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81.
Formation of Carbon and Hydrogen Species in Magmas at Low Oxygen Fugacity   总被引:5,自引:0,他引:5  
Studies of iron-bearing silicate melt (ferrobasalt) + iron metallicphase + graphite + hydrogen equilibria show that carbon andhydrogen solubilities in melts are important for the evolutionof the upper mantle. In a series of experiments conducted at3·7 GPa and 1520–1600°C, we have characterizedthe nature (oxidized vs reduced) and quantified the abundancesof C- and H-compounds dissolved in iron-bearing silicate melts.Experiments were carried out in an anvil-with-hole apparatuspermitting the achievement of equal chemical potentials of H2in the inner Pt capsule and outer furnace assembly. The fO2for silicate melt–iron equilibrium was 2·32 ±0·04 log units below iron–wüstite (IW). Theferrobasalt used as starting material experienced a reductionof its iron oxides and silicate network. The counterpart wasa liberation of oxygen reacting with the hydrogen entering thecapsule. The amount of H2O dissolved in the glasses was measuredby ion microprobe and by step-heating and was found to be between1 and 2 wt %. The dissolved carbon content was found to be 1600ppm C by step-heating. The speciation of C and H componentswas determined by IR and Raman spectroscopy. It was establishedthat the main part of the liberated oxygen was used to formOH and to a much lesser extent H2O, and only traces ofH2, CO2 and  相似文献   
82.
Abstract. Primary fluid inclusions in quartz and carbonates from the Kanggur gold deposit are dominated by aqueous inclusions, with subsidiary CO2-H2O inclusions that have a constant range in CO2 content (10–20 vol %). Microthermometric results indicate that total homogenization temperatures have a wide but similar range for both aqueous inclusions (120 to 310C) and CO2-H2O inclusions (140 to 340C). Estimates of fluid salinity for CO2-H2O inclusions are quite restricted (5.9∼10.3 equiv. wt% NaCl), whereas aqueous inclusions show much wider salinity ranging from 2.2 to 15.6 equivalent wt %NaCl.
The 6D values of fluid inclusions in carbonates vary from -45 to -61 %, in well accord with the published δD values of fluid inclusions in quartz (-46 to -66 %). Most of the δ18O and δD values of the ore-forming fluids can be achieved by exchanged meteoric water after isotopic equilibration with wall rock by fluid/rock interaction at a low water/rock ratio. However, the exchanged meteoric water alone cannot explain the full range of δ18O and δD values, magmatic and/or meta-morphic water should also be involved. The wide salinity in aqueous inclusions may also result from mixing of meteoric water and magmatic and/or metamorphic water.  相似文献   
83.
This paper outlines an interdisciplinary project on recent environmental change and atmospheric contamination on the high Arctic archipelago of Svalbard (76°30′N–80°30′N). It describes the rationale and aims of the project and summarises the location, climate, geology, vegetation, and land-use of Svalbard.  相似文献   
84.
Abstract The Solund‐Stavfjord ophiolite complex (SSOC) in western Norway represents a remnant of the Late Ordovician oceanic lithosphere, which developed in an intermediate‐ to fast‐spreading Caledonian back‐arc basin. The internal architecture and magmatic features of its crustal component suggest that the SSOC has a complex, multistage sea floor spreading history in a supra‐subduction zone environment. The youngest crustal section associated with the propagating rift tectonics consists of a relatively complete ophiolite pseudostratigraphy, including basaltic volcanic rocks, a transition zone between the sheeted dyke complex and the extrusive sequence, sheeted dykes, and high‐level isotropic gabbros. Large‐scale variations in major and trace element distributions indicate significant remobilization far beyond that which would result from magmatic processes, as a result of the hydrothermal alteration of crustal rocks. Whereas K2O is strongly enriched in volcanic rocks of the extrusive sequence, Cu and Zn show the largest enrichment in the dyke complex near the dyke–volcanic transition zone or within this transition zone. The δ18O values of the whole‐rock samples show a general depletion structurally downwards in the ophiolite, with the largest and smallest variations observed in volcanic rocks and the transition zone, respectively. δ18O values of epidote–quartz mineral pairs indicate 260–290°C for volcanic rocks, 420°C for the transition zone, 280–345°C for the sheeted dyke complex and 290–475°C for the gabbros. The 87Sr/86Sr isotope ratios show the widest range and highest values in the extrusive rocks (0.70316–0.70495), and generally the lowest values and the narrowest range in the sheeted dyke complex (0.70338–0.70377). The minimum water/rock ratios calculated show the largest variations in volcanic rocks and gabbros (approximately 0–14), and generally the lowest values and range in the sheeted dyke complex (approximately 1–3). The δD values of epidote (?1 to ?12‰), together with the δ18O calculated for Ordovician seawater, are similar to those of present‐day seawater. Volcanic rocks experienced both cold and warm water circulation, resulting in the observed K2O‐enrichment and the largest scatter in the δ18O values. As a result of metal leaching in the hot reaction zone above a magma chamber, Zn is strongly depleted in the gabbros but enriched in the sheeted dyke complex because of precipitation from upwelling of discharged hydrothermal fluids. The present study demonstrates that the near intact effect of ocean floor hydrothermal activity is preserved in the upper part of the SSOC crust, despite the influence of regional lower greenschist facies metamorphism.  相似文献   
85.
Haloxylon ammodendron is a desert shrub used extensively in China for restoring degraded dry lands. An understanding of the water source used by H. ammodendron plantations is critical achieving sustainable vegetation restoration. We measured mortality, shoot size, and rooting depth in 5‐, 10‐, 20‐, and 40‐year‐old H. ammodendron plantations. We examined stable isotopic ratios of oxygen (δ18O) in precipitation, groundwater, and soil water in different soil layers and seasons, and in plant stem water to determine water sources at different shrub ages. We found that water acquisition patterns in H. ammodendron plantations differed with plantation age and season. Thus, the main water source for 5‐year‐old shrubs was shallow soil water. Water sources of 10‐year‐old shrubs shifted depending on the soil water conditions during the season. Although their tap roots could absorb deep soil water, the plantation main water sources were from soil water, and about 50% of water originated from shallow and mid soil. This pattern might occur because main water sources in these plantations were changeable over time. The 20‐ and 40‐year‐old shrubs acquired water mainly from permanent groundwater. We conclude that the main water source of a young H. ammodendron plantation was soil water recharged by precipitation. However, when roots reached sufficient depth, water originated mainly from the deep soil water, especially in the dry season. The deeply rooted 20‐ and 40‐year‐old shrubs have the ability to exploit a deep and reliable water source. To achieve sustainability in these plantations, we recommend a reduction in the initial density of H. ammodendron in the desert‐oasis ecotone to decelerate the consumption of shallow soil water during plantation establishment.  相似文献   
86.
This paper presents a novel triple‐layer model, called VART DO‐3L, for simulation of spatial variations in dissolved oxygen (DO) in fine‐grained streams, characterized by a fluid mud (fluff or flocculent) layer (an advection‐dominated storage zone) as the interface between overlying stream water and relatively consolidated streambed sediment (a diffusion‐dominated storage zone). A global sensitivity analysis is conducted to investigate the sensitivity of VART DO‐3L model input parameters. Results of the sensitivity analysis indicate that the most sensitive parameter is the relative size of the advection‐dominated storage zones (As/A), followed by a lumped reaction term (R) for the flocculent layer, biological reaction rate (μo) in diffusive layer and biochemical oxygen demand concentration (L) in water column. In order to address uncertainty in model input parameters, Monte Carlo simulations are performed to sample parameter values and to produce various parameter combinations or cases. The VART DO‐3L model is applied to the Lower Amite River in Louisiana, USA, to simulate vertical and longitudinal variations in DO under the cases. In terms of longitudinal variation, the DO level decreases from 7.9 mg l at the Denham Springs station to about 2.89 mg l?1 at the Port Vincent station. In terms of vertical variation, the DO level drops rapidly from the overlying water column to the advection‐dominated storage zone and further to the diffusive layer. The DO level (CF) in the advective layer (flocculent layer) can reach as high as 40% of DO concentration (C) in the water column. The VART DO‐3L model may be applied to similar rivers for simulation of spatial variations in DO level. Copyright © 2014 John Wiley & Sons, Ltd.  相似文献   
87.
Isotope data of precipitation and groundwater in parts of the Voltaian Basin in Northern Ghana were used to explain the groundwater recharge regime in the area. Groundwater recharge is an important parameter in the development of a decision support system for the management and efficient utilization of groundwater resources in the area. It is therefore important to establish the processes and sources of groundwater recharge. δ18O and δ2H data for local precipitation suggest enrichment relative to the Global Meteoric Water Line (GMWL) and indicate that precipitation takes place at a relative humidity less than 100%. The groundwater data plot on an evaporation line with a slope of 5, suggesting a high degree of evaporative enrichment of the precipitation in the process of vertical infiltration and percolation through the unsaturated zone into the saturated zone. This finding is consistent with the observation of high evapotranspiration rates in the area and ties in with the fact that significant clay fraction in the unsaturated zone limits vertical percolation and thus exposes the percolating rainwater to the effects of high temperatures and low humidities resulting in high evapotranspiration rates. Groundwater recharge estimates from the chloride mass balance, CMB, method suggest recharge in the range of 1.8–32% of the annual average precipitation in the form of rainfall. The highest rates are associated with areas where open wells encourage significant amount of groundwater recharge from precipitation in the area. In the northern parts of the study area, groundwater recharge is lower than 12%. The recharge so computed through the application of the CMB methodology takes on a spatial distribution akin to the converse of the spatial pattern of both δ18O and δ2H in the area. As such, the locations of the highest recharge are associated with the most depleted values of the two isotopes. This observation is consistent with the assertion that low vertical hydraulic conductivities slow down vertical percolation of precipitation down to the groundwater water. The percolating precipitation water thus gets enriched in the heavier isotopes through high evapotranspiration rates. At the same time, the amount of water that finally reaches the water table is considerably reduced. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   
88.
Soil moisture is essential for vegetation restoration in arid and semi-arid regions. Ascertaining the vertical distribution and transportation of soil moisture under different vegetation types has a profound effect on the ecological construction. In this study, the soil moisture at a depth of 500 cm for four typical vegetation types, including Robinia pseudoacacia, Caragana korshinskii, Stipa bungeana, and corn, were investigated and compared in the Zhifanggou watershed of the Loess plateau. Additionally, hydrogen and oxygen stable isotopes were detected to identify the transport mechanism of soil moisture. The results showed vertical distribution and transportation of soil moisture were different under different vegetation types. Depth-averaged soil moisture under S. bungeana and corn generally increased along the profile, while C. korshinskii and R. pseudoacacia showed weakly increasing and relatively stable after an obvious decreasing trend (0–40 cm). The soil moisture under R. pseudoacacia was lower than that under other vegetation types, especially in deep layer. However, the effect of R. pseudoacacia on soil moisture in the topsoil (< 30 cm) could be positive. For R. pseudoacacia (160–500 cm), C. korshinskii (0–500 cm), and S. bungeana (0–100 cm), the soil moisture declined with increased in vegetation age. Planting arbor species such as R. pseudoacacia intensified the decline of soil moisture on the Loess Plateau. The capacity of evaporation fractionation of soil moisture followed the sequence: corn > S. bungeana > R. pseudoacacia > C. korshinskii. The δ18O values in soil water fluctuated across the profile. The δ18O values changed sharply in upper layer and generally remained stable in deep layer. However, in middle layer, the vertical distribution characteristics of the δ18O values were different under different vegetation types. We estimated that piston flow was the main mode of precipitation infiltration, and the occurrence of preferential flow was related to vegetation types. These results were helpful to improve the understanding of the response of deep soil moisture to vegetation restoration and inform practices for sustainable water management.  相似文献   
89.
In situ analysis of a garnet porphyroblast from a granulite facies gneiss from Sør Rondane Mountains, East Antarctica, reveals discontinuous step‐wise zoning in phosphorus and large δ18O variations from the phosphorus‐rich core to the phosphorus‐poor rim. The gradually decreasing profile of oxygen isotope from the core (δ18O = ~15‰) to the rim (δ18O = ~11‰) suggests that the 18O/16O zoning was originally step‐wise, and modified by diffusion after the garnet rim formation at ~800°C and 0.8 GPa. Fitting of the 18O/16O data to the diffusion equation constrains a duration of the high‐T event (~800°C) to c. 0.5–40 Ma after the garnet rim formation. The low δ18O value of the garnet rim, together with the previously reported low δ18O values in metacarbonates, indicates regional infiltration, probably along a detachment fault, of low δ18O fluid/melt possibly derived from meta‐mafic to ultramafic rocks.  相似文献   
90.
Stable isotopes in precipitation are useful tracers to strengthen understanding of climate change and hydrological processes. In this study, the moisture sources of 190 precipitation events in Beijing were analysed using the Hybrid Single‐particle Lagrangian Integrated Trajectory model, based on which we studied the relation between variations in precipitation δ18O and dynamics in moisture sources and atmospheric circulation in seasonal and interannual timescales. Categorization of 7 groups of moisture sources was performed, among which oceanic moisture sources presented lower δ18O in precipitation than continental moisture sources. The results show that seasonal variations of precipitation δ18O were caused by changes of moisture sources. In summer, moisture from proximal oceans dominated vapour transport to Beijing due to increasing monsoon strength and resulted in a relatively small variation of precipitation δ18O. At the interannual timescale, the variations of δ18O in summer precipitation were related to dynamics in oceanic moistures, showing depleted values when the contribution of oceanic moistures, especially the proportion of long‐distance oceanic moisture, was high. Further analysis indicated that changes of oceanic moisture sources were controlled by the strength of summer monsoons. These findings address the complexity of moisture sources in midlatitude monsoon areas and suggest that isotopic signals in precipitation have the potential to deduce changes in moisture sources and atmospheric circulation and can therefore serve for palaeoclimate reconstruction.  相似文献   
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