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21.
Fariborz Goodarzi Hamed Sanei 《中国地球化学学报》2006,25(B08):47-48
Particles, less than PM10 in size, emitted from the stack of pulverized coal-fired power plants are of environmental concern since they can easily enter the human respiratory track. These fine particles are examined by Scanning Electron Microscope/Electron Dispersive Spectrometry (SEM/EDX). Plerospheres are found in fly ash and are particles containing smaller particles formed during combustion of coal. The large plerospheres 〉50 μm mostly are present in ESP fly ash, indicating that they are effectively capturing fine particles and reducing their stack emission. 相似文献
22.
Xinghui XIA 《中国地球化学学报》2006,25(B08):263-263
Photodegradation of chrysene, benzo (a) pyrene and benzo (g, h, i) perylene in natural water of the Yellow River was studied using simulation sunlight. The effects of particulates on the photodegradation were explored. Several results arose from this study. (1) The photodegradation of PAHs can be fitted with first-order kinetics when no particulate exists in water system, and the first-order constant increases with decreasing of initial concentration of PAHs. The photodegradation rates of the three PAHs are related to their molecule absorption spectrum. (2) The existence of loess exerts two kinds of effects on the photodegradation of PAHs, including the inner filter effects and the photosensitizing effects of humic substance in loess. These two contrary effects lead to the difference of net effects among different contents of loess. When the loess contents are 0.1 and 5.0 g/L, the existence of loess stimulates the photodegradation of chrysene, benzo (a) pyrene. When the loess content is 5.0 g/L, the existence of loess stimulates the photodegradation of benzo (g, h, i) perylene. In addition, the photodegradation of PAHs can be fitted with the second-order kinetics when there is loess in the water system. (3) The soluble humic substances in loess can accelerate the photodegradation of PAHs while the in soluble part cannot. (4) Since the soluble humic substances in the suspended solids of the river have been dissolved in water, 相似文献
23.
大气CO2浓度升高对土壤中不同粒级碳的影响 总被引:4,自引:0,他引:4
不同粒级土壤中的碳有着不同的周转规律,在高CO2浓度条件下,它们含量的变化将在一定程度上反映土壤碳是累积还是减少,对明确土壤碳的变化趋势有重要意义.采用田间培养试验初步模拟研究在高CO2浓度条件下土壤不同粒级碳的分布.结果表明,加入秸秆培养1年,由于CO2浓度升高的原因导致在低氮(LN)、常规氮(NN)和高氮(HN)水平下土壤中碳分别增加0.01、1.10、1.22g/kg,表现为粒级〈53μm土壤颗粒中碳分别增加1.53、2.19、2.70g/kg.粒级〈53μmm土壤颗粒碳量的增加,主要是由于其重量分配百分数显著增加36.2%,碳浓度增加5.4%;粒级〉250μm和250~53μm土壤颗粒部分虽然其碳浓度分别增加20.8%和17.3%(P〈0.05),怛由于重量分配百分数分别显著降低22.8%和36.1%,结果碳量降低.试验表明高CO2浓度导致不同粒级土壤的分配及碳浓度的变化;高氮施肥水平下有增加土壤碳量特别是小粒级土壤碳量的趋势. 相似文献
24.
A. Ankilov A. Baklanov M. Colhoun K. -H. Enderle J. Gras Yu. Julanov D. Kaller A. Lindner A. A. Lushnikov R. Mavliev F. McGovern T. C. O'Connor J. Podzimek O. Preining G. P. Reischl R. Rudolf G. J. Sem W. W. Szymanski A. E. Vrtala P. E. Wagner W. Winklmayr V. Zagaynov 《Atmospheric Research》2002,62(3-4)
During an international workshop at the Institute for Experimental Physics of the University of Vienna, Austria, which was coordinated within the Committee on Nucleation and Atmospheric Aerosols (IAMAS-IUGG), 10 instruments for aerosol number concentration measurement were studied, covering a wide range of methods based on various different measuring principles. In order to investigate the detection limits of the instruments considered with respect to particle size, simultaneous number concentration measurements were performed for monodispersed aerosols with particle sizes ranging from 1.5 to 50 nm diameter and various compositions.The instruments considered show quite different response characteristics, apparently related to the different vapors used in the various counters to enlarge the particles to an optically detectable size. A strong dependence of the 50% cutoff diameter on the particle composition in correlation with the type of vapor used in the specific instrument was found. An enhanced detection efficiency for ultrafine hygroscopic sodium chloride aerosols was observed with water operated systems, an analogous trend was found for n-butanol operated systems with nonhygroscopic silver and tungsten oxide particles. 相似文献
25.
银川市初夏气溶胶粒子谱分布特征 总被引:4,自引:5,他引:4
利用美制APS—3310A型激光粒谱仪,在中国西北城市银川对大气气溶胶粒子进行现场观测,结合气象条件,并通过理论计算分析,给出了银川市初夏大气气溶胶的日变化特征、3种不同粒径粒子分布特点及飘尘谱分布特征,以期为银川市大气污染总量控制方案及对策提供科学依据。 相似文献
26.
粘粒含量对南京粉细砂液化影响的试验研究 总被引:16,自引:1,他引:16
南京粉细砂是一种以片状颗粒成分为主的粉细砂,与通常的圆形颗粒石英砂有一定区别,片状颗粒成分使得南京粉细砂具有各向异性的性质。通过对不同粘粒含量的南京粉细砂进行液化试验,分析其试验结果发现:对于粘粒含量ρc=5%、10%和15%三种情况,在均压固结情况下,当南京粉细砂达到初始液化时,采用变形标准和孔压标准是一致的;而偏压固结时,只能采用变形标准作为南京粉细砂达到初始液化的标准,此时振动孔压仅达到围压的50%-70%。粘粒含量对南京粉细砂的抗液化强度影响很大,随粘粒含量增加,在不同固结比时,其抗液化强度并不是单调变化,而是在粘粒含量ρc=10%左右处于一个低谷,其抗液化强度最低。 相似文献
27.
We compare flux and concentration footprint estimates of athree-dimensional Lagrangian stochastic dispersion modelapplying backward trajectories with the results of ananalytical footprint model by Kormann and Meixner.The comparison is performed for varying stability regimesof the surface layer as well as for different measurementheights. In general, excellent correspondence is found. 相似文献
28.
铂族元素迁移富集机理的新探 总被引:2,自引:1,他引:2
在岩浆及高温热液中,拍族元素以纳米液态铂族元素单质、铂族元素与其它金属元素的纳米液态合金、纳米液态铂族元素的硫、砷化物迁移。在中、低温热液及表生条件下,除呈上述固态纳米铂族矿物随流体迁移外,还呈配合物形式迁移。然后它们在合适的条件下沉淀富集形成矿床。此外,还讨论了铂族元素与金地球化学条件的异同。 相似文献
29.
Frédérick Delay Hélène Housset-Resche Gilles Porel Ghislain de Marsily 《Mathematical Geology》1996,28(1):45-71
A new method for solving the transport equation based on the management of a large numbe of particles in a discretized 2-D domain is presented. The method uses numerical variables to represent the number of particles in a given mesh and is more complex than the 1-D problem. The first part of the paper focuses on the specific management of particles in a 2-D problem. The method also would be valid for three dimensions as long as the medium can be modeled similar to a layered system. As the particles are no longer tracked individually, the algorithm is fast and does not depend on the number of particles present. The numerical tests show that the method is nearly numerical dispersion free and permits accurate calculations even for simulations of low-concentration transport. Because each mesh is considered as a closed system between two successive time steps, it is easy to add adsorption phenomenon without any problem of numerical stability. The model is tested under conditions that are extremely demanding for its operating mode and gives a good fit to analytical solutions. The conditions in which it can be used to best advantage are discussed. 相似文献
30.
The application of X-ray photoelectron spectroscopy (XPS) to coal surface characterisation for preparation research is described. Progress towards the acquisition of complementary surface chemical information by time-of-flight secondary ion mass spectrometry (ToF-SIMS) is also discussed. Surface-based beneficiation techniques such as flotation are assuming greater importance as the proportion of fines in raw coal increases due to the proliferation of high capacity mining methods. A necessary condition for the floatability of a coal particle is adequate hydrophobicity, and the degree of hydrophobicity of the flotation concentrate is one factor influencing the ease with which its dewatering can be affected. The hydrophobicity of a coal is very difficult to measure directly because of microporosity, and it is often necessary to deduce the degree of hydrophobicity from a knowledge of the surface chemistry. XPS is able to provide sufficient analytical data to allow relative levels of hydrophobicity to be estimated. In principle, ToF-SIMS should be able to supply additional information enabling refinement of such estimates; however, there are insufficient data at present to allow the ionic fragments detected to be related to specific functional groups at the coal surface. 相似文献