overall Cl- deficits in sea-salt aerosol were small, difficult to quantify against analytical uncertainty and at most a few percent; (2) Br- deficits were large, averaging –30% to –50% on an annual basis, with strong seasonality ranging from about –10% in some winter samples to –80% or more in some summer samples; and (3) the Br- and Cl- deficits were clearly linked to the availability of strong, S-acidity in the aerosol, confirming the importance of acid catalysis to the dehalogenation process. 相似文献
94.
The aim of the study is to investigate the interaction between waters of Lake Girdev and groundwater in the allochthonous
limestone units exposed in the area between Lake Girdev and Kazanpınarı Spring, southwestern Turkey. The features analyzed
include the flow direction and apparent groundwater velocity, their relationship with Lake Girdev, and the effect of lithological
and structural features on the groundwater circulation. The results of a fluorescein tracer test indicate that groundwater
flows east-northeast and the apparent flow velocity ranges from 26.2 to 35.6 m h–1 between the injection site and various observation points. Tritium data suggest that the water of Lake Girdev and groundwater
are probably similar in age, and oxygen-18 isotope data indicate that water derived from Lake Girdev is the main source of
recharge to the aquifer. The aquifer is fed not only by Lake Girdev but also by rainfall percolating through allochthonous
limestones; together, these provide the discharge of springs in Elmalı Polje. The permeability of the allochthonous limestone
aquifer has been enhanced as a result of jointing and faulting.
Received, June 1997 / Revised, June 1998, March 1999 / Accepted, July 1999 相似文献
95.
DNA tracers with information capacity and high detection sensitivity tested in groundwater studies 总被引:1,自引:0,他引:1
In order to investigate the usefulness of unique synthetic DNA tracers in groundwater, a field experiment was conducted in
Norway. DNA tracers and a sodium-chloride tracer were injected into an aquifer. The transport of DNA molecules was interpreted
by comparing with the plume of chloride ions under forced-gradient steady-state flow conditions. Spatial concentration moments
described the migration of conservative tracers. Mobility and migration of DNA in groundwater demonstrate that DNA tracers
can be detected by using the polymerase chain reaction (PCR) and DNA sequence analysis. The results indicate that DNA tracers
can be valuable tools as tracers in groundwater investigations.
Received, June 1997 / Revised, July 1998, December 1998 / Accepted, January 1999 相似文献
96.
Determining concentration fields of tracer plumes for layered porous media in flow-tank experiments 总被引:1,自引:0,他引:1
In the laboratory, computer-assisted image analysis provides an accurate and efficient way to monitor tracer experiments.
This paper describes the determination of detailed temporal concentration distributions of tracers in a flow-tank experiment
by analyzing photographs of plumes of Rhodamine dye through the glass wall of the tank. The methodology developed for this
purpose consists of four steps: (1) digitally scanning black and white negatives obtained from photographs of the flow–tank
experiment; (2) calibrating and normalizing each digitized image to a standard optical-density scale by determining the relation
between the optical density and pixel value for each image; (3) constructing standard curves relating the concentration in
an optical density from five experimental runs with predetermined concentrations (2–97 mg/L); and (4) converting the optical
density to concentration. The spatial distribution of concentration for two photographs was determined by applying these calibration
and conversion procedures to all pixels of the digitized images. This approach provides an efficient way to study patterns
of plume evolution and transport mechanisms.
Received, March 1998 Revised, September 1998 Accepted, October 1998 相似文献
97.
Danyang Li Minfang Zheng Yusheng Qiu Limin Lai Nengwang Chen Hongmei Jing Run Zhang Min Chen 《海洋学报(英文版)》2023,42(1):75-82
Nitrogen fixation is one of the most important sources of new nitrogen in the ocean and thus profoundly affects the nitrogen and carbon biogeochemical processes. The distribution, controlling factors, and flux of N2 fixation in the global ocean remain uncertain, partly because of the lack of methodological uniformity. The 15N2 tracer assay (the original bubble method → the 15N2-enriched seawater method → the modified bubble method) is the mainstream method for field measurements of N2 fixation rates (NFRs), among which the original bubble method is the most frequently used. However, accumulating evidence has suggested an underestimation of NFRs when using this method. To improve the availability of previous data, we compared NFRs measured by three 15N2 tracer assays in the South China Sea. Our results indicate that the relationship between NFRs measured by the original bubble method and the 15N2-enriched seawater method varies obviously with area and season, which may be influenced by incubation time, diazotrophic composition, and environmental factors. In comparison, the relationship between NFRs measured by the original bubble method and the modified bubble method is more stable, indicating that the N2 fixation rates based on the original bubble methods may be underestimated by approximately 50%. Based on this result, we revised the flux of N2 fixation in the South China Sea to 40 mmol/(m2·a). Our results improve the availability and comparability of literature NFR data in the South China Sea. The comparison of the 15N2 tracer assay for NFRs measurements on a larger scale is urgently necessary over the global ocean for a more robust understanding of the role of N2 fixation in the marine nitrogen cycle. 相似文献
98.
Shin Giek Goh Stéphane Bayen David Burger Barry C. Kelly Ping Han Vladan Babovic Karina Yew-Hoong Gin 《Marine pollution bulletin》2017,114(1):627-634
Water quality in Singapore's coastal area was evaluated with microbial indicators, pathogenic vibrios, chemical tracers and physico-chemical parameters. Sampling sites were grouped into two clusters (coastal sites at (i) northern and (ii) southern part of Singapore). The coastal sites located at northern part of Singapore along the Johor Straits exhibited greater pollution. Principal component analysis revealed that sampling sites at Johor Straits have greater loading on carbamazepine, while turbidity poses greater influence on sampling sites at Singapore Straits. Detection of pathogenic vibrios was also more prominent at Johor Straits than the Singapore Straits. This study examined the spatial variations in Singapore's coastal water quality and provided the baseline information for health risk assessment and future pollution management. 相似文献
99.
Mesocosm experiments identifying hotspots of groundwater upwelling in a water column by fibre optic distributed temperature sensing
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Amaya Irene Marruedo Arricibita Stefan Krause Jesus Gomez‐Velez David M. Hannah Jörg Lewandowski 《水文研究》2018,32(2):185-199
Lacustrine groundwater discharge (LGD) can substantially impact ecosystem characteristics and functions. Fibre optic distributed temperature sensing (FO‐DTS) has been successfully used to locate groundwater discharge into lakes and rivers at the sediment–water interface, but locating groundwater discharge would be easier if it could be detected from the more accessible water surface. So far, it is not clear if how and under which conditions the LGD signal propagates through the water column to the water surface–atmosphere interface, and what perturbations and signal losses occur along this pathway. In the present study, LGD was simulated in a mesocosm experiment. Under winter conditions, water with temperatures of 14 to 16 °C was discharged at the bottom of a 10 × 2.8‐m mesocosm. Water within this mesocosm ranged from 4.0 to 7.4 °C. Four layers (20, 40, 60, and 80 cm above the sediment) of the 82 cm deep mesocosm were equipped with FO‐DTS for tracing thermal patterns in the mesocosm. Aims are (a) to test whether the positive buoyancy of relatively warm groundwater imported by LGD into shallow water bodies allows detection of LGD at the lake's water surface–atmosphere interface by FO‐DTS, (b) to analyse the propagation of the temperature signal from the sediment‐water interface through the water column, and (c) to learn more about detectability of the signal under different discharge rates and weather conditions. The experiments supported the benchmarking of scale dependencies and robustness of FO‐DTS applications for measuring upwelling into aquatic environments and revealed that weather conditions can have important impacts on the detection of upwelling at water surface–atmosphere interfaces at larger scales. 相似文献
100.
Spatio‐temporal tracer variability in the glacier melt end‐member — How does it affect hydrograph separation results?
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Geochemical and isotopic tracers were often used in mixing models to estimate glacier melt contributions to streamflow, whereas the spatio‐temporal variability in the glacier melt tracer signature and its influence on tracer‐based hydrograph separation results received less attention. We present novel tracer data from a high‐elevation catchment (17 km2, glacierized area: 34%) in the Oetztal Alps (Austria) and investigated the spatial, as well as the subdaily to monthly tracer variability of supraglacial meltwater and the temporal tracer variability of winter baseflow to infer groundwater dynamics. The streamflow tracer variability during winter baseflow conditions was small, and the glacier melt tracer variation was higher, especially at the end of the ablation period. We applied a three‐component mixing model with electrical conductivity and oxygen‐18. Hydrograph separation (groundwater, glacier melt, and rain) was performed for 6 single glacier melt‐induced days (i.e., 6 events) during the ablation period 2016 (July to September). Median fractions (±uncertainty) of groundwater, glacier melt, and rain for the events were estimated at 49±2%, 35±11%, and 16±11%, respectively. Minimum and maximum glacier melt fractions at the subdaily scale ranged between 2±5% and 76±11%, respectively. A sensitivity analysis showed that the intraseasonal glacier melt tracer variability had a marked effect on the estimated glacier melt contribution during events with large glacier melt fractions of streamflow. Intra‐daily and spatial variation of the glacier melt tracer signature played a negligible role in applying the mixing model. The results of this study (a) show the necessity to apply a multiple sampling approach in order to characterize the glacier melt end‐member and (b) reveal the importance of groundwater and rainfall–runoff dynamics in catchments with a glacial flow regime. 相似文献