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41.
42.
On the significance of CO2 inclusions in plagioclase microphenocrysts in tholeiite from Moeraki,New Zealand 总被引:1,自引:0,他引:1
Liquid plus vapour inclusions of CO2 are widespread in plagioclase microphenocrysts in small tholeiitic intrusions and tephra of the Moeraki and adjacent areas
of northeast Otago, New Zealand. They imply the presence of immiscible CO2 droplets in the magma at depths of about 7–14 km. Their presence within 5 μm of the edges of microphenocrysts as little as
35 μm thick and 118 μm long indicates minimal feldspar crystal growth during the final ascent and quenching of the magma.
Delicate branching clusters of lath-like microphenocrysts escaped disruption during this ascent. Such CO2 inclusions are a potential source of ‘excess argon’ perturbing K-Ar age determinations.
Received March 24, 1993/Accepted September 10, 1993 相似文献
43.
采用了单柱离子色谱法测MnO2产品中无机离子杂质;提出了消除干扰的可行途径,将La(OH)3加入后能同时消除进样峰的干扰和溶剂峰的出现。选用1.75mmol/L邻苯二甲酸1.75mmol/L三羟甲基氨基甲烷为混合淋洗剂测定F^-,Cl^-,NO3^和SO^2-4,其标准加入回收率为95%-105%;RSD(n=7)为2.47%-8.08%。 相似文献
44.
The biogeochemical sulfur cycle in the marine boundary layer over the Northeast Pacific Ocean 总被引:1,自引:0,他引:1
T. S. Bates J. E. Johnson P. K. Quinn P. D. Goldan W. C. Kuster D. C. Covert C. J. Hahn 《Journal of Atmospheric Chemistry》1990,10(1):59-81
The major components of the marine boundary layer biogeochemical sulfur cycle were measured simultaneously onshore and off the coast of Washington State, U.S.A. during May 1987. Seawater dimethylsulfide (DMS) concentrations on the continental shelf were strongly influenced by coastal upwelling. Concentration further offshore were typical of summer values (2.2 nmol/L) at this latitude. Although seawater DMS concentrations were high on the biologically productive continental shelf (2–12 nmol/L), this region had no measurable effect on atmospheric DMS concentrations. Atmospheric DMS concentrations (0.1–12 nmol/m3), however, were extremely dependent upon wind speed and boundary layer height. Although there appeared to be an appreciable input of non-sea-salt sulfate to the marine boundary layer from the free troposphere, the local flux of DMS from the ocean to the atmosphere was sufficient to balance the remainder of the sulfur budget. 相似文献
45.
46.
A. Waltrop S. K. Mitra A. I. Flossmann H. R. Pruppacher 《Journal of Atmospheric Chemistry》1991,12(1):1-17
An experimental study involving the Mainz vertical wind tunnel is described where the rate of SO2 removed from the air by freely suspended water drops was measured for SO2 concentrations in the gas phase ranging between 50 and 500 ppb, and for various H2O2 concentrations in the liquid phase. In a first set of experiments, the pH inside the SO2 absorbing drops was monitored by means of colour pH indicators added to the drops. In a second set of experiments, the amount of SO2 scavenged by the drops was determined as sulfate by an ionchromatograph after the drops had been removed from the vertical air stream of the wind tunnel after various times of exposure to SO2. The results of our experimental study were compared with the theoretical gas diffusion model of Walcek and Pruppacher which was reformulated for the case of SO2 concentrations in the ppbv(v) range for which the main resistance to diffusion lies in the gas phase surrounding the drop. Excellent agreement between experiment and theory was obtained. Encouraged by this agreement, the theory was used to investigate the rate of sulfate production inside a drop as a function of pH. The sulfate production rate, which includes transport and oxidation, was compared with the production rate based on bulk equilibrium, as cited in the literature. 相似文献
47.
The correlation between sulfate concentrations in Finnish headwater streams and atmospheric sulfate deposition has been studied by using data from the streamwater chemistry in August–September 1990 and computed S deposition from the anthropogenic emissions. The sulfate concentrations and acidity in water are interpolated and smoothed into a deposition model grid. These data are compared with geological and pedogeochemical (glacial till) background information. The areas where the streamwater SO4 concentrations are mainly controlled by either anthropogenic S deposition or sulfur in till is estimated by applying the fuzzy Gustafsson-Kessel algorithm, which provides a soft clustering suitable for overlapping control factors. Residual areas can be well explained by the SO4-rich Littorina clay deposits. The higher overall background SO4 concentrations in streams in south Finland compared with central and northern Finland are an indisputable consequence of the heavier S deposition load in the south. However, anthropogenic sulfur deposition has a clear correlation with the sulfates in streamwaters only in northeastern Lapland impacted by the large industrial emissions in the Kola Peninsula. The secondary sulfide and sulfate minerals of marine Littorina sediments are dominating sources in the broad coastal belts, as are the primary sulfide minerals locally in the Pori-Vammala area, at the eastern end of the main sulfide ore belt between Lake Ladoga and the Gulf of Bothnia, in the Outokumpu area, and in the Peräpohja and central Lapland schist belts. Consequently, in addition to the anthropogenic deposition, there are natural sources of sulfur which cause acidity of streamwaters. 相似文献
48.
49.
S. Madronich D. R. Hastie B. A. Ridley H. I. Schiff 《Journal of Atmospheric Chemistry》1984,1(2):151-157
The photodissociation coefficient, J
NO2 of NO2 in the atmosphere was calculated at 235 and 298 K using the measured temperature dependences of the absorption cross-sections and quantum yields. These calculations gave a ratio J
NO2(298 K)/J
NO2(235 K)=1.155±0.010 which is only weakly dependent on altitude, surface albedo and solar zenith angle. 相似文献
50.
Mean growing season soil PCO2 data were obtained for 19 regions of the world in nine countries. Bivariate and multiple linear regression analysis with soil log(PCO2) as the dependent variable and TEMP, PRECIP, log(AET), and log(PET) as the four climatic independent variables demonstrated that AET was the best independent predictor of soil PCO2. An improved soil PCO2-AET model was developed by assuming (1) that as AET approaches zero, soil PCO2 approaches the atmospheric value and (2) that there is an upper limit to soil PCO2 at very high AET. This model has the form log(PCO2) = ?3·47 + 2·09 (1 ?e?0·0172 AET) where AET is in mm. It explains 67 per cent of the initial variation in the soil PCO2 data, predicts a soil log(PCO2) of ? 3·47 at AET = 0, and an upper limit of 3·5 per cent (log(PCO2) = ? 1·45) for mean growing season soil PCO2 at AET values of 2000 mm and above. The results of this study suggest that soil PCO2 levels in tropical areas are, on average, higher than those in temperate, alpine, and arctic regions. 相似文献