Aerosol concentrations and size distribution in the troposphere and lower stratosphere over Thumba

Rocket-borne ultraviolet photometers operating at =0.31 m have been used at Thumba (8°33N, 76°52E) to make measurements of atmospheric scattering at tropospheric and lower stratospheric altitudes. Measurements could be made of the amplitude of the scattered fluxes and the angular distribution up to an altitude of about 24 km on three rocket flights conducted as part of the 16 February 1980 solar eclipse campaign. These measurements have been used to study the size distribution as well as the number densities of aerosols in the troposphere and lower stratosphere over Thumba.     

Transport and deposition of suspended particles in saturated porous media: hydrodynamic effect

A laboratory study was undertaken to determine the transport and deposition rate of suspended particles in columns of saturated porous media (gravel and glass beads), where the porous media were subjected to steady-state flow. Silt particles with a mode of 14 μm diameter (used as the suspended particles) and fluorescein (as the conservative tracer) were injected into the columns in short pulses. The breakthrough curves were competently described with the analytical solution of a convection–dispersion equation with a first-order deposition rate. The experiments were performed using different flow rates. The suspended particle size distribution, the porous media, and the flow rates themselves were the main factors retained in this study to investigate the mechanisms governing the transport and deposition kinetics in detail. The results showed the existence of a flow rate, beyond which suspended particles travel faster than the conservative tracer. A decrease of the deposition rate of suspended particles beyond a critical flow velocity was also observed. Such behaviour led to consideration of the couple hydrodynamic-gravity forces at high flow rates. As the hydrodynamic force increases, particle deposition rates are reduced due to the effect of hydrodynamic forces inhibiting the deposition.     

Paleolimnological assessment of human impacts on an urban South African lake

North End Lake is a polluted and eutrophic freshwater system located in Port Elizabeth, South Africa. Since the lake is expected to be used for recreational/tourist purposes by 2010, a rehabilitation program will have to be designed. For this reason, we retrieved a sediment core from the central region of the lake to decipher the effect of historical human impacts on the water body. Pre-disturbance paleolimnological inferences indicate that the lake was likely mesotrophic. After ∼1831, when sheep farming activities were undertaken in the catchment, increases in trophic state and changes in sediment composition were observed. After ∼1937, increases in trace metal levels, organic matter, spheroidal carbonaceous particles (SCP) and changes in sediment composition were recorded. The system became eutrophic as indicated by the dominance of the diatom Actinocyclus normanii, a cosmopolitan species often observed in systems where water quality has been dramatically degraded. The conditions worsened after 1986 because of the construction of a storm-water retention system, which intentionally channeled storm-water runoff into the lake. Because of this, extremely high values of fecal coliforms (i.e. 2 × 10⁶ every 100 ml) have been measured in the water column. The paleolimnological information identified the sharp increase in organic content in the uppermost section of the core, and this could be correlated to the operation of the storm-water retention system. Therefore, as an immediate management measure, we suggest that the storm-water retention system should either no longer be utilized, or the storm-water runoff should be treated before disposal into the lake. In addition, an effective sewage system has to be constructed.     

北京地区春末-秋初气溶胶理化特性的观测研究

分析了1997年5～9月和1998年4～9月北京整层大气气溶胶光学厚度、近地面气溶胶粒子数浓度的日变化、季节变化及其与气象要素的关系,还分析了 1997年5月16日、7月21日和8月2日收集的北京单个气溶胶粒子样品的形态、大小和化学元素组成.结果显示,北京地区春末-秋初整层大气气溶胶光学厚度在0.1～1.6之间变化;气溶胶数浓度(D>0.3μm)为几～几百个/cm3;整层大气气溶胶光学厚度的日变化型式与近地面气溶胶数浓度呈现相反的走向;气溶胶光学厚度和数浓度的日、季节变化显示了整层大气和近地面大气气溶胶与该地区气象、气候条件的关系.气溶胶数浓度与大气相对湿度呈正相关,与风向的关系是偏东风数浓度大,西、西南风数浓度小.电子显微镜分析的结果表明:颗粒物的形态以不规则形、丸形、液态滴形和方形为主;颗粒物化学元素组成有Si、K、S、Al、Mg、Ca、Fe等元素;人类活动排放的Zn、P、Ti、pb、Ba等元素也探测到;北京近地面粒子的一个显著特点是富含Ca和K元素,它们可能分别来自建筑粉尘和有机物的燃烧;给出了一个典型的碳黑粒子和一个粒子经过凝结过程的"卫星"滴环绕的矿物粒子的照片和元素谱图.     

VARIABILITY OF AEROSOL OPTICAL PROPERTIES OVER HEFEI DURING SEPTEMBER 1993 TO SEPTEMBER 1994

An 8-wavelength sun-photometer has been operated at Hefei (31.31°N, 117.17°E) to monitoroptical properties of atmospheric aerosols. Altogether 133 solar spectral extinction data were ob-tained on clear days during the period from September 1993 through September 1994, In this pa-per, the feature of the sun-photometer is briefly described. A relative aureole method is intro-duced. which can be used to monitor temporal evolution of aerosol loading during the sun-pho-tometer calibration period. Temporal variabilities of spectral aerosol optical depths and Angstromturbidity parameters are presented. Relation of these variabilities with synoptic and local meteoro-logical conditions are analyzed and discussed, From measured spectral aerosol optical depths undersome representative atmospheric conditions, columnar aerosol size distributions have been retrievedby a linearly constrained inversion method. These typical columnar aerosol size distributions are al-so presented and discussed.     

考虑湿度影响的城市气溶胶夜晚温度效应

本文利用一维非定常模式，研究了城市上空干、湿气溶胶粒子对夜间边界层温度的影响。结果表明，湿气溶胶粒子对低层大气有明显的升温作用，而对中上层大气则起降温作用，同时改变了贴地逆温层结构和边界层稳定度。     

大气臭氧与气溶胶垂直分布的高空气球探测

本文给出了1993年9月12日利用高空科学气球在河北省香河地区探测到的大气臭氧和气溶胶的垂直分布。结果发现:(1) 大气臭氧的数密度在整个对流层较低(～10[12]mol/cm3)，并从地面到对流层顶略有下降；对流层顶以上开始快速增加，极值层高度在～24 km，其值为4.78×10[12]mol/cm3；臭氧分压有类似的分布特征，极值146×10[-4]Pa，位于同一高度；(2) 在平流层低层，臭氧分压有一个次极值62×10[-4]Pa，位于15～16 km；(3) 0～30 km大气气溶胶数密度呈现出三个峰值:143，8和1.1 个/cm[3]，分别位于近地面、5 km和21 km；（4）气溶胶的数密度谱在对流层为双模态；在平流层，次峰消失。同时，我们还与其他观测结果作了比较分析。     

火山气溶胶的辐射影响

本文应用辐射传输计算研究了火山气溶胶,特别是大的火山爆发后短时期及火山周围地区内的火山气溶胶,对到达地面的向下的总的太阳辐射通量、行星反照率及大气加热率的可能影响.     

Contamination of a well in a uniform background flow

In this paper we describe the transport of pollution in groundwater in the neighbourhood of a well in a uniform background flow. We compute the rate at which contaminated particles reach the well as a function of the place of the source of pollution. The motion of a particle in a dispersive flow is seen as a random walk process. The Fokker-Planck equation for the random motion of a particle is transformed using the complex potential for the advective flow field. The resulting equation is solved asymptotically after a stretching transformation. Finally, the analytical solution is compared with results from Monte Carlo simulations with the random walk model. The method can be extended to arbitrary flow fields. Then by a numerical coordinate transformation the analytical results can still be employed.     

Tests for individual Sulfate－Containing Particles in Urban Atmosphere in Beijing

Thin film methods and X ray energy dispersive technique were applied to analyze sulfate-containing particles in Beijing in order to examine their features and sources. Atmospheric aerosol particles were collected on electron mi-croscope meshes according to two size ranges: coarse particles (r>0.5μm) and fine particles (0.5μm≥r≥0.1μm) by using a two-stage impactor. It was found fiat more than seventy percent of the fine particles and about twenty percent of the coarse particles were sulfate-containing particles. These particles were formed mainly through heterogeneous nucleation. The element composition analyses revealed that the atmospheric aerosol particles in Beijing were domi-nated by crustal particles and construction dust.