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181.
Photoluminescence (PL) spectra of Si nanocrystals (NCs) prepared by 130 keV Si ions implantation onto SiO2 matrix were investigated as a function of annealing temperature and implanted ion dose. PL spectra consist of two PL peaks, originated from smaller Si NCs due to quantum confinement effect (QCE) and the interface states located at the surface of larger Si NCs. The evolution of number of dangling bonds (DBs) on Si NCs was also investigated. For hydrogen-passivated samples, a monotonic increase in PL peak intensity with the dose of implanted Si ions up to 3× 1017 ions /cm2 is observed. The number of DBs on individual Si NC, the interaction between DBs at the surface of neighbouring Si NCs and their effects on the efficiency of PL are discussed. 相似文献
182.
This paper reports that vibrational spectroscopic analysis on hydrogen-bonding between acetone and water comprises both experimental Raman spectra and ab initio calculations on structures of various acetone/water complexes with changing water concentrations. The optimised geometries and wavenumbers of the neat acetone molecule and its complexes are calculated by using ab initio method at the MP2 level with 6-311+G(d,p) basis set. Changes in wavenumber position and linewidth (fullwidth at half maximum) have been explained for neat as well as binary mixtures with different mole fractions of the reference system, acetone, in terms of intermolecular hydrogen bonding. The combination of experimental Raman data with ab initio calculation leads to a better knowledge of the concentration dependent changes in the spectral features in terms of hydrogen bonding. 相似文献
183.
We have studied the temporal bond polarisabilities of para-nitroaniline from the Raman intensities by the algorithm proposed by Wu et al. in 1987 (Tian B, Wu G, Liu G 1987 J. Chem. Phys. 87 7300). The bond polarisabilities provide much information concerning the electronic structure of the non-resonant Raman excited virtual state. At the initial moment by the 514.5 nm excitation, the tendency of the excited electrons (mapped out by the bond polarisabilities) is to spread to the molecular periphery, and the electronic structure of the Raman virtual state is close to the pseudo-quinonoidic state. When the final stage of relaxation is approached, the bond polarisabilities of those peripheral bonds relax faster than those closer to the molecular core, the phenyl ring. The molecule is in the benzenoidic form as demonstrated by the bond polarisabilities after relaxation. 相似文献
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鉴于新疆地区对中国乃至中亚有着特殊的战略意义,本文针对不同数据源及分类系统在土地覆被数据的空间分布上缺乏互通性问题,结合2010年目视解译土地利用现状遥感监测数据、GlobeLand30和GlobCover2009共3种土地覆被数据,采用类型相似分析、类型混淆分析、混淆矩阵分析、空间一致性分析4种方法开展精度评价及一致性分析,以期对土地覆被数据在中国西北干旱区的适用性及适用范围提供有效建议。结果表明,3种土地覆被数据对新疆地区土地覆被类型构成基本一致,且对裸地类型的辨识度最高;新疆地区中高度一致区域占新疆总面积的95%;3种数据两两对比时,总体精度在64.11%~72.57%之间,其中目视解译数据/GlobeLand 30组合表现出最高水平,且仍有提高空间,反映出目前相同卫星传感器是提升精度评价结果的重要因素之一,且不同分类系统、分类方法、空间分辨率及卫星过境时间等因素对精度评价结果也会产生巨大影响。为解决此类问题,利用多源土地覆被遥感数据的融合技术提高数据精度,或是利用深度学习对遥感影像资料进行精确地解译和判读,将是今后全球土地覆被制图及应用领域的主要发展趋势。 相似文献
187.
Multivariate analysis of fluorescence and source identification of dissolved organic matter in Jiaozhou Bay, China 总被引:1,自引:0,他引:1
Hierarchical clustering analysis and principal component analysis (PCA) methods were used to assess the similarities and dissimilarities of the entire Excitation-emission matrix spectroscopy (EEMs) data sets of samples collected from Jiaozhou Bay, China. The results demonstrate that multivariate analysis facilitates the complex data treatment and spectral sorting processes, and also enhances the probability to reveal otherwise hidden information concerning the chemical characteristics of the dissolved organic matter (DOM). The distribution of different water samples as revealed by multivariate results has been used to track the movement of DOM material in the study area, and the interpretation is supported by the results obtained from the numerical simulation model of substance tracing technique, which show that the substance discharged by Haibo River can be distributed in Jiaozhou Bay. 相似文献
188.
The offshore jacket platform is a complex and time-varying nonlinear system,which can be excited of harmful vibration by external loads.It is difficult to obtain an ideal control performance for passive control methods or traditional active control methods based on accurate mathematic model.In this paper,an adaptive inverse control method is proposed on the basis of novel rough neural networks (RNN) to control the harmful vibration of the offshore jacket platform,and the offshore jacket platform model is established by dynamic stiffness matrix (DSM) method.Benefited from the nonlinear processing ability of the neural networks and data interpretation ability of the rough set theory,RNN is utilized to identify the predictive inverse model of the offshore jacket platform system.Then the identified model is used as the adaptive predictive inverse controller to control the harmful vibration caused by wave and wind loads,and to deal with the delay problem caused by signal transmission in the control process.The numerical results show that the constructed novel RNN has advantages such as clear structure,fast training speed and strong error-tolerance ability,and the proposed method based on RNN can effectively control the harmfid vibration of the offshore jacket platform. 相似文献
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近景摄影测量是实现地面目标高精度三维建模的主要方法之一。实际摄影测量过程中,普通数字摄像机在拍摄与镜头距离不同的多个目标时,无法同时聚焦到所有目标而使近景影像各处都清晰。本文以不同聚焦点近景影像的融合为研究内容,以图像一层小波分解的高频系数能量为影像清晰度衡量指标。通过计算小波影像能量,将整幅影像划分为清晰区域、模糊区域及二者的交界区域。对于清晰区域和模糊区域,将清晰区域的像元值直接应用于融合影像,而对于二者的交界区域,将curvelet变换所得初始融合影像的像元值应用于对应位置处的融合影像,从而得到融合影像。最后,用两组实例数据对融合方法进行了验证,并采用信息熵、均方根误差和峰值信噪比三种客观评价准则,对所得融合影像进行定量分析。 相似文献