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71.
利用溶胶凝胶法自制了碳纳米管和纳米二氧化钛的复合光催化剂,采用投射电子显微镜和X光衍射仪对粉体的粒径、物象、形貌和热稳定性等进行表征。通过研究光照条件、催化剂的投加量、油的初始浓度、催化剂制备的煅烧条件等因素,考察了自制碳纳米管和纳米二氧化钛的复合催化剂对降解模拟海洋柴油污染的海水去除率的影响。研究发现,在可见光照条件下,400℃煅烧2 h的复合催化剂,投加量为0.4 g/L、柴油的初始浓度为0.6 g/L、反应的光照时间为4 h时效果最好,去除率可达到67.65%。  相似文献   
72.
This paper evaluates the global economic damage arising from the effects of climate change and associated carbon dioxide concentrations on the loss of coral reefs. We do this by first estimating the effects of sea surface temperature and carbon dioxide concentrations on coral cover. We develop a statistical relationship between coral coverage and sea surface temperature that indicates that the effects are dependent on the temperature range. For example, we find that increasing sea surface temperature causes coral coverage to decrease when sea surface temperature is higher than 26.85 °C, with the estimated reduction being 2.3% when sea surface temperature increases by 1%. In addition, we find that a 1% carbon dioxide increase induces a 0.6% reduction in global coral coverage. We also estimate the resultant loss in economic value based on a meta-analysis of the recreational and commercial value of reef coverage and a crude proportional approach for other value factors. The meta-analysis shows that the coral reef value decreases by 3.8% when coral cover falls by 1%. By combining these two steps we find that the lost value in terms of the global coral reef value under climate change scenarios ranges from US$3.95 to US$23.78 billion annually.  相似文献   
73.
The purple-tipped sea urchin, Psammechinus miliaris, was exposed to artificially acidified seawater treatments (pH(w) 6.16, 6.63 or 7.44) over a period of 8 days. Urchin mortality of 100% was observed at pH(w) 6.16 after 7 days and coincided with a pronounced hypercapnia in the coelomic fluid producing an irrecoverable acidosis. Coelomic fluid acid-base measures showed that an accumulation of CO(2) and a significant reduction in pH occurred in all treatments compared with controls. Bicarbonate buffering was employed in each case, reducing the resultant acidosis, but compensation was incomplete even under moderate environmental hypercapnia. Significant test dissolution was inferred from observable increases in the Mg(2+) concentration of the coelomic fluid under all pH treatments. We show that a chronic reduction of surface water pH to below 7.5 would be severely detrimental to the acid-base balance of this predominantly intertidal species; despite its ability to tolerate fluctuations in pCO(2) and pH in the rock pool environment. The absence of respiratory pigment (or any substantial protein in the coelomic fluid), a poor capacity for ionic regulation and dependency on a magnesium calcite test, make echinoids particularly vulnerable to anthropogenic acidification. Geological sequestration leaks may result in dramatic localised pH reductions, e.g. pH 5.8. P. miliaris is intolerant of pH 6.16 seawater and significant mortality is seen at pH 6.63.  相似文献   
74.
南海西部东方1-1、崖城13-1和乐东等气田具有CO2含量高的特点,每年从生产出的天然气中分离出大量的CO2。为了减少CO2在大气中的排放,考虑在莺歌海地区选择合适的盐水层埋存体,拟进行CO2地质埋存示范工程。根据CO2在盐水层中的各种埋存机理,并考虑盐水层构造特征对CO2运移分布的影响,提出了一种较为准确的CO2埋存潜力评估方法,并利用此方法对筛选出的5个备选盐水层进行了评估。评估结果表明,各盐水层埋存潜力巨大,都远远大于示范工程期限内预计的CO2埋存总量,并可将这些盐水层作为将来海南省及临近广东省人为CO2的埋存场所。南海西部东方1-1、崖城13-1和乐东等气田具有CO2含量高的特点,每年从生产出的天然气中分离出大量的CO2。为了减少CO2在大气中的排放,考虑在莺歌海地区选择合适的盐水层埋存体,拟进行CO2地质埋存示范工程。根据CO2在盐水层中的各种埋存机理,并考虑盐水层构造特征对CO2运移分布的影响,提出了一种较为准确的CO2埋存潜力评估方法,并利用此方法对筛选出的5个备选盐水层进行了评估。评估结果表明,各盐水层埋存潜力巨大,都远远大于示范工程期限内预计的CO2埋存总量,并可将这些盐水层作为将来海南省及临近广东省人为CO2的埋存场所。  相似文献   
75.
Neoproterozoic chemostratigraphy   总被引:3,自引:0,他引:3  
Chemostratigraphy has diverse applications to investigating the rock record, such as reconstructing paleoenvironments, determining the tectonic setting of sedimentary basins, indirect dating, and establishing regional or global correlations. Chemostratigraphy is thus an integral component of many investigations of the ancient sedimentary record. In this contribution, we review the principle inorganic geochemical methods that have been applied to the Neoproterozoic sedimentary record. Analysis of the traditional stable and radiogenic isotope systems, such as δ13C, δ18O, δ34S, and 87Sr/86Sr, is routine, particularly in successions rich in carbonate. These mainstay applications have yielded invaluable data and information bearing on the chronology and evolution of this eventful era in Earth history. Alongside the growing database of traditional data, a series of novel geochemical techniques have given rise to important new models and constraints on Neoproterozoic biogeochemical change. In particular, a range of proxies for water column redox, mainly obtained from black shales, have shed light on the pace and tempo of Neoproterozoic oxygenation and its link to the appearance of early animal evolution. Increased integration of diverse geochemical, sedimentological, and paleontological datasets, and the gradual radiometric calibration of the stratigraphic record promise to bring the details of the evolution of the Neoproterozoic Earth system into ever greater focus.  相似文献   
76.
77.
The possibility of extreme sea-level rise is one of the commonly cited reasons for concern about climate change. Major increases in sea level would likely be driven by the melting or collapse of major ice sheets. This possibility has implications for the social cost of carbon dioxide, which is a key policy value as well as a useful summary measure of damage caused by greenhouse gas emissions.This paper extends earlier work on the importance of low-probability, high-impact events for the social cost of carbon dioxide to incorporate the possibility of extreme sea-level rise.To estimate its impact, an integrated assessment model is used, which allows a probabilistic assessment of climate change damages based on the linkages between the economic and climate systems. In the model, the generic discontinuity damage is replaced with the possibility of large-scale damage from factors that are taken to be correlated with temperature rise and, crucially for this paper, explicit consideration of extreme sea-level rise.Estimates of the amount of increase in the social cost of carbon dioxide that can be expected from incorporating extreme sea-level rise show that the increase is significant, though not especially large in percentage terms.The paper contributes to the literature of how to represent uncertain climate impacts in integrated assessment models and the associated estimation of the social cost of carbon dioxide.  相似文献   
78.
《Atmósfera》2014,27(2):193-214
For the first time, maps of surface concentration of nitrogen dioxide (NO2) are presented for the Colombian territory. NO2 surface concentrations for the year 2007 are inferred based on two sources of tropospheric NO2 column data: (1) a simulation using a three-dimensional global model (GEOS-Chem) and (2) measurements made by the ozone monitoring instrument (OMI) onboard the NASA Aura satellite. Results show monthly averages between 0.1 and 6 ppbv. We compare these inferred values to corrected ground measurements of NO2. We find correlation coefficients of up to 0.91 between the inferred data and the corrected observational data. A significant source of NO2 is biomass burning, which can be diagnosed by data of fire radiative power (FRP) from the Monitoring of Atmospheric Composition and Climate (MACC) reanalysis. We find a close relationship between high values of inferred NO2 surface concentrations and biomass burning for a large area which encompasses the departments of Caquetá, Meta, Guaviare, Vichada, and Putumayo.  相似文献   
79.
2013年世界硫黄市场处于供不应求的状态。全球各种形式硫产量7531万吨,同比增长4.2%。硫黄贸易量3100万吨,同比下降3.1%。2012年硫黄视消费量为5422.9万吨,同比增长4.4%。2013年全球硫黄价格呈下降趋势,近期开始上涨。  相似文献   
80.
The Junction gold deposit, in Western Australia, is an orogenic gold deposit hosted by a differentiated, iron‐rich, tholeiitic dolerite sill. Petrographic, microthermometric and laser Raman microprobe analyses of fluid inclusions from the Junction deposit indicate that three different vein systems formed at three distinct periods of geological time, and host four fluid‐inclusion populations with a wide range of compositions in the H2O–CO2–CH4–NaCl ± CaCl2 system. Pre‐shearing, pre‐gold, molybdenite‐bearing quartz veins host fluid inclusions that are characterised by relatively consistent phase ratios comprising H2O–CO2–CH4 ± halite. Microthermometry suggests that these veins precipitated when a highly saline, >340°C fluid mixed with a less saline ≥150°C fluid. The syn‐gold mineralisation event is hosted within the Junction shear zone and is associated with extensive quartz‐calcite ± albite ± chlorite ± pyrrhotite veining. Fluid‐inclusion analyses indicate that gold deposition occurred during the unmixing of a 400°C, moderately saline, H2O–CO2 ± CH4 fluid at pressures between 70 MPa and 440 MPa. Post‐gold quartz‐calcite‐biotite‐pyrrhotite veins occupy normal fault sets that slightly offset the Junction shear zone. Fluid inclusions in these veins are predominantly vapour rich, with CO2?CH4. Homogenisation temperatures indicate that the post‐gold quartz veins precipitated from a 310 ± 30°C fluid. Finally, late secondary fluid inclusions show that a <200°C, highly saline, H2O–CaCl2–NaCl–bearing fluid percolated along microfractures late in the deposit's history, but did not form any notable vein type. Raman spectroscopy supports the microthermometric data and reveals that CH4–bearing fluid inclusions occur in syn‐gold quartz grains found almost exclusively at the vein margin, whereas CO2–bearing fluid inclusions occur in quartz grains that are found toward the centre of the veins. The zonation of CO2:CH4 ratios, with respect to the location of fluid inclusions within the syn‐gold quartz veins, suggest that the CH4 did not travel as part of the auriferous fluid. Fluid unmixing and post‐entrapment alteration of the syn‐gold fluid inclusions are known to have occurred, but cannot adequately account for the relatively ordered zonation of CO2:CH4 ratios. Instead, the late introduction of a CH4–rich fluid into the Junction shear zone appears more likely. Alternatively, the process of CO2 reduction to CH4 is a viable and plausible explanation that fits the available data. The CH4–bearing fluid inclusions occur almost exclusively at the margin of the syn‐gold quartz veins within the zone of high‐grade gold mineralisation because this is where all the criteria needed to reduce CO2 to CH4 were satisfied in the Junction deposit.  相似文献   
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