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181.
182.
183.
Nitrogen and sulfur species in Antarctic aerosols at Mawson,Palmer Station,and Marsh (King George Island) 总被引:4,自引:0,他引:4
D. L. Savoie J. M. Prospero R. J. Larsen F. Huang M. A. Izaguirre T. Huang T. H. Snowdon L. Custals C. G. Sanderson 《Journal of Atmospheric Chemistry》1993,17(2):95-122
High volume bulk aerosol samples were collected continuously at three Antarctic sites: Mawson (67.60° S, 62.50° E) from 20 February 1987 to 6 January 1992; Palmer Station (64.77° S, 64.06° W) from 3 April 1990 to 15 June 1991; and Marsh (62.18° S, 58.30° W) from 28 March 1990, to 1 May 1991. All samples were analyzed for Na+, SO
4
2–
, NO
3
–
, methanesulfonate (MSA), NH
4
+
,210Pb, and7Be. At Mawson for which we have a multiple year data set, the annual mean concentration of each species sometimes vary significantly from one year to the next: Na+, 68–151 ng m–3; NO
3
–
, 25–30 ng m–3; nss SO
4
2–
, 81–97 ng m–3; MSA, 19–28 ng m–3; NH
4
+
, 16–21 ng m–3;210Pb, 0.75–0.86 fCi m–3. Results from multiple variable regression of non-sea-salt (nss) SO
4
2–
with MSA and NO
3
–
as the independent variables indicates that, at Mawson, the nss SO
4
2–
/MSA ratio resulting from the oxidation of dimethylsulfide (DMS) is 2.80±0.13, about 13% lower than our earlier estimate (3.22) that was based on 2.5 years of data. A similar analysis indicates that the ratio at Palmer is about 40% lower, 1.71±0.10, and more comparable to previous results over the southern oceans. These results when combined with previously published data suggest that the differences in the ratio may reflect a more rapid loss of MSA relative to nss SO
4
2–
during transport over Antarctica from the oceanic source region. The mean210Pb concentrations at Palmer and Marsh and the mean NO
3
–
concentration at Palmer are about a factor of two lower than those at Mawson. The210Pb distributions are consistent with a210Pb minimum in the marine boundary layer in the region of 40°–60° S. These features and the similar seasonalities of NO
3
–
and210Pb at Mawson support the conclusion that the primary source regions for NO
3
–
are continental. In contrast, the mean concentrations of MSA, nss SO
4
2–
, and NH
4
+
at Palmer are all higher than those at Mawson: MSA by a factor of 2; nss SO
4
2–
by 10%; and NH
4
+
by more than 50%. However, the factor differences exhibit substantial seasonal variability; the largest differences generally occur during the austral summer when the concentrations of most of the species are highest. NH
4
+
/(nss SO
4
2–
+MSA) equivalent ratios indicate that NH3 neutralizes about 60% of the sulfur acids during December at both Mawson and Palmer, but only about 30% at Mawson during February and March. 相似文献
184.
185.
186.
187.
This article summarizes work on multiple scattering based on models of media with randomly distributed scatterers. The scatterers are isotropic and statistically uniform. Measuring distance in terms of mean-free pathL
s and time in terms of the mean-free timesL
s/V, whereV is the velocity of scattered waves, we have more convenient dimensionless distance and time. It can be shown that after the dimensionless time equals 0.65 energy contributed from multiple scattering becomes predominant. Thus the later coda reflects the effect of multiple scattering rather than single scattering. Treating the seismic record, including starting and tail parts, as a whole, the diffusion theory predicts that at a dense distribution of scatterers and a small distance between source and receiver, codas reflect mainly intrinsicQ
i. Of course, this conclusion is coincident with the presumption of the diffusion theory,Q
s>Q
i. However, from a new integral equation of multiple scattering, which deals with the scattered waves and primary waves separately, the conclusion is similar but clearer. This article quotes the new expression for coda energy in two-dimensional space. It shows that if the receiver is close to the source, the coda decay reflects only intrinsicQ
i, then as the distance increases, effects of scatteringQ
s, are involved in the decay feature. The theoretical plots of coda decay show that it seems in most cases in the earthQ
i should not be smaller than one tenth ofQ
s.Project Sponsored by the Joint Earthquake Science Foundation of China. 相似文献
188.
用改进的数学公式,便于用单钻孔资料和岩层复平求面理倾斜、求岩层厚度、求地层断距等多个课题。 相似文献
189.
190.
A. Hallberg J. A. Ogren K. J. Noone K. Okada J. Heintzenberg I. B. Svenningsson 《Journal of Atmospheric Chemistry》1994,19(1-2):153-171
A difference in partitioning between cloud droplets and interstitial air for two chemical species (elemental carbon and sulphur) with different expected behaviour in nucleation scavenging was observed in clouds at Mt. Kleiner Feldberg (825 m asl), near Frankfurt, Germany. The fraction of sulphur incorporated in cloud droplets was always higher than the fraction of elemental carbon. This difference in partitioning has also been observed in fog but under different pollution conditions in the Po Valley, Italy. Both these studies were based on bulk samples. In the present study at Kleiner Feldberg, impactor samples of the particles in the interstitial air and the cloud droplet residuals were taken and a single particle analysis was done on the samples. It was found that, for a given particle size, the majority of particles forming cloud droplets were soluble and that insoluble particles preferentially remained in the interstitial air. 相似文献