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21.
The early diagenesis of trace elements (V, Cr, Co, Cu, Zn, As, Cd, Ba, U) in anoxic sediments of the Achterwasser, a shallow lagoon in the non-tidal Oder estuary in the Baltic Sea, was investigated in the context of pyrite formation. The dissolved major redox parameters show a two-tier distribution with transient signals in the occasionally re-suspended fluid mud layer (FM) and a permanently established diagenetic sequence in the sediment below. Intense microbial respiration leads to rapid depletion of O2 within the uppermost mm of the FM. The reduction zones of Mn, Fe and sulfate overlap in the FM and in the permanently anoxic sediment section which appears to be a typical feature of estuarine sediments, under low-sulfate conditions. Degrees of pyritization (DOP) range from 50% in the FM to remarkably high values > 90% at 50 cm depth. Pyrite formation at the sediment surface is attributed to the reaction of Fe-monosulfides with intermediate sulfur species via the polysulfide pathway. By contrast, intense pyritization in the permanently anoxic sediment below is attributed to mineral growth via adsorption of aqueous Fe-sulfide complexes onto pyrite crystals which had originally formed in the surface layer.The studied trace elements show differential behavior patterns which are closely coupled to the diagenetic processes described above: (i) Zn, Cu and Cd are liberated from organic matter in the thin oxic layer of the sediment and diffuse both upwards across the sediment/water boundary and downwards to be trapped as monosulfides, (ii) V, Cr, Co and As are released during reductive dissolution of Mn- and Fe-oxyhydroxides, (iii) U removal from pore water occurs concomitantly to Fe reduction in the FM and is attributed to reduction of U(VI) to U(IV), (iv) the Ba distribution is controlled by reductive dissolution of authigenic barite in the sulfate reduction zone coupled with upward diffusion and re-precipitation. The incorporation of trace elements into pyrite is most intense for Co, Mn and As, intermediate for Cu and Cr and little to negligible for U, Zn, Cd, V and Ba. The observed trend is largely in agreement with previous studies and may be explained with differing rates for ligand exchange. Slow and fast ligand exchange and thus precipitation kinetics are also displayed by downcore increasing (Mn, Cr, Co and As) or constantly low (Zn, Cu, Cd) pore water concentrations. The downward increasing degrees of trace metal pyritization (DTMP) for Co, Cu, Zn and As are, in analogy to pyrite growth, assigned to adsorption of sulfide complexes or As oxyanions onto preexisting pyrite minerals. 相似文献
22.
23.
根据1987年6,8,11月和1988年2月4个航次珠江口伶汀洋的调查资料,分析了溶解氧的特征。结果表明:溶解氧含量表层均高于底层,周年变化呈现从夏季到冬季逐渐上升,且明显受珠江径流的影响,溶解氧(基本上是不饱和状态)与盐度成负相关。有机物和营养盐均影响溶解氧,但水温仍为溶解氧主要影响因素。 相似文献
24.
海沧邻近海域表层沉积物中重矿物研究 总被引:3,自引:0,他引:3
对厦门海沧邻近海域表层沉积物中的重矿物(0.063~0.125mm粒级)进行了分析和研究,结果表明该粒级的重矿物共计49种,其优势和特征矿物为磁铁矿、赤铁矿、褐铁矿、绿帘石、铁铁矿、角闪石、锆石、红柱石等;重矿物的平均质量分数为9.56%;根据重矿物的分布和含量,并结合主要标志矿物的颗粒百分含量和分布特征,将该海域划分为5个矿物组合区,根据各区的矿物组合类型分析了该海域的物质来源及影响重矿物分布和组合的因素,进而探讨了九龙江河口湾和厦门西港海湾的沉积环境。 相似文献
25.
大亚湾海域锥状斯氏藻赤潮及其与孢囊的关系 总被引:22,自引:0,他引:22
用沉积物捕捉器取样,研究了大亚湾海域2000年6~9月孢囊(Cyst)种群动态,同时 分析了浮游植物种群动态。研究期间(8~9月)该海域发生了一起大规模的锥状斯氏藻赤潮。 赤潮前一个月,锥状斯氏藻孢囊的平均日形成率为2.05× 105cysts/(m2·d),丰度为50.22%, 该时期以有性生殖产生的静止期孢囊为主;在赤潮盛期的8,9月初,孢囊的平均日形成率达到 2.01 ×106cysts/(m2·d),丰度为96.97%,此时期的孢囊多为营养细胞所形成的暂时性孢囊; 赤潮结束后,由于环境条件的恶化,暂时性孢囊的形成达到高峰,平均日形成率为1.24×l07 cysts/( m2·d),丰度为99.53%。结果表明大亚湾丰富的孢囊是潜在的种源(Seed bed),2000年 的夏季、秋李持续高温(>25℃),台风减少及风力减弱等有利锥状斯氏藻的环境条件诱发孢 囊萌发,开始了该种类的赤潮。 相似文献
26.
Modelling nitrogen and phosphorus cycles and dissolved oxygen in the Zhujiang Estuary Ⅰ. Model development 总被引:1,自引:0,他引:1
wrmcrloxHuman activities related to the population growth and developrnent of industry and rnwhci-pality have led to the incrouing hadings of various POllutants into estudries during the past fewdecades. These increasing edlutant lOadings have caused declined estuallne hedth which can bemereured by a vdriety of indices. In order to obtain solutions to environrnent problerns, re-sources manageTnnt apencies are supporting a holistic approach to envirorirnental management.An effcient strategy t… 相似文献
27.
Predation by the big brackish-water isopod Saduria entomon on two age-classes (juveniles and adults) of the small deposit-feeding amphipod Monoporeia (syn. Pontoporeia) affinis was studied at different oxygen conditions (normoxia>11 mg/l O2, and moderate hypoxia 4 mg/l O2). Vulnerability of juvenile and adult M. affinis was studied in single and mixed age-class treatments. The proportions of juveniles and adults were varied at one total numerical density. The predatory effects were measured as numbers of individuals consumed and of total biomass intake (mg ash-free dry weight). The highest predation rate (in numbers) was detected in the single-prey treatment with juvenile M. affinis, both in normoxia and moderate hypoxia. No preference for any of the two size classes was found in the treatment with equal numbers of adults and juveniles. In normoxia, the total number of prey consumed decreased with increasing proportions of adults, while intake increased in terms of biomass. In moderate hypoxia, high proportions of adults reduced the predation rate of S. entomon to such an extent that also the intake in terms of biomass was significantly negatively affected. 相似文献
28.
台湾海峡中北部夏季溶解氧饱和度分布与上升流的关系 总被引:1,自引:1,他引:1
本文据台湾海峡中北部1983年5月至1984年5月、1987年7,8月和1988年5~7月调查资料,讨论了该海域夏季溶解氧饱和度分布特征及其与上升流的关系,结果表明该海区夏季上升流的中心位置经常出现于海坛岛北侧至湄洲岛一带海域,西南季风是该区上升流产生的主要动力因子,该区上升流平均流速为4.4×10~(-3)cm/s。 相似文献
29.
本文对菊花岛海区沉积物类型,重矿物和粘土矿物组合分区及其分布特征进行了分析,同时对测区沉积物来源进行探讨。 相似文献
30.