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1.
The kinetics of the reactions of C2H radical with ethane (k1), propane (k2), and n-butane (k3) are studied over the temperature range of T = 96-296 K with a pulsed Laval nozzle apparatus that utilizes a pulsed laser photolysis-chemiluminescence technique. The C2H decay profiles in the presence of both the alkane reactant and O2 are monitored by the CH(A2Δ) chemiluminescence tracer method. The results, together with available literature data, yield the following Arrhenius expressions: k1(T) = (0.51 ± 0.06) × 10−10 exp[(−76 ± 30)K/T] cm3 molecule−1 s−1 (T = 96-800 K), k2(T) = (0.98 ± 0.32) × 10−10exp[(−71 ± 60)K/T] cm3 molecule−1 s−1 (T = 96-361 K), and k3(T) = (1.23 ± 0.26) × 10−10 cm3 molecule−1 s−1 (T = 96-297 K). At T = 296 K, k1 is measured as a function of total pressure and has little or no pressure dependence. The results from this work support a direct hydrogen abstraction mechanism for the title reactions. Implications to the atmospheric chemistry of Titan are discussed. 相似文献
2.
Tidal effects on temperature front in the Yellow Sea 总被引:5,自引:0,他引:5
Temperature front (TF) is one of the important features in the Yellow Sea, which forms in spring, thrives in summer, and fades
in autumn as thermocline declines. TF intensity ⋎S
T
⋎ is defined to describe the distribution of TF. Based on the MASNUM wave-tide-circulation coupled model, temperature distribution
in the Yellow Sea was simulated with and without tidal effects. Along 36°N, distribution of TF from the simulated results
are compared with the observations, and a quantitative analysis is introduced to evaluate the tidal effects on the forming
and maintaining processes of the TF. Tidal mixing and the circulation structure adapting to it are the main causes of the
TF.
Supported by the National Basic Research Program of China (No. G1999043809) and the National Science Foundation of China (No.
49736190). 相似文献
3.
Jonathan S. Price 《水文研究》1994,8(2):167-177
Over an oceanic peatland, the concentration of Na in fog averaged 38.1 mgl?1 compared with 1.8 mgl?1 in rain, resulting in a significant flux of mineral elements to the surface. Between 16 May and 20 June 1990 the average mass flux of Na to the bog surface by fog, rain, and dry deposition was 21.9, 10.4 and 7.0 mg m?2 d?1. There was little long-term storage of Na within the peatland system, where Na losses measured in stream runoff averaged 34.8 mg m2 d?1, and deep groundwater losses 4 mg m?2 d?1. Calcium and Mg were preferentially retained in the organic soil, whereas K was relatively mobile. Potassium tended to become concentrated in the unsaturated zone. Stream runoff had a consistently higher pH than groundwater, corresponding to higher Ca and Mg concentrations, which may have been from mineral sources in the headwater ponds. Otherwise, the stream water chemistry was closely related to groundwater in the upper layers of the peat deposit. 相似文献
4.
Wang Yanhui 《水文研究》1992,6(2):241-251
Black locust (Robina pseudoacacia) has become one of the most important shelter species in the loess area of northwest China. This paper summarizes recent research concerning its hydrological influence, including canopy interception, litter absorption capacity, its effect on rainfall kinetic energy, infiltration rates, surface runoff, soil moisture, and evapotranspiration, and its role in soil conservation. Several predictive models are listed. on the basis of existing results, optimum characteristics for an effective plantation are defined, and problems requiring further research are identified. 相似文献
5.
Application of MODFLOW and geographic information system to groundwater flow simulation in North China Plain, China 总被引:2,自引:0,他引:2
Shiqin Wang Jingli Shao Xianfang Song Yongbo Zhang Zhibin Huo Xiaoyuan Zhou 《Environmental Geology》2008,55(7):1449-1462
MODFLOW is a groundwater modeling program. It can be compiled and remedied according to the practical applications. Because
of its structure and fixed data format, MODFLOW can be integrated with Geographic Information Systems (GIS) technology for
water resource management. The North China Plain (NCP), which is the politic, economic and cultural center of China, is facing
with water resources shortage and water pollution. Groundwater is the main water resource for industrial, agricultural and
domestic usage. It is necessary to evaluate the groundwater resources of the NCP as an entire aquifer system. With the development
of computer and internet information technology it is also necessary to integrate the groundwater model with the GIS technology.
Because the geological and hydrogeological data in the NCP was mainly in MAPGIS format, the powerful function of GIS of disposing
of and analyzing spatial data and computer languages such as Visual C and Visual Basic were used to define the relationship
between the original data and model data. After analyzing the geological and hydrogeological conditions of the NCP, the groundwater
flow numerical simulation modeling was constructed with MODFLOW. On the basis of GIS, a dynamic evaluation system for groundwater
resources under the internet circumstance was completed. During the process of constructing the groundwater model, a water
budget was analyzed, which showed a negative budget in the NCP. The simulation period was from 1 January 2002 to 31 December
2003. During this period, the total recharge of the groundwater system was 49,374 × 106 m3 and the total discharge was 56,530 × 106 m3 the budget deficit was −7,156 × 106 m3. In this integrated system, the original data including graphs and attribution data could be stored in the database. When
the process of evaluating and predicting groundwater flow was started, these data were transformed into files that the core
program of MODFLOW could read. The calculated water level and drawdown could be displayed and reviewed online. 相似文献
6.
Ibticem Chamtouri Habib Abida Hafedh Khanfir Salem Bouri 《Environmental Geology》2008,55(5):1123-1133
Groundwater in Sfax City (Tunisia) has been known since the beginning of the century for its deterioration in quality, as
a result of wastewater recharge into the aquifer. An average value of 12 × 106 m3 of untreated wastewater reaches the groundwater aquifer each year. This would result not only in a chemical and biological
contamination of the groundwater, but also in an increase of the aquifer piezometric level. Quantitative impacts were evaluated
by examining the groundwater piezometric level at 57 surface wells and piezometers. The survey showed that, during the last
two decades, the groundwater level was ever increasing in the urban area with values reaching 7 m in part; and decreasing
in Sidi Abid (agricultural area) with values exceeding −3 m. Groundwater samples for chemical and microbial analysis were
collected from 41 wells spread throughout the study area. Results showed significantly elevated levels of sodium, chlorides,
nitrates and coliform bacteria all over the urban area. High levels (NO3: 56–254 mg/l; Na >1,500 mg/l; Coliforms >30/100 ml) can be related to more densely populated areas with a higher density
of pit latrine and recharge wells. Alternatively results showed a very variable chemical composition of groundwater, e.g.
electrical conductivity ranges from 4,040 to19,620 μs/cm and the dry residual varies between 1.4 and 14 g/l with concentrations
increasing downstream. Furthermore a softening of groundwater in Set Ezzit (highly populated sector) was observed. 相似文献
7.
Recharge source and hydrogeochemical evolution of shallow groundwater in a complex alluvial fan system,southwest of North China Plain 总被引:4,自引:0,他引:4
Fadong Li Guoying Pan Changyuan Tang Qiuying Zhang Jingjie Yu 《Environmental Geology》2008,55(5):1109-1122
Many cities around the world are developed at alluvial fans. With economic and industrial development and increase in population,
quality and quantity of groundwater are often damaged by over-exploitation in these areas. In order to realistically assess
these groundwater resources and their sustainability, it is vital to understand the recharge sources and hydrogeochemical
evolution of groundwater in alluvial fans. In March 2006, groundwater and surface water were sampled for major element analysis
and stable isotope (oxygen-18 and deuterium) compositions in Xinxiang, which is located at a complex alluvial fan system composed
of a mountainous area, Taihang Mt. alluvial fan and Yellow River alluvial fan. In the Taihang mountainous area, the groundwater
was recharged by precipitation and was characterized by Ca–HCO3 type water with depleted δ18O and δD (mean value of −8.8‰ δ18O). Along the flow path from the mountainous area to Taihang Mt. alluvial fan, the groundwater became geochemically complex
(Ca–Na–Mg–HCO3–Cl–SO4 type), and heavier δ18O and δD were observed (around −8‰ δ18O). Before the surface water with mean δ18O of −8.7‰ recharged to groundwater, it underwent isotopic enrichment in Taihang Mt. alluvial fan. Chemical mixture and ion
exchange are expected to be responsible for the chemical evolution of groundwater in Yellow River alluvial fan. Transferred
water from the Yellow River is the main source of the groundwater in the Yellow River alluvial fan in the south of the study
area, and stable isotopic compositions of the groundwater (mean value of −8.8‰ δ18O) were similar to those of transferred water (−8.9‰), increasing from the southern boundary of the study area to the distal
end of the fan. The groundwater underwent chemical evolution from Ca–HCO3, Na–HCO3, to Na–SO4. A conceptual model, integrating stiff diagrams, is used to describe the spatial variation of recharge sources, chemical
evolution, and groundwater flow paths in the complex alluvial fan aquifer system. 相似文献
8.
Hydrogeochemical investigations and groundwater provinces of the Friuli Venezia Giulia Plain aquifers,northeastern Italy 总被引:2,自引:0,他引:2
Water resources are a key factor, particularly for the planning of the sustainable regional development of agriculture, as
well as for socio-economic development in general. A hydrochemical investigation was conducted in the Friuli Venezia Giulia
aquifer systems to identify groundwater evolution, recharge and extent of pollution. Temperature, pH, electric conductivity,
total dissolved solids, alkalinity, total hardness, SAR, Ca2+, Na+, K+, Mg2+, Cl−, SO4
2−, NO3
−, HCO3
−
, water quality and type, saturation indexes and the environmental stable isotope δ18O were determined in 149 sampling stations. The pattern of geochemical and oxygen stable isotope variations suggests that
the sub-surface groundwater (from phreatic and shallow confined aquifers) is being recharged by modern precipitations and
local river infiltrations. Four hydrogeological provinces have been recognised and mapped in the Friuli Venezia Giulia Plain
having similar geochemical signatures. These provinces have different degrees of vulnerability to contamination. The deep
confined groundwater samples are significantly less impacted by surface activities; and it appears that these important water
resources have very low recharge rates and would, therefore, be severely impacted by overabstraction. 相似文献
9.
Glacier change and glacier runoff variation in the Tuotuo River basin,the source region of Yangtze River in western China 总被引:3,自引:0,他引:3
Glaciers in the Tuotuo River basin, western China, have been monitored in recent decades by applying topographical maps and
high-resolution satellite images. Results indicate that most of glaciers in the Tuotuo River basin have retreated in the period
from 1968/1971 to 2001/2002, and their shrinkage area is 3.2% of the total area in the late 1960s. To assess the influence
of glacier runoff on river runoff, a modified degree–day model including potential clear-sky direct solar radiation has been
applied to the glaciated regions of the river basin over the period 1961–2004. It was found that glacier runoff has increased
in the last 44 years, especially in the 1990s when a two-thirds increase in river runoff was derived from the increase in
glacier runoff caused by loss of ice mass in the entire Tuotuo River basin. 相似文献
10.
Water management and engineering in the karstic High Atlas of Morocco are difficult tasks under the prevailing geological, hydrogeological, geomorphological, vegetational and climatic conditions. It is important to be able to understand and predict the characteristics and availability of water for future water planning in the region under changing climatic and agricultural conditions. An interdisciplinary analysis of problems and adequate hydrological modelling tools developed by geologists, hydrologists and biologists are necessary. The karst areas of the High Atlas Mountains are characterised by impermeable triassic basalt underlying substantial subsurface reservoirs with high potential discharge rates. The karst groundwater aquifers are extensive but largely unknown in dimension, probably with a hierarchical network of groundwater flow paths. It is estimated that approximately 70% of the surface water is directly lost to groundwater. Steep landslide- and debris flow prone slopes exist next to coarse-grained, highly porous river beds. Infrequent, high intensity rainfall or snowmelt causes a particularly high flood risk to these karst areas. In addition, agriculture and land use changes have degraded the karst areas. The most important driving forces for degradation include permanent overgrazing even during droughts and the use of firewood by a continually growing population. Large scale degradation of vegetation has occurred in the oro-mediterranean (mountainous Mediterranean) zone, between 2600 and 3400 m which coincides with the most important zone for karstic groundwater creation. The combination of high amounts of groundwater flow and rapid surface flow due to sparse vegetation has increased the problems of flood flow. 相似文献