卫星对地观测中大气与地表辐射贡献的参数化

卫星对地观测定量遥感地表与大气特性是当前地球科学与应用研究的关键手段之一。在定量遥感中区分大气和地表在地-气系统对空间散射辐射中各自的贡献与作用是关键的一步。这一问题的核心是基于辐射传输方程的数值计算建立起适合应用于遥感反演中分离大气与地表贡献的参数化表达式。本文对特定的气溶胶气候类型和可见/近红外波段建立起定量的表达形式,并对表达式的物理含义和拟合精度进行了分析。最后讨论了其应用的可行性和进一步的工作。     

Effects of geomagnetic activity on the mesospheric electric fields

The results of three series of rocket measurements of mesospheric electric fields carried out under different geomagnetic conditions at polar and high middle latitudes are analysed. The measurements show a clear dependence of the vertical electric fields on geomagnetic activity at polar and high middle latitudes. The vertical electric fields in the lower mesosphere increase with the increase of geomagnetic indexes K_p and K_p. The simultaneous increase of the vertical electric field strength and ion conductivity was observed in the mesosphere during geomagnetic disturbances. This striking phenomenon was displayed most clearly during the solar proton events of October, 1989 accompanied by very strong geomagnetic storm (K_p = 8+). A possible mechanism of generation of the vertical electric fields in the mesosphere caused by gravitational sedimentation of charged aerosol particles is discussed. Simultaneous existence in the mesosphere of both the negative and positive multiply charged aerosol particles of different sizes is assumed for explanation of the observed V/m vertical electric fields and their behaviour under geomagnetically disturbed conditions.Paper Presented at the Second IAGA/ICMA (IAMAS) Workshop on Solar Activity Forcing of the Middle Atmosphere, Prague, August 1997     

Nitrate in the atmospheric boundary layer of the tropical South Pacific: Implications regarding sources and transport

Weekly bulk aerosol samples collected at Funafuti, Tuvalu (8°30S, 179°12E), American Samoa (14°15S, 170°35W), and Rarotonga (21°15S, 159°45W), from 1983 through most of 1987 have been analyzed for nitrate and other constituents. The mean nitrate concentration is about 0.11 g m^–3 at each of these stations: 0.107±0.011 g m^–3 at Funafuti; 0.116±0.008 at American Samoa; and 0.117±0.010 at Rarotonga. Previous measurements of mineral aerosol and trace metal concentrations at American Samoa are among the lowest ever recorded for the near-surface troposphere and indicate that this region is minimally affected by transport of soil material and pollutants from the continents. Consequently, the nitrate concentration of 0.11 g m^–3 can be regarded as the natural level for the remote marine boundary layer of the tropical South Pacific Ocean. In contrast, over the tropical North Pacific which is significantly impacted by the transport of material from Asia and North America, the mean nitrate concentrations are about three times higher, 0.29 and 0.36 g m^–3 at Midway and Oahu, respectively. The major sources of the nitrate over the tropical South Pacific are still very uncertain. A very significant correlation between the nitrate concentrations at American Samoa and the concentrations of ²¹⁰Pb suggests that transport from continental sources might be important. This continental source could be lightning, which occurs most frequently over the tropical continents. A near-zero correlation with ⁷Be indicates that the stratosphere and upper troposphere are probably not the major sources. A significant biogenic source would be consistent with the higher mean nitrate concentrations, 0.16 to 0.17 g m^–3, found over the equatorial Pacific at Fanning Island (3°55N, 159°20W) and Nauru (0°32S, 166°57E). The lack of correlation between nitrate and nss sulfate at American Samoa does not necessarily preclude an important role for marine biogenic sources.     

Meteorology and haze structure during AGASP-II,Part 2: Canadian Arctic flights, 13–16 April 1986

In April 1986, a well-instrumented NOAA WP-3D research aircraft conducted three flights in the Canadian Arctic tied to the Canadian Atmospheric Environment Service baseline station in Alert, Northwest Territories. Two of the flights were coordinated with the National Aeronautical Establishment of Canada Twin Otter and the University of Washington C-131 research aircraft. The haze observed in the Canadian Arctic was well-aged and mixed throughout the troposphere in concentrations well below those observed during the previous weeks in the Alaskan Arctic. Over the ice, beneath the surface temperature inversion, ozone was generally depleted to near zero. Over the coast at Alert, there is evidence that topography and downslope winds reduce the strength of the inversion, thus allowing lower tropospheric gases and aerosols to mix down to the surface. At the top of the troposphere, an aerosol-depleted region was observed. In the lower stratosphere, aerosol concentrations were elevated above those observed in the troposphere.     

Features of the atmospheric cycle of aerosol trace elements and sulphur dioxide revealed by baseline observations in Canada

Selected applications of baseline aerosol, SO₂ and deposition chemistry observations in Canada are reviewed to illustrate how new insight can be gained into features of the atmospheric pathway of trace substances such as sources, transformation and removal. A strong annual variation in Arctic aerosol concentration is a manifestation of particle residence times that are much longer in winter than in summer. Differences in the variation of SO₄ ⁼ and V concentrations in the Arctic winter are due to SO₂ oxidation. The mean rate of oxidation between November and April ranges from 0.04 to 0.25%/h and is a minimum in December, January and February. Br measured on filters in the Arctic peaks in concentration later (March and April) than anthropogenic particulate matter suggesting photochemical production. Acidity in Arctic aerosol and in glacial ice are correlated. The relationship yields a best estimate of acidity in the absence of anthropogenic influences of 5.8 mole/l. Coincident air and precipitation measurements of sulphur oxides indicate that on average in eastern Canada 60% of SO₄ ⁼ in rain originates from SO₂ oxidation in the storm. Trends in Arctic ice core acidity and SO₂ emissions in Europe are similar, that is, little variation in the first half of the century and a marked increase since the mid 1950's. This is consistent with meteorological and chemical evidence linking Arctic air pollution with Eurasian sources.     

The Global Atmospheric Electrical Circuit and Climate

Evidence is emerging for physical links among clouds, global temperatures, the global atmospheric electrical circuit and cosmic ray ionisation. The global circuit extends throughout the atmosphere from the planetary surface to the lower layers of the ionosphere. Cosmic rays are the principal source of atmospheric ions away from the continental boundary layer: the ions formed permit a vertical conduction current to flow in the fair weather part of the global circuit. Through the (inverse) solar modulation of cosmic rays, the resulting columnar ionisation changes may allow the global circuit to convey a solar influence to meteorological phenomena of the lower atmosphere. Electrical effects on non-thunderstorm clouds have been proposed to occur via the ion-assisted formation of ultra-fine aerosol, which can grow to sizes able to act as cloud condensation nuclei, or through the increased ice nucleation capability of charged aerosols. Even small atmospheric electrical modulations on the aerosol size distribution can affect cloud properties and modify the radiative balance of the atmosphere, through changes communicated globally by the atmospheric electrical circuit. Despite a long history of work in related areas of geophysics, the direct and inverse relationships between the global circuit and global climate remain largely quantitatively unexplored. From reviewing atmospheric electrical measurements made over two centuries and possible paleoclimate proxies, global atmospheric electrical circuit variability should be expected on many timescales.     

Detection of marine aerosols with IRS P4-Ocean Colour Monitor

The atmospheric correction bands 7 and 8 (765nm and 865nm respectively) of the Indian Remote Sensing Satellite IRS P4-0CM (Ocean Colour Monitor) can be used for deriving aerosol optical depth (AOD) over the oceans. A retrieval algorithm has been developed which computes the AOD using band 7 data by treating the ocean surface as a dark background after removing the Rayleigh path radiance in the sensor-detected radiances. This algorithm has been used to detect marine aerosol distributions at different coastal and offshore locations around India. A comparison between OCM derived AOD and the NOAA operational AOD shows a correlation ∼0.92 while that between OCM derived AOD and the ground-based sun photometer measurements near the coast of Trivandrum shows a correlation of ∼0.90.     

有效辐射强迫的概念及其最新估值:IPCC AR6解读

依据政府间气候变化专门委员会 (IPCC) 第六次评估报告 (AR6) 第一工作组 (WGI) 报告第七章的内容,详细介绍了AR6最新定义的有效辐射强迫 (ERF)及其计算方法,并给出了自工业革命以来 (1750—2019年) 各气候辐射强迫因子ERF的最佳估值。根据AR6的最新评估,工业革命以来总人为ERF的估值为2.72 (1.96～3.48) W·m^-2,相较于AR5 估计结果 (1750—2011年) 增长了0.43 W·m^-2。2011年后温室气体浓度的增加及其辐射效率的修正是造成总人为ERF增加的主要原因。自工业革命以来温室气体浓度变化造成的ERF为3.84 (3.46～4.22) W·m^-2,二氧化碳仍然是其中的最大贡献因素 (56％±16％)。而气溶胶的总ERF (气溶胶-辐射相互作用 (ERFari) 与气溶胶-云相互作用 (ERFaci) 的总和) 为-1.1(-1.7～-0.4) W·m^-2,其中ERFari贡献20％～25％,ERFaci贡献接近75％～80％。AR6中气溶胶的总ERF的估算相较于AR5在数值上有所增加,而不确定性有所减少。但由于没有考虑部分重要的调整过程,ERFaci仍然存在较大的不确定性。     

Meso-scale effects of tropical deforestation in Amazonia: preparatory LBA modelling studies

As part of the preparation for the Large-Scale Biosphere Atmosphere Experiment in Amazonia, a meso-scale modelling study was executed to highlight deficiencies in the current understanding of land surface atmosphere interaction at local to sub-continental scales in the dry season. Meso-scale models were run in 1-D and 3-D mode for the area of Rondonia State, Brazil. The important conclusions are that without calibration it is difficult to model the energy partitioning of pasture; modelling that of forest is easier due to the absence of a strong moisture deficit signal. The simulation of the boundary layer above forest is good, above deforested areas (pasture) poor. The models’ underestimate of the temperature of the boundary layer is likely to be caused by the neglect of the radiative effects of aerosols caused by biomass burning, but other factors such as lack of sufficient entrainment in the model at the mixed layer top may also contribute. The Andes generate patterns of subsidence and gravity waves, the effects of which are felt far into the Rondonian area The results show that the picture presented by GCM modelling studies may need to be balanced by an increased understanding of what happens at the meso-scale. The results are used to identify key measurements for the LBA atmospheric meso-scale campaign needed to improve the model simulations. Similar modelling studies are proposed for the wet season in Rondonia, when convection plays a major role.     

Mountain wave motions determined by the Esrange MST radar

A European campaign of ground-based radar, lidar and optical measurements was carried out during the winter of 1996/1997 (28 December–2 February) to study lee waves in the northern part of Scandinavia. The participants operated ozone lidars, backscatter lidars and MST radars at ALOMAR/Andoya and Esrange/Kiruna, and an ALIS imaging system in Kiruna. The Andoya site was generally windward of the Scandinavian mountains, the Kiruna site on the leeward side. The goal of the experiment was to examine the influence of lee waves on the formation of Polar Stratospheric Clouds (PSCs). This paper studies the radar data from MST-radar ESRAD located at Esrange [68.°N, 21.°E], i.e. in the lee of the mountains. We present three cases where strong lee waves were observed: in one case they propagated upwards to the lower stratosphere and in the other two cases they were trapped or absorbed in the troposphere. We examine the local waves and the direction and strength of the local wind using the radar, the synoptic meteorological situation using weather maps (European Meteorological Bulletin) and the synoptic stratospheric temperatures using ECMWF data. We observed that waves propagate up to the stratosphere during frontal passages. When anticyclonic ridges are present, the propagation to the stratosphere is very weak. This is due to trapping of the waves at or below the tropopause. We also show that the radar data alone can be used to characterise the different weather conditions for the three cases studied (through the variation of the height of the tropopause). The synoptic stratospheric temperatures in the three cases were similar, and were above the expected threshold for PSC formation. Lidar and visual observation of PSCs and nacreous clouds, respectively, showed that these were present only in the case when the lee waves propagated up to the lower stratosphere.