Aerosol polarized phase function and single-scattering albedo retrieved from ground-based measurements

Aerosol optical parameters, polarized phase function and single-scattering albdeo, have been retrieved from ground-based sun photometer measurements in Beijing 2003. The measured aerosol optical thickness varies from 0.12 to 0.77 with an average value of 0.39. The measured Ångström coefficient ranges from 0.75 to 1.47 with an average value of 1.21. The retrieved single-scattering albedo at 870 nm is within the 0.76–0.94 range and the average value is 0.85, suggests there are considerable aerosol absorptions in Beijing. The maximum value of retrieved polarized phase function at 870 nm ranges from 0.068 to 0.225 with an average value of 0.16, and it illustrates good correlations with the Ångström coefficient, i.e. the relative size of aerosol particles. Analyses of measurements and theoretical calculations show the polarized phase function is sensitive to aerosol size distribution and complex refractive index, especially the imaginary part of the refractive index which denotes aerosol light absorbing effects. These results suggest that the polarized phase function is an effective and unique aerosol optical parameter and is able to improve the retrieval of aerosol physical properties.     

冷岛效应的分析解

本文将冷岛视为一个负的扰动加热源,即冷源,用小扰动方法求出了冷岛效应的分析解,给出了解例,并与热岛效应的结果作了对比分析。     

1999年与2003年我国北方地区夏季气温异常原因初探

分析了1999年与2003年我国北方地区夏季气温的变化特点和同期大气环流主要特征。结果表明:中国夏季气温变化有明显的年代际特征,这一特征与亚洲上空大气环流的年代际变化紧密相关,表明我国北方地区夏季气温异常一个很重要的原因或许是缘于气候年代际变化。2003年夏季中高纬环流形势呈两槽两脊的配置,与近十几年气候态分布刚好相反,因而从气候年代际变化的特征来看,2003年为预示年代际气候转型的征兆。     

An asynchronous Geoprocessing Workflow and its application to an Antarctic ozone monitoring and mapping service

The integration of Sensor Web Enablement services with other Open Geospatial Consortium (OGC) Web Services as Geospatial Processing Workflows (GPW) is essential for future Sensor Web application scenarios. With the help of GPW technology, distributed and heterogeneous OGC Web Services can be organized and integrated as compound Web Service applications that can direct complicated earth observation tasks. Under the Sensor Web environment, asynchronous communications between Sensor Web Services are common. We have proposed an asynchronous GPW architecture for the integration of Sensor Web Services into a Web Service Business Process Execution Language workflow technology. We designed a Sensor Information Accessing and Processing workflow, an asynchronous GPW instance, to take an experiment of observing and mapping ozone over Antarctica. Based on our results, our proposed asynchronous workflow method shows the advantages of taking environmental monitoring and mapping tasks.     

A modeling study of effective radiative forcing and climate response due to tropospheric ozone

This study simulates the effective radiative forcing(ERF) of tropospheric ozone from 1850 to 2013 and its effects on global climate using an aerosol–climate coupled model, BCC AGCM2.0.1 CUACE/Aero, in combination with OMI(Ozone Monitoring Instrument) satellite ozone data. According to the OMI observations, the global annual mean tropospheric column ozone(TCO) was 33.9 DU in 2013, and the largest TCO was distributed in the belts between 30°N and 45°N and at approximately 30°S; the annual mean TCO was higher in the Northern Hemisphere than that in the Southern Hemisphere;and in boreal summer and autumn, the global mean TCO was higher than in winter and spring. The simulated ERF due to the change in tropospheric ozone concentration from 1850 to 2013 was 0.46 W m~(-2), thereby causing an increase in the global annual mean surface temperature by 0.36℃, and precipitation by 0.02 mm d~(-1)(the increase of surface temperature had a significance level above 95%). The surface temperature was increased more obviously over the high latitudes in both hemispheres, with the maximum exceeding 1.4?C in Siberia. There were opposite changes in precipitation near the equator,with an increase of 0.5 mm d~(-1)near the Hawaiian Islands and a decrease of about-0.6 mm d~(-1)near the middle of the Indian Ocean.     

相对湿度和PM2.5浓度对大气能见度的影响研究:基于小时资料的多站对比分析

为了全面分析浙江省不同区域能见度变化基本特征及影响机理,基于杭州、宁波、温州3个国家基本气象站2013-2014年逐时能见度观测资料,比较分析了3市能见度变化的基本特征。发现3市不同等级能见度出现频率基本一致,随着能见度等级的提高,出现频率逐渐降低;从能见度的日变化来看,07时（北京时）前后最低,之后缓慢上升,14-15时达到最高,随后逐渐下降;全年有两个能见度较低时段,分别出现在12月-次年2月和5-6月;总体而言,宁波能见度最优,杭州和温州大体相当。功率谱分析结果表明,3市能见度均有显著的日周期,高频波段呈现出多个显著谱峰,低频波段存在若干显著谱峰。进一步开展机理分析,发现相对湿度和PM_2.5浓度是调制大气能见度的关键因子,相对湿度增大、PM_2.5浓度升高导致能见度降低。在同一相对湿度等级下,初始阶段能见度随PM_2.5浓度的升高迅速降低,到达“拐点”之后降低速率趋于缓慢。在同一PM_2.5浓度水平下,相对湿度越大,能见度越低,说明水汽对能见度也有重要影响。基于相对湿度和PM_2.5浓度两个因子,采用非线性拟合方案构建了大气能见度定量统计模型,总体而言模型拟合效果较好。最后针对研究中存在的不足和未来值得进一步发掘的科学问题进行了讨论。     

中国中东部冬季霾日的形成与东亚冬季风和大气湿度的关系

利用1961-2013年中国地面台站长期观测资料和同期NCEP/NCAR再分析资料,以华北、江淮和华南为研究区,分析了中国中东部冬季霾日的形成与东亚冬季风以及大气湿度的关系。结果表明:(1)冬季霾日与东亚冬季风强度成显著的负相关。首先,东亚冬季风强度的减弱使得地面风速减小,进而导致冬季霾日增多。其中,华北7-8 m/s最大风速日数和江淮6-8 m/s最大风速日数的减少,及华南≤2 m/s最大风速日数的增多对各区冬季霾日的增多作用较大。其次,东亚冬季风减弱引起冬季气温的持续升高,易导致冬季霾日的增多,这在华北地区较之在江淮和华南更为明显。(2)由于气候变暖,冬季气温升高,使得近地面相对湿度减小。在江淮和华南地区,冬季霾日的增多与近地面相对湿度的减小显著相关,而在华北地区这种相关较弱。(3)冬季气温升高也有利于大气层结稳定度的增强,3个区域冬季霾日的增多均与大气层结稳定度的增强显著相关,特别是与对流层中低层(850-500 hPa)大气饱和度的降低显著相关。(4)冬季霾日数变化与区域水汽输送关系密切。其中,华北地区的冬季霾日数与水汽总收入成显著正相关,江淮地区与纬向水汽收入成显著正相关,与经向水汽收入成显著负相关,华南地区与经向水汽收入成显著负相关。     

卫星臭氧资料的发展与应用

随着卫星探测技术的进步、天气学和气候学理论的不断完善,以及高性能计算机广泛应用,卫星臭氧资料的种类得到极大丰富并被应用到多个研究领域中,取得了一系列重要成果。文中介绍了主要星载臭氧探测仪的发展概况,回顾了卫星臭氧资料在气象领域的应用研究成果,主要包括卫星臭氧资料在气旋或低压过程中、全球或区域臭氧的气候分布及变化特征、高原臭氧分布及变化特点、数值应用等方面的应用研究,并展望了卫星臭氧资料研究的未来发展趋势。      

无锡梅雨期湿沉降综合分析

利用2008—2014年梅雨期间酸雨观测资料及2014年6月16—27日降水个例加密采样资料,结合大气污染物资料分析了近7 a无锡梅雨期酸雨特征,研究降水过程中空气污染物、p H值、电导率的变化及降水对污染物的清除作用。结果表明:无锡市梅雨期酸雨年平均p H值呈现逐年递增趋势。降水过程中,颗粒物质量浓度显著降低;气体浓度变化受其自身日变化及排放源影响大于雨水的清除作用;样品的p H值、K值每个过程变化并不一致,K值变化与颗粒物质量浓度变化大致保持一致。降水、风对颗粒物质量浓度影响大于对气体浓度的影响。长时间连续降水时,降水对颗粒污染物的清除存在极限。小时雨量在0~0.5 mm时,降水对颗粒物浓度做负清除,其值反而略有增加;小时雨量在0.6~5.0 mm时,降水对颗粒物质量浓度做正清除;小时雨量达到5.1 mm及以上时,对PM_(2.5)和PM_(2.5-10)做正清除,对PM_(10)做负清除。降水对SO_2有稀释清除作用;对NO_2的稀释作用取决于其开始浓度值;对CO、O_3的清除作用不显著。     

同化FY3B/IRAS资料对GRAPES分析场影响诊断

GRAPES(Globe and Regional Assimilation and Prediction System)变分系统能够同化常规资料和非常规卫星资料,这些被同化的资料究竟对同化系统得到的分析场有何影响,目前国内外尚未见相关的研究文献。为此,首次采用基于信息熵信号自由度思想,诊断风云三号B星(FY3B)红外分光计(Infrared Atmospheric Sounder,IRAS)资料对GRAPES分析场的影响。诊断过程中,采用数值逼近方法,统计2012年12月24日18时到2013年1月22日00时共114个时次IRAS资料对GRAPES分析场影响,结果表明,IRAS中高层通道亮温资料对GRAPES分析场影响比地表通道20观测亮温的影响大,地表通道8和9观测亮温对分析场影响较大。前24个GRAPES变分同化时次每个时次IRAS通道亮温对分析场影响的贡献率分析结果显示,高层通道和H_2O通道贡献率较大。个例分析结果表明,在同化探空资料基础上加入IRAS资料后,温度和湿度增量场变化幅度较大,表明IRAS资料对分析场有降温和增湿作用。