Measurement of lower-stratospheric aerosol by a balloon-borne photometer

Height distribution of the stratospheric aerosol extinction coefficient was measured in the altitude range 10 to 20 km by a balloon-borne multi-color sunphotometer in May 1978. It is demonstrated that detailed structures of the distribution of stratospheric aerosol can be remotely measured by the solar occultation method as well as by lidar andin situ particle counter observations. In the aerosol layer appearing at 18 km altitude the extinction coefficient at 800–1000 nm wavelength reached to 3×10^–7 m^–1, which was reasonable compared with lidar observations. Wavelength dependence of the aerosol optical depth was crudely estimated to be proportional to ^–1.5.     

The Henry's Law Constants of the Haloacetic Acids

Henry's law constants K_H (mol kg^-1 atm^-1) have been measured between 278.15 K and 308.15 K for the following organic acids: CH₂FCOOH (ln(K_H[298.15 K]) = 11.3 ± 0.2), CH₂ClCOOH (11.59 ± 0.14), CH₂BrCOOH (11.94 ± 0.21), CHF₂COOH (10.32 ± 0.10), CHCl₂COOH (11.69 ± 0.11), CHBr₂COOH (12.33 ± 0.29), CBr₃COOH (12.61 ± 0.21), and CClF₂COOH (10.11 ± 0.12). The variation of K_H with temperature was determined for all acids except CH₂FCOOH and CBr₃COOH, with _r H° for the dissolution reaction ranging from –85.2 ± 2.6 to –57.1 ± 2.5 kJ mol^-1, meaning that their solubility is generally more sensitive to temperature than is the case for the simple carboxylic acids. The Henry's law constants show consistent trends with halogen substitution and, together with their high solubility compared to the parent (acetic) acid (ln(K_H[298.15 K]) = 8.61), present a severe test of current predictive models based upon molecular structure. The solubility of haloacetic acids and strong dissociation at normal pH mean that they will partition almost entirely into cloud and fog in the atmosphere (0.05–1.0 g H₂O m^-3), but can reside in both phases for the liquid water contents typical of aerosols (10^-5-10^-4 g H₂O m^-3).     

中国地区大气气溶胶辐射强迫及区域气候效应的数值模拟

利用太阳直接辐射日总量和日照时数等多年观测资料,反演了中国地区大气气溶胶0.75 μm光学厚度的年、月平均值,分析了我国大气气溶胶状况的时空分布特征。据此,在中国区域气候模式中考虑气溶胶的辐射影响,模拟中国地区气溶胶直接辐射强迫的大小及气候响应的季节变化特征。计算结果表明: 我国大气气溶胶光学厚度多年平均分布状况是以四川盆地为大值中心向四周减少;长江中下游武汉附近和南疆盆地为另两个大值中心;青藏高原为气溶胶低值区;我国绝大部分地区春季气溶胶光学厚度值最大,各地气溶胶光学厚度最小值出现的季节则有所不同。气溶胶辐射强迫介于-5.3～-13 W/m2之间;辐射强迫具有春、夏季大,秋、冬季小,冬季南方偏大,夏季北方偏大的特征。气溶胶辐射强迫的分布与其光学厚度的分布基本一致。由于气溶胶的影响,中国大陆地区地面气温均有所下降,四川盆地到长江中下游地区以及青藏高原北侧到河套地区降温最为明显,分别可达-0.4℃和-0.5℃。气候响应具有明显的季节特征。地面气温的变化除与辐射强迫的大小有关外,还受大气环流的影响。     

中国地区气溶胶的辐射强迫及其气候响应试验

根据国内测定的排放因子数据和国家、部委及各省市统计年鉴公布的排放源数据,得到的中国大陆的1°×1°网格精度的SO2的排放分布,计算了中国地区人为扰动气溶胶的辐射强迫。应用近期开发的二维能量平衡模式计算了由该种气溶胶所引起的中国地区地面温度变化。模式结果表明,最大辐射强迫和最大地面温度变化都集中在中国的沿海和四川地区。最大辐射强迫达3 W/m2。     

Mean bulk densities of samples of dry atmospheric aerosol particles: A summary of measured data

Mean bulk densities of various samples of dry atmospheric aerosol particles sampled at different sites and during different seasons and weather situations range between 1.8 and more than 3 gm cm³.     

Evaluation of an empirical orthogonal function–based method to downscale soil moisture patterns based on topographical attributes

Soil moisture influences many hydrologic applications including agriculture, land management and flood prediction. Most remote‐sensing methods that estimate soil moisture produce coarse resolution patterns, so methods are required to downscale such patterns to the resolutions required by these applications (e.g. 10‐ to 30‐m grid cells). At such resolutions, topography is known to affect soil moisture patterns. Although methods have been proposed to downscale soil moisture based on topography, they usually require the availability of past high‐resolution soil moisture patterns from the application region. The objective of this article is to determine whether a single topographic‐based downscaling method can be used at multiple locations without relying on detailed local observations. The evaluated downscaling method is developed on the basis of empirical orthogonal function (EOF) analysis of space–time soil moisture data at a reference catchment. The most important EOFs are then estimated from topographic attributes, and the associated expansion coefficients are estimated on the basis of the spatial‐average soil moisture. To test the portability of this EOF‐based method, it is developed separately using four data sets (Tarrawarra, Tarrawarra 2, Cache la Poudre and Satellite Station), and the relationships that are derived from these data sets to estimate the EOFs and expansion coefficients are compared. In addition, each of these downscaling methods is applied not only for the catchment where it was developed but also to the other three catchments. The results suggest that the EOF downscaling method performs well for the location where it is developed, but its performance degrades when applied to other catchments. Copyright © 2011 John Wiley & Sons, Ltd.     

Assessment of intermediate fine sediment storage in a braided river reach (southern French Prealps)

This paper presents a field investigation on river channel storage of fine sediments in an unglaciated braided river, the Bès River, located in a mountainous region in the southern French Prealps. Braided rivers transport a very large quantity of bedload and suspended sediment load because they are generally located in the vicinity of highly erosive hillslopes. Consequently, these rivers play an important role because they supply and control the sediment load of the entire downstream fluvial network. Field measurements and aerial photograph analyses were considered together to evaluate the variability of fine sediment quantity stored in a 2·5‐km‐long river reach. This study found very large quantities of fine sediment stored in this reach: 1100 t per unit depth (1 dm). Given that this reach accounts for 17% of the braided channel surface area of the river basin, the quantities of fine sediment stored in the river network were found to be approximately 80% of the mean annual suspended sediment yields (SSYs) (66 200 t year^?1), comparable to the SSYs at the flood event scale: from 1000 t to 12 000 t depending on the flood event magnitude. These results could explain the clockwise hysteretic relationships between suspended sediment concentrations and discharges for 80% of floods. This pattern is associated with the rapid availability of the fine sediments stored in the river channel. This study shows the need to focus on not only the mechanisms of fine sediment production from hillslope erosion but also the spatiotemporal dynamics of fine sediment transfer in braided rivers. Copyright © 2010 John Wiley & Sons, Ltd.     

在大洋环流模型中对应于惯性内波破碎的垂直混合的一个参数化方案

Based on the theoretical spectral model of inertial internal wave breaking(fine structure) proposed previously, in which the effects of the horizontal Coriolis frequency component f-tilde on a potential isopycnal are taken into account, a parameterization scheme of vertical mixing in the stably stratified interior below the surface mixed layer in the ocean general circulation model(OGCM) is put forward preliminarily in this paper. Besides turbulence, the impact of sub-mesoscale oceanic processes(including inertial internal wave breaking product) on oceanic interior mixing is emphasized. We suggest that adding the inertial internal wave breaking mixing scheme(F-scheme for short) put forward in this paper to the turbulence mixing scheme of Canuto et al.( T-scheme for short) in the OGCM, except the region from 15°S to 15°N. The numerical results of F-scheme by using WOA09 data and an OGCM(LICOM, LASG/IAP climate system ocean model) over the global ocean are given. A notable improvement in the simulation of salinity and temperature over the global ocean is attained by using T-scheme adding F-scheme, especially in the mid- and high-latitude regions in the simulation of the intermediate water and deep water. We conjecture that the inertial internal wave breaking mixing and inertial forcing of wind might be one of important mechanisms maintaining the ventilation process. The modeling strength of the Atlantic meridional overturning circulation(AMOC) by using T-scheme adding F-scheme may be more reasonable than that by using T-scheme alone, though the physical processes need to be further studied, and the overflow parameterization needs to be incorporated. A shortcoming in F-scheme is that in this paper the error of simulated salinity and temperature by using T-scheme adding F-scheme is larger than that by using T-scheme alone in the subsurface layer.     

一次霾天气条件下石家庄上空大气气溶胶数浓度的飞行探测与特征分析

利用2010年8月30日河北省石家庄一次霾天气条件下的气溶胶飞行探测资料,分析了石家庄地区上空658—6933 m高度范围内大气气溶胶粒子平均数浓度、平均直径的垂直分布特征和9个水平飞行高度上的谱分布特征。结果表明:轻度霾天气条件下的气溶胶平均数浓度为325个/cm3,平均直径为0.169μm。在约1000 m高度以下,气溶胶平均数浓度随高度的增加呈线性减少趋势。粒径也随高度增加而减小,由0.187μm减小至0.164μm。1000 m高度以上,气溶胶平均数浓度随高度减少趋势变缓,粒子平均直径在0.167~0.171μm范围内波动。9个不同高度上的谱分布都呈单峰型,随着高度增加,谱宽变小,峰值向小尺度方向移动。后向轨迹计算分析表明:污染气团的远距离输送可能是导致大气1500 m高度层气溶胶数浓度突增的原因。     

基于FastICA算法和MODIS数据的水稻面积提取

以苏、皖、赣三省为研究区域,采用FastICA算法从MODIS数据中提取2010年水稻种植面积,并验证该算法在混合像元分解中的有效性。在对2010年46景8 d合成地表反射率产品数据进行预处理的基础上,结合MODIS土地利用产品和平滑滤波算法,构建耕地类型像元的I_LSW和I_NDV时相变化曲线。依据I_LSW和I_NDV曲线在水稻移栽期前后的变化规律,并根据由各地区水稻I_NDV时相曲线计算得到水稻相似性指数,从MODIS影像中提取水稻像元。采用FastICA算法对潜在水稻像元水稻生长期内的I_NDV时相曲线进行分解,计算每个像元的水稻丰度,绘制水稻丰度图,获取研究区各省水稻分布和种植面积。利用统计年鉴数据和样方资料对FastICA算法提取的水稻面积进行了验证。结果显示:采用水稻相似性曲线有利于提高稻田识别效率,所获取的水稻分布与实际情况吻合;FastICA算法能够分解不同地区水稻I_NDV时相曲线;与统计资料比较,江苏、安徽、江西三省水稻面积的提取精度分别为86.4%、87.9%、51.5%。江西水稻面积提取误差主要出现在地形起伏较大的山区。