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51.
The concentrations of lipids were determined in atmospheric particle, gas and rain samples collected from the tropical North Pacific to assess lipid sources, transport mechanisms and fluxes to the ocean surface. Four lipid compound classes (aliphatic hydrocarbons, fatty alcohols, fatty acid esters, and salts) all unequivocally show a terrestrial vascular plant source. These aerosol lipids originate from wind erosion of Asian and American soils and direct emission from vegetation. The major fluxes result from rain rather than dry deposition. These fluxes are large enough to have a major potential impact on the inventory of terrestrially derived lipid material found in deep-sea sediments. This has been showm for n-alkanes, fatty alcohols, fatty acids, total lipids and for organic carbon. By comparing atmospheric and sediment trap fluxes with sediment accumulation rates, it is suggested that some biogenic terrestrial material is more protected from degradation than marine-derived material. 相似文献
52.
Transport and deposition of suspended particles in saturated porous media: hydrodynamic effect 总被引:1,自引:1,他引:1
Nasre-Dine Ahfir Hua Qing Wang Ahmed Benamar Adbellah Alem Nicolas Massei Jean-Paul Dupont 《Hydrogeology Journal》2007,15(4):659-668
A laboratory study was undertaken to determine the transport and deposition rate of suspended particles in columns of saturated porous media (gravel and glass beads), where the porous media were subjected to steady-state flow. Silt particles with a mode of 14 μm diameter (used as the suspended particles) and fluorescein (as the conservative tracer) were injected into the columns in short pulses. The breakthrough curves were competently described with the analytical solution of a convection–dispersion equation with a first-order deposition rate. The experiments were performed using different flow rates. The suspended particle size distribution, the porous media, and the flow rates themselves were the main factors retained in this study to investigate the mechanisms governing the transport and deposition kinetics in detail. The results showed the existence of a flow rate, beyond which suspended particles travel faster than the conservative tracer. A decrease of the deposition rate of suspended particles beyond a critical flow velocity was also observed. Such behaviour led to consideration of the couple hydrodynamic-gravity forces at high flow rates. As the hydrodynamic force increases, particle deposition rates are reduced due to the effect of hydrodynamic forces inhibiting the deposition. 相似文献
53.
North End Lake is a polluted and eutrophic freshwater system located in Port Elizabeth, South Africa. Since the lake is expected
to be used for recreational/tourist purposes by 2010, a rehabilitation program will have to be designed. For this reason,
we retrieved a sediment core from the central region of the lake to decipher the effect of historical human impacts on the
water body. Pre-disturbance paleolimnological inferences indicate that the lake was likely mesotrophic. After ∼1831, when
sheep farming activities were undertaken in the catchment, increases in trophic state and changes in sediment composition
were observed. After ∼1937, increases in trace metal levels, organic matter, spheroidal carbonaceous particles (SCP) and changes
in sediment composition were recorded. The system became eutrophic as indicated by the dominance of the diatom Actinocyclus normanii, a cosmopolitan species often observed in systems where water quality has been dramatically degraded. The conditions worsened
after 1986 because of the construction of a storm-water retention system, which intentionally channeled storm-water runoff
into the lake. Because of this, extremely high values of fecal coliforms (i.e. 2 × 106 every 100 ml) have been measured in the water column. The paleolimnological information identified the sharp increase in
organic content in the uppermost section of the core, and this could be correlated to the operation of the storm-water retention
system. Therefore, as an immediate management measure, we suggest that the storm-water retention system should either no longer
be utilized, or the storm-water runoff should be treated before disposal into the lake. In addition, an effective sewage system
has to be constructed. 相似文献
54.
考虑湿度影响的城市气溶胶夜晚温度效应 总被引:10,自引:0,他引:10
本文利用一维非定常模式,研究了城市上空干、湿气溶胶粒子对夜间边界层温度的影响。结果表明,湿气溶胶粒子对低层大气有明显的升温作用,而对中上层大气则起降温作用,同时改变了贴地逆温层结构和边界层稳定度。 相似文献
55.
In this paper we describe the transport of pollution in groundwater in the neighbourhood of a well in a uniform background flow. We compute the rate at which contaminated particles reach the well as a function of the place of the source of pollution. The motion of a particle in a dispersive flow is seen as a random walk process. The Fokker-Planck equation for the random motion of a particle is transformed using the complex potential for the advective flow field. The resulting equation is solved asymptotically after a stretching transformation. Finally, the analytical solution is compared with results from Monte Carlo simulations with the random walk model. The method can be extended to arbitrary flow fields. Then by a numerical coordinate transformation the analytical results can still be employed. 相似文献
56.
Thin film methods and X ray energy dispersive technique were applied to analyze sulfate-containing particles in Beijing in order to examine their features and sources. Atmospheric aerosol particles were collected on electron mi-croscope meshes according to two size ranges: coarse particles (r>0.5μm) and fine particles (0.5μm≥r≥0.1μm) by using a two-stage impactor. It was found fiat more than seventy percent of the fine particles and about twenty percent of the coarse particles were sulfate-containing particles. These particles were formed mainly through heterogeneous nucleation. The element composition analyses revealed that the atmospheric aerosol particles in Beijing were domi-nated by crustal particles and construction dust. 相似文献
57.
We present for the first time a statistical study of 50 keV ion events of a magnetospheric origin upstream from Earths bow shock. The statistical analysis of the 50–220 keV ion events observed by the IMP-8 spacecraft shows: (1) a dawn-dusk asymmetry in ion distributions, with most events and lower intensities upstream from the quasi-parallel pre-dawn side (4 LT-6 LT) of the bow shock, (2) highest ion fluxes upstream from the nose/dusk side of the bow shock under an almost radial interplanetary magnetic field (IMF) configuration, and (3) a positive correlation of the ion intensities with the solar wind speed and the index of geomagnetic index Kp, with an average solar wind speed as high as 620 km s–1 and values of the index Kp 2. The statistical results are consistent with (1) preferential leakage of 50 keV magnetospheric ions from the dusk magnetopause, (2) nearly scatter free motion of 50 keV ions within the magnetosheath, and (3) final escape of magnetospheric ions from the quasi-parallel dawn side of the bow shock. An additional statistical analysis of higher energy (290–500 keV) upstream ion events also shows a dawn-dusk asymmetry in the occurrence frequency of these events, with the occurrence frequency ranging between 16%-34% in the upstream region. 相似文献
58.
山西义兴寨金矿床金矿物颗粒的产出及其成矿动力学意义 总被引:1,自引:0,他引:1
山西义兴寨金矿床的金主要呈包体金和裂隙金两种产出状态.文章根据成矿地球化学动力学理论,论证了金元素在含矿断裂发生脆性破裂和脆-韧性扩张活动中析出的化学反应类型,以及受反应动力学条件的制约,形成矿石中金不同产出状态的规律.指出热液矿床中普遍存在的包体金为热液成矿早期阶段断裂发生脆性破裂和成矿流体沸腾,导致快速反应结晶的产物;而裂隙金和晶隙金为成矿晚期金等矿质在流体中残余富集,同时成矿断裂再次发生脉动破裂,即成矿热力学演化与有利的构造动力学因素耦合作用的结果.得出金矿物颗粒的产出状态具有成矿动力学意义的结论. 相似文献
59.
U. von Zahn G. von Cossart J. Fiedler K. H. Fricke G. Nelke G. Baumgarten D. Rees A. Hauchecorne K. Adolfsen 《Annales Geophysicae》2000,18(7):815-833
We report on the development and current capabilities of the ALOMAR Rayleigh/Mie/Raman lidar. This instrument is one of the core instruments of the international ALOMAR facility, located near Andenes in Norway at 69°N and 16°E. The major task of the instrument is to perform advanced studies of the Arctic middle atmosphere over altitudes between about 15 to 90 km on a climatological basis. These studies address questions about the thermal structure of the Arctic middle atmosphere, the dynamical processes acting therein, and of aerosols in the form of stratospheric background aerosol, polar stratospheric clouds, noctilucent clouds, and injected aerosols of volcanic or anthropogenic origin. Furthermore, the lidar is meant to work together with other remote sensing instruments, both ground- and satellite-based, and with balloon- and rocket-borne instruments performing in situ observations. The instrument is basically a twin lidar, using two independent power lasers and two tiltable receiving telescopes. The power lasers are Nd:YAG lasers emitting at wavelengths 1064, 532, and 355 nm and producing 30 pulses per second each. The power lasers are highly stabilized in both their wavelengths and the directions of their laser beams. The laser beams are emitted into the atmosphere fully coaxial with the line-of-sight of the receiving telescopes. The latter use primary mirrors of 1.8 m diameter and are tiltable within 30° off zenith. Their fields-of-view have 180 rad angular diameter. Spectral separation, filtering, and detection of the received photons are made on an optical bench which carries, among a multitude of other optical components, three double Fabry-Perot interferometers (two for 532 and one for 355 nm) and one single Fabry-Perot interferometer (for 1064 nm). A number of separate detector channels also allow registration of photons which are produced by rotational-vibrational and rotational Raman scatter on N2 and N2+O2 molecules, respectively. Currently, up to 36 detector channels simultaneously record the photons collected by the telescopes. The internal and external instrument operations are automated so that this very complex instrument can be operated by a single engineer. Currently the lidar is heavily used for measurements of temperature profiles, of cloud particle properties such as their altitude, particle densities and size distributions, and of stratospheric winds. Due to its very effective spectral and spatial filtering, the lidar has unique capabilities to work in full sunlight. Under these conditions it can measure temperatures up to 65 km altitude and determine particle size distributions of overhead noctilucent clouds. Due to its very high mechanical and optical stability, it can also employed efficiently under marginal weather conditions when data on the middle atmosphere can be collected only through small breaks in the tropospheric cloud layers. 相似文献
60.
J. M. C. Plane 《Annales Geophysicae》2000,18(7):807-814
It is proposed that a component of meteoric smoke, sodium bicarbonate (NaHCO3), provides particularly effective condensation nuclei for noctilucent clouds. This assertion is based on three conditions being met. The first is that NaHCO3 is present at sufficient concentration (104 cm–3) in the upper mesosphere between 80 and 90 km. It is demonstrated that there is strong evidence for this based on recent laboratory measurements coupled with atmospheric modelling. The second condition is that the thermodynamics of NaHCO3(H2O)n cluster formation allow spontaneous nucleation to occur under mesospheric conditions at temperatures below 140 K. The Gibbs free energy changes for forming clusters with n = 1 and 2 were computed from quantum calculations using hybrid density functional/Hartree-Fock (B3LYP) theory and a large basis set with added polarization and diffuse functions. The results were then extrapolated to higher n using an established dependence of the free energy on cluster size and the free energy for the sublimation of H2O to bulk ice. A 1-dimensional model of sodium chemistry was then employed to show that spontaneous nucleation to form ice particles (n > 100) should occur between 84 and 89 km in the high-latitude summer mesosphere. The third condition is that other metallic components of meteoric smoke are less effective condensation nuclei, so that the total number of potential nuclei is small relative to the amount of available H2O. Quantum calculations indicate that this is probably the case for major constituents such as Fe(OH)2, FeO3 and MgCO3. 相似文献